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Using a recently obtained (general) formula for the interaction energy between an excited and a ground-state atom (Sherkunov Y 2007 Phys. Rev. A 75 012705), we consider the interaction energy between two such atoms near the interface…

Quantum Physics · Physics 2008-04-10 Marin-Slobodan Tomas

A quantum electrodynamic calculation of the interaction of an excited-state atom with a ground-state atom is performed. For an excited reference state and a lower-lying virtual state, the contribution to the interaction energy naturally…

Quantum Physics · Physics 2017-05-19 U. D. Jentschura , V. Debierre

In this paper we employ the hydrodynamic formulation of time-dependent density functional theory to obtain the van der Waal coefficients $C_{6}$ and $C_{8}$ of alkali-metal clusters of various sizes including very large clusters. Such…

Atomic and Molecular Clusters · Physics 2007-05-23 Arup Banerjee , Manoj K. Harbola

Exchange-correlation functionals with corrections for van der Waals interactions (PBE-D2, PBE-D3, PBE-D3(BJ), PBE-TS, optPBE-vdW and vdW-DF2) are tested for graphene and hexagonal boron nitride, both in the form of bulk and bilayer. The…

Mesoscale and Nanoscale Physics · Physics 2018-08-22 Irina V. Lebedeva , Alexander V. Lebedev , Andrey M. Popov , Andrey A. Knizhnik

The recently developed method combining the configuration interaction and the coupled-cluster method was demonstrated to provide accurate treatment of correlation corrections in divalent atomic systems [M.S.Safronova, M.G.Kozlov, and…

Atomic Physics · Physics 2013-06-12 S. G. Porsev , M. S. Safronova , M. G. Kozlov

We have computed the widely neglected first-order interaction between neutral atoms. At interatomic separations typical of condensed media, it is nearly equal to the 1/r^6 second-order London energy inferred from interactions in gasses. Our…

Biomolecules · Quantitative Biology 2007-07-01 Kevin Cahill , V. Adrian Parsegian

The dynamic electric dipole polarizability function for the magnesium atom is formed by assembling the atomic electric dipole oscillator strength distribution from combinations of theoretical and experimental data for resonance oscillator…

Atomic Physics · Physics 2015-08-28 James F. Babb

We employ the closed-shell perturbed relativistic coupled-cluster (RCC) theory developed by us earlier [Phys. Rev. A {\bf 77}, 062516 (2008)] to evaluate the ground state static electric dipole polarizabilities (\alpha s) of several atomic…

Atomic Physics · Physics 2013-12-09 Yashpal Singh , B. K. Sahoo , B. P. Das

We report on the analysis of FM selective reflection experiments on the 6S1/2->8P3/2 transition of Cs at 388 nm, and on the measurement of the surface van der Waals interaction exerted by a sapphire interface on Cs(8P3/2). Various…

We present an estimate of the nuclear electric polarizability of the 6He halo nucleus based on six-body microscopic calculations. Wave functions are obtained from semi-realistic two-body interactions using the hyperspherical harmonics…

Nuclear Theory · Physics 2015-06-11 Raymond Goerke , Sonia Bacca , Nir Barnea

We introduce a class of variational wavefunctions that capture the long-range interaction between neutral systems (atoms and molecules) without changing the diagonal of the density matrix of each monomer. The corresponding energy…

Chemical Physics · Physics 2019-03-26 Derk P. Kooi , Paola Gori-Giorgi

The electric dipole polarizabilities of $^3$H, $^3$He, and $^4$He are calculated directly using the Schr\"odinger equation with the latest generation of two- and three-nucleon interactions. These polarizabilities are necessary in order to…

Nuclear Theory · Physics 2010-05-27 I. Stetcu , S. Quaglioni , J. L. Friar , A. C. Hayes , P. Navrátil

We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that beam velocity can be determined with a precision below 1 \% using matter-wave interferometry. The profile…

Atomic Physics · Physics 2021-09-22 J Morley , R. Flack , B. J. Hiley , P. F. Barker

Within the frame of macroscopic quantum electrodynamics in causal media, the van der Waals interaction between an atomic system and an arbitrary arrangement of dispersing and absorbing dielectric bodies including metals is studied. It is…

Quantum Physics · Physics 2007-05-23 Stefan Yoshi Buhmann , Ho Trung Dung , Dirk-Gunnar Welsch

We estimate polarizabilities of atoms in molecules without electron density, using a Voronoi tesselation approach instead of conventional density partitioning schemes. The resulting atomic dispersion coefficients are calculated, as well as…

Chemical Physics · Physics 2015-08-31 Tristan Bereau , O. Anatole von Lilienfeld

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

Different computational methods are employed to evaluate elastic (rotationally summed) integral and differential cross sections for low energy (below about 10 eV) positron scattering off gas-phase C$_2$H$_2$ molecules. The computations are…

Chemical Physics · Physics 2009-11-13 J. Franz , F. A. Gianturco , K. L. Baluja , J. Tennyson , R. Carey , R. Montuoro , R. R. Lucchese , T. Stoecklin

We construct a new Skyrme interaction Sk$\chi$m$^*$ by fitting the equation of state and nucleon effective masses in asymmetric nuclear matter from chiral two- and three-body forces as well as the binding energies of finite nuclei.…

Nuclear Theory · Physics 2018-01-17 Zhen Zhang , Yeunhwan Lim , Jeremy W. Holt , Che Ming Ko

We formulate an adiabatic connection for the exchange-correlation energy in terms of pairing matrix fluctuation. This connection opens new channels for density functional approximations based on pairing interactions. Even the simplest…

Chemical Physics · Physics 2015-06-16 Helen van Aggelen , Yang Yang , Weitao Yang

By explicitly including fractionally ionic contributions to the polarizability of a many-component system we are able to significantly improve on previous atom-wise many-body van der Waals approaches with essentially no extra numerical…

Chemical Physics · Physics 2017-03-28 Tim Gould , Sébastien Lebègue , János G. Ángyán , Tomáš Bučko