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The long-range part of the interatomic interactions plays a substantial role in the collisional dynamics of ultracold gases. Here, we report on the calculation of the isotropic and anisotropic $C_6$ coefficients characterizing the van der…

Atomic Physics · Physics 2024-01-24 Klaudia Zaremba-Kopczyk , Michał Tomza , Maxence Lepers

The van der Waals coefficients for the alkali-metal atoms from Na to Fr interacting in their ground states, are calculated using relativistic ab initio methods. The accuracy of the calculations is estimated by also evaluating atomic static…

Atomic Physics · Physics 2007-05-23 A. Derevianko , W. R. Johnson , M. S. Safronova , J. F. Babb

We present semiempirical calculations of long-range van der Waals interactions for two interacting metastable rare-gas atoms Ne through Xe. Dispersion coefficients $C_6$ are obtained for homonuclear molecular potentials asymptotically…

Atomic Physics · Physics 2009-11-06 A. Derevianko , A. Dalgarno

The efficiency of optical trapping of ultracold atoms depend on the atomic dynamic dipole polarizability governing the atom-field interaction. In this article, we have calculated the real and imaginary parts of the dynamic dipole…

Atomic Physics · Physics 2017-04-11 Hui Li , Jean-Francois Wyart , Olivier Dulieu , Sylvain Nascimbene , Maxence Lepers

By inferring the dynamic permittivity of different material media from the observations and calculating dynamic electric dipole polarizabilties of the Li through Cs alkali atoms, precise values of $C_3$ coefficients were estimated in Phys.…

Atomic Physics · Physics 2023-10-02 Harpreet Kaur , Vipul Badhan , Bindiya Arora , B. K. Sahoo

We calculate pair potential curves for interacting Rydberg atoms in a constant electric field and use them to determine the effective $C_3$ dipole-dipole and $C_6$ van der Waals coefficients. We compare the $C_3$ and $C_6$ with experiments…

Positronium (Ps) scattering by noble-gas atoms (He, Ne, Ar, Kr, and Xe) is studied in the frozen-target approximation and with inclusion of the van der Waals interaction. Single-particle electron and positron states in the field of the…

Atomic Physics · Physics 2018-01-23 A. R. Swann , G. F. Gribakin

A local approximation for dynamic polarizability leads to a nonlocal functional for the long-range dispersion interaction energy via an imaginary-frequency integral. We analyze several local polarizability approximations and argue that the…

Chemical Physics · Physics 2015-03-17 Oleg A. Vydrov , Troy Van Voorhis

Apropos to the growing interest in the study of long-range interactions which for their applications in cold atom physics, we have performed theoretical calculation for the two-dipole $C_6$ and three-dipole $C_9$ dispersion coefficients…

Atomic Physics · Physics 2020-08-12 Neelam Shukla , Bindiya Arora , Lalita Sharma , Rajesh Srivastava

A method for determination of atomic dipole matrix elements of principal transitions from the value of dispersion coefficient C_6 of molecular potentials correlating to two ground-state atoms is proposed. The method is illustrated on atomic…

Atomic Physics · Physics 2009-11-07 Andrei Derevianko

Relativistic many-body calculations of van der Waals coefficients C_6 for dimers correlating to two ground state alkaline-earth atoms at large internuclear separations are reported. The following values and uncertainties were determined :…

Atomic Physics · Physics 2009-11-07 Sergey Porsev , Andrei Derevianko

Largely motivated by a number of applications, the van der Waals dispersion coefficients ($C_3$s) of the alkali ions (Li$^+$, Na$^+$, K$^+$ and Rb$^+$), the alkaline-earth ions (Ca$^+$, Sr$^+$, Ba$^+$ and Ra$^+$) and the inert gas atoms…

Atomic Physics · Physics 2015-09-16 Kiranpreet Kaur , Bindiya Arora , B. K. Sahoo

Using time-dependent density functional theory (tdDFT) with exchange kernels we calculate and test imaginary frequency-dependent dipole polarizabilities for all atoms and many ns in rows 1-6 of the periodic table. These are then integrated…

Computational Physics · Physics 2016-07-08 Tim Gould , Tomas Bucko

We investigate the influence of the appearance of excitonic states on van der Waals interactions among two Rydberg atoms. The atoms are assumed to be in different Rydberg states, e.g., in the $|ns\rangle$ and $|np\rangle$ states. The…

Atomic Physics · Physics 2015-08-12 Hashem Zoubi

A systematic study of the leading isotropic van der Waals coefficients for the alkali-metal atom + molecule and molecule + molecule systems is presented. Dipole moments and static and dynamic dipole polarizabilities are calculated employing…

Atomic Physics · Physics 2013-02-22 P. S. Zuchowski , M. Kosicki , M. Kodrycka , P. Soldan

We evaluate the electric-dipole and electric-quadrupole static and dynamic polarizabilities for the 6s^2 ^1S_0, 6s6p ^3P_0, and 6s6p ^3P_1 states and estimate their uncertainties. A methodology is developed for an accurate evaluation of the…

Atomic Physics · Physics 2015-06-16 S. G. Porsev , M. S. Safronova , A. Derevianko , Charles W. Clark

The van der Waals coefficients, from C_11 through to C_16 resulting from 2nd, 3rd and 4th order perturbation theory are estimated for the alkali (Li, Na, K and Rb) atoms. The dispersion coefficients are also computed for all possible…

Atomic Physics · Physics 2007-05-23 J. Mitroy , M. W. J. Bromley

We study the van der Waals interaction between Rydberg alkali-metal atoms with fine structure ($n^2L_j$; $L\leq 2$) and heteronuclear alkali-metal dimers in the ground rovibrational state ($X^1\Sigma^+$; $v=0$, $J=0$). We compute the…

Atomic Physics · Physics 2020-04-01 Vanessa Olaya , Jesús Pérez-Ríos , Felipe Herrera

In this work we investigate how atomic $C_6$ coefficients and static dipole polarizabilities $\alpha$ scale with effective volume. We show, using confined atoms covering rows 1-5 of the periodic table, that $C_6/C_6^R\approx (V/V^R)^{p_Z}$…

Chemical Physics · Physics 2016-09-06 Tim Gould

A simple and computationally efficient scheme to calculate approximate imaginary-frequency dependent polarizability, hence asymptotic van der Waals coefficient, within density functional theory is proposed. The dynamical dipolar…

Materials Science · Physics 2009-04-20 Huy-Viet Nguyen , Stefano de Gironcoli
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