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We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…

Generation of second-harmonic waves is one of the universal nonlinear phenomena that have found numerous technical applications in many modern technologies, in particular, in photonics. This phenomenon also has great potential in the field…

Mesoscale and Nanoscale Physics · Physics 2024-03-01 K. O. Nikolaev , S. R. Lake , G. Schmidt , S. O. Demokritov , V. E. Demidov

Strong coupling between light and matter in an optical cavity provides a pathway to giant polariton nonlinearity, where effective polariton-polariton interactions are mediated by materials' nonlinear responses. The pursuit of such enhanced…

Optics · Physics 2024-11-26 Zhi Wang , Li He , Bumho Kim , Bo Zhen

We investigate Second Harmonic Generation from individual silicon nanowires and study the influence of resonant optical modes on the far-field nonlinear emission. We find that the polarization of the Second Harmonic has a size-dependent…

Mesoscale and Nanoscale Physics · Physics 2016-03-18 Peter R. Wiecha , Arnaud Arbouet , Christian Girard , Thierry Baron , Vincent Paillard

Recent advances in emerging atomically thin transition metal dichalcogenide semiconductors with strong light-matter interactions and tunable optical properties provide novel approaches for realizing new material functionalities. Coupling…

Nanophotonics research has focused recently on the ability of non-linear optical processes to mediate and transform optical signals in a myriad of novel devices, including optical modulators, transducers, color filters, photodetectors,…

Quantifying and controlling the coherent dynamics and couplings of optically active excitations in solids is of paramount importance in fundamental research in condensed matter optics and for their prospective optoelectronic applications in…

Electrically controlled photonic circuits hold promise for information technologies with greatly improved energy efficiency and quantum information processing capabilities. However, weak nonlinearity and electrical response of typical…

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the beam's intensity profile or wave front. While shaping and controlling the light field is a highly researched topic,…

Nonlinear optical effects have been studied extensively in microresonators as more photonics applications transition to integrated on-chip platforms. Due to low optical losses and small mode volumes, microresonators are demonstrably the…

Optics · Physics 2018-07-04 Joshua B. Surya , Xiang Guo , Chang-Ling Zou , Hong X. Tang

Nonlinear optical generation has been a well-established way to realize frequency conversion in nonlinear optics, whereas previous studies were just focusing on the scalar light fields. Here we report a concise yet efficient experiment to…

Optics · Physics 2018-11-20 Li Zhang , Fei Lin , Xiaodong Qiu , Lixiang Chen

Electronic states in two-dimensional layered materials can exhibit a remarkable variety of correlated phases including Wigner-crystals, Mott insulators, charge density waves, and superconductivity. Recent experimental and theoretical…

Mesoscale and Nanoscale Physics · Physics 2021-08-16 Kai Hao , Robert Shreiner , Alexander A. High

Controlling exciton recombination in atomically thin semiconductors is central to their optoelectronic functionality, as the competition between radiative and non-radiative decay channels governs emission efficiency. Existing approaches,…

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

We report ultra-strong high-order nonlinear multiphoton processes in monolayer MoS$_2$ (1L-MoS$_2$): the third harmonic is thirty times stronger than the second harmonic, and the fourth harmonic is comparable to the second harmonic. We find…

Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can…

Topological photonics enables robust light manipulation with third-order optical nonlinearity, yet integrating second-order optical nonlinearity into a topological system faces fundamental challenges: frequency-dependent topological…

Optics · Physics 2025-06-30 Ruoyu Wang , Yiming Pan , Xiaoqin Shen

Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…

Materials Science · Physics 2021-10-12 Shingo Toyoda , Manfred Fiebig , Taka-hisa Arima , Yoshinori Tokura , Naoki Ogawa

Frequency conversion processes, such as second- and third-harmonic generation, are one of the most common effects in nonlinear optics which offer many opportunities for photonics, chemistry, material science, characterization, and…

Optics · Physics 2017-06-26 Alexander Krasnok , Mykhailo Tymchenko , Andrea Alu
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