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Related papers: Electronic Transitions in Strained SmNiO_3 Thin Fi…

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Bulk NdNiO3 exhibits a metal-to-insulator transition (MIT) as the temperature is lowered that is also seen in tensile strained films. In contrast, films that are under a large compressive strain typically remain metallic at all…

Strongly Correlated Electrons · Physics 2016-04-05 Jack Y. Zhang , Honggyu Kim , Evgeny Mikheev , Adam J. Hauser , Susanne Stemmer

We report a temperature-dependent Raman scattering investigation of thin film rare earth nickelates SmNiO3, NdNiO3 and Sm0.60Nd0.40NiO3, which present a metal-to-insulator (MI) transition at TMI and an antiferromagnetic-paramagnetic Neel…

Materials Science · Physics 2009-11-13 C. Girardot , J. Kreisel , S. Pignard , N. Caillault , F. Weiss

We have investigated the temperature driven first order metal-insulator (M-I) transition in thin films of NdNiO$_3$ and have compared it with the bulk behavior. The M-I transition of thin films is sensitive to epitaxial strain and a partial…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Devendra Kumar , K. P. Rajeev , A. K. Kushwaha , R. C. Budhani

The origin of simultaneous electronic, structural and magnetic transitions in bulk rare-earth nickelates ($RE$NiO$_3$) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure…

Strongly Correlated Electrons · Physics 2019-07-15 Shashank Kumar Ojha , Sujay Ray , Tanmoy Das , S. Middey , Sagar Sarkar , Priya Mahadevan , Zhen Wang , Yimei Zhu , Xiaoran Liu , M. Kareev , J. Chakhalian

Interaction between the lattice and the orbital degrees of freedom not only makes rare-earth nickelates unusually "bad metal", but also introduces a temperature driven insulator-metal phase transition. Here we investigate this…

Strongly Correlated Electrons · Physics 2014-08-20 Anindita Sahoo , Sieu D. Ha , Shriram Ramanathan , Arindam Ghosh

Bulk NdNiO_3 and thin films grown along the pseudocubic (001)_pc axis display a 1st order metal to insulator transition (MIT) together with a N\'eel transition at T=200K. Here, we show that for NdNiO3 films deposited on (111)_pc NdGaO_3 the…

Strongly Correlated Electrons · Physics 2015-05-05 S. Catalano , M. Gibert , V. Bisogni , F. He , R. Sutarto , M. Viret , P. Zubko , R. Scherwitzl , G. A. Sawatzky , T. Schmitt , J. -M. Triscone

We have synthesized epitaxial NdNiO$_{3}$ ultra-thin films in a layer-by-layer growth mode under tensile and compressive strain on SrTiO$_{3}$ (001) and LaAlO$_3$ (001), respectively. A combination of X-ray diffraction, temperature…

Strongly Correlated Electrons · Physics 2015-05-18 Jian Liu , M. Kareev , B. Gray , J. W. Kim , P. Ryan , B. Dabrowski , J. W. Freeland , J. Chakhalian

We present evidence that the metal-insulator transition (MIT) in a tensile strained NdNiO3 (NNO) film is facilitated by a redistribution of electronic density and neither requires Ni charge disproportionation nor symmetry change [1, 2].…

Strongly Correlated Electrons · Physics 2015-07-20 M. H. Upton , Yongseong Choi , Jian Liu , D. Meyers , S. Middey , J. Chakhalian , Jong-Woo Kim , Philip J. Ryan

The correlated oxide SmNiO3 (SNO) exhibits an insulator to metal transition (MIT) at 130 {\deg}C in bulk form. We report on synthesis and electron transport in SNO films deposited on LaAlO3 (LAO) and Si single crystals. X-ray diffraction…

Materials Science · Physics 2013-01-09 Sieu D. Ha , Gulgun H. Aydogdu , Shriram Ramanathan

Metallic transition-metal oxides undergo a metal-to-insulator transition (MIT) as the film thickness decreases across a ritical thickness of several monolayers (MLs), but its driving mechanism remains controversial. We have studied the…

The effect of high tensile strain and low dimensionality on the magnetic and electronic properties of CaMnO$_3$ ultrathin films, epitaxially grown on SrTiO$_3$ substrates, are experimentally studied and theoretically analyzed. By means of…

Materials Science · Physics 2020-09-02 A. López Pedroso , M. A. Barral , M. E. Graf , A. M. Llois , M. H. Aguirre , L. B. Steren , S. Di Napoli

Rare-earth nickelates RNiO3 (R=rare-earth element) exhibit three kinds of phase transitions with decreasing temperature: a structural transition from a pseudo-cubic to a monoclinic phase, a metal- insulator transition (MIT), and a magnetic…

The nature of the metal insulator transition in thin films and superlattices of LaNiO3 with only few unit cells in thickness remains elusive despite tremendous effort. Quantum confinement and epitaxial strain have been evoked as the…

In transition metal oxides electron-electron interaction and lattice degree of freedom are basic ingredients of emergent phenomena, such as metal-to-insulator transition (MIT) and superconductivity. Perovskite rare-earth nickelates are…

We study the electronic structure, magnetic state, and phase stability of paramagnetic BiNiO$_3$ near a pressure-induced Mott insulator-to-metal transition (MIT) by employing a combination of density functional and dynamical mean-field…

Strongly Correlated Electrons · Physics 2019-11-06 I. Leonov , A. S. Belozerov , S. L. Skornyakov

The rare-earth nickelates (RNiO3) exhibit interesting phenomena such as unusual antiferromagnetic order at wavevector q = (1/2, 0, 1/2) and a tunable insulator-metal transition that are subjects of active research. Here we present…

Ultrathin epitaxial films of EuNiO3 were grown on a series of substrates traversing highly compressive (- 2.4%) to highly tensile (2.5%) lattice mismatch. X-ray diffraction measurements showed the expected c-lattice parameter shift for…

Strongly Correlated Electrons · Physics 2014-04-25 D. Meyers , S. Middey , M. Kareev , M. van Veenendaal , E. J. Moon , B. A. Gray , J. W. Freeland , J. Chakhalian

The metal-insulator transition (MIT) of bulk rare-earth nickelates is accompanied by a simultaneous charge ordering (CO) transition. We have investigated low-frequency resistance fluctuations (noise) across the MIT and magnetic transition…

Strongly Correlated Electrons · Physics 2019-09-05 Gopi Nath Daptary , Siddharth Kumar , M. Kareev , J. Chakhalian , Aveek Bid , S. Middey

Mott physics is characterized by an interaction-driven metal-to-insulator transition in a partially filled band. In the resulting insulating state, antiferromagnetic orders of the local moments typically develop, but in rare situations no…

Nickelates are a rich class of materials, ranging from insulating magnets to superconductors. But for stoichiometric materials, insulating behavior is the norm, as for most late transition metal oxides. Notable exceptions are the 3D…

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