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We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from…

Atomic Physics · Physics 2026-01-30 R. Esteban Goetz , Anh-Thu Le

Collinear double-pulse seeding of the High-Gain Harmonic Generation (HGHG) process in a free-electron laser (FEL) is a promising approach to facilitate various coherent nonlinear spectroscopy schemes in the extreme ultraviolet (XUV)…

We investigated the influence of sub-cycle driving fields on high-order harmonic generation (HHG), with a focus on intrinsic chirp, carrier-envelope phase (CEP), and number of laser cycles. Our findings reveals that the center frequency of…

Optics · Physics 2025-12-08 Rambabu Rajpoot , Eiji J. Takahashi

We report the realization and characterization of parametric amplification in high harmonic generation around 100 eV using He gas in a double gas jet arrangement. The delay of the seed XUV pulse with respect to the amplifier gas jet was…

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Chiral (highly helical) extreme ultraviolet (XUV) sources are pivotal for investigating chiroptical phenomena on the ultrafast electronic timescale. Table-top, coherent High Harmonic Generation (HHG)-based sources are particularly…

Optics · Physics 2025-03-07 Eran Ben Arosh , Eldar Ragonis , Lev Merensky , Avner Fleischer

We experimentally and numerically study the atomic response and pulse propagation effects of high-order harmonics generated in Xe, Kr, and Ar driven by a 2.1-\mu m infrared femtosecond light source. The light source is an optical parametric…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

Strongly Correlated Electrons · Physics 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

A theoretical model is developed describing high-order harmonic generation (HHG) from a gas of multiply-charged ions driven by a laser field of relativistic intensity. Macroscopic propagation of harmonics is investigated in a relativistic…

Atomic Physics · Physics 2012-02-21 Markus C. Kohler , Karen Z. Hatsagortsyan

Extreme ultraviolet (XUV) lasers are essential for the investigation of fundamental physics. Especially high repetition rate, high photon flux sources are of major interest for reducing acquisition times and improving signal to noise ratios…

We report on continuous high-harmonic generation at 1 kHz repetition rate from a liquid-sheet plasma mirror driven by relativistic-intensity near-single-cycle light transients. Through precise control of both the surface plasma density…

High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…

Atomic Physics · Physics 2022-04-15 L. Ortmann , C. Hofmann , I. A. Ivanov , A. S. Landsman

High-order harmonic generation driven by intense extreme ultraviolet (EUV) fields merges quantum optics and attosecond science, giving rise to an appealing route for the generation of coherent EUV and soft X-ray light for high-resolution…

We report generation of high harmonics in a gas-jet pumped by pulses self-compressed in a He-filled hollow-core photonic crystal fiber through the soliton effect. The gas-jet is placed directly at the fiber output. As the energy increases…

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

It is demonstrated by single-atom simulations that X-ray signals in the 3.4 to 4 keV region from an 8 micron laser driven high harmonic generation can be increased by more than two orders of magnitude when a single-cycle pulse centered at…

Atomic Physics · Physics 2019-04-24 Zenghu Chang

We report a novel quasi-phase matching technique for high-order harmonic generation in low-density gases. Numerical simulations show that in few-optical cycle pulsed Bessel beams it is possible to control the pulse envelope and phase…

High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the…

Atomic Physics · Physics 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Carsten Müller , Christoph H. Keitel

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

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