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We perform a post-compression of high energy pulses by using optical-field ionization of low pressure helium gas in a guided geometry. We apply this approach to a TW chirped-pulse-amplification based Ti:Sapphire laser chain and show that…

Isolated attosecond pulses (IAPs) produced through laser-driven high-harmonic generation (HHG) hold promise for unprecedented insight into biological processes via attosecond x-ray diffraction with tabletop sources. However, efficient…

Coherent sources of attosecond extreme ultraviolet (XUV) radiation present many challenges if their full potential is to be realized. While many applications benefit from the broadband nature of these sources, it is also desirable to…

High harmonic spectroscopy can access structural and dynamical information on molecular systems encoded in amplitude and phase of high harmonic generation (HHG) signals4. However, measurement of the harmonic phase is a daunting task. Here…

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

High harmonic generation (HHG) is a crucial technology for compact, high-brightness extreme ultraviolet (XUV) and soft X-ray sources, which are key to advancing both fundamental and applied sciences. The availability of advanced driving…

Optics · Physics 2025-10-07 Robert Klas , Martin Gebhardt , Jan Rothhardt , Jens Limpert

Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics…

Recent demonstrations of high-harmonic generation (HHG) at very high repetition frequencies (~100 MHz) may allow for the revolutionary transfer of frequency combs to the vacuum ultraviolet (VUV). This advance necessitates unifying optical…

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

Plasma high harmonics generation from an extremely intense short-pulse laser is explored by including the effects of ion motion, electron-ion collisions and radiation reaction force in the plasma dynamics. The laser radiation pressure…

Plasma Physics · Physics 2017-05-17 Suo Tang , Naveen Kumar , Christoph H. Keitel

Circularly polarized extreme ultraviolet (XUV) radiation is highly interesting for investigation of chirality-sensitive light-matter interactions. Recent breakthroughs have enabled generation of such light sources via high harmonic…

Optics · Physics 2019-02-19 Zi-Yu Chen , Rui Qin

This study demonstrates the potential to generate a soft X-ray single-cycle attosecond pulse using a single-cycle mid-infrared pulse from the advanced dual-chirped optical parametric amplification. Supercontinuum high harmonic (HH) spectrum…

Optics · Physics 2024-10-07 Kaito Nishimiya , Feng Wang , Pengfei Lan , Eiji J. Takahashi

We propose a method for programmable shaping of the amplitude and phase of the XUV and x-ray attosecond pulses produced by high-order harmonic generation. It overcomes the bandwidth limitations of existing spectral filters and enables…

Optics · Physics 2015-06-17 Dane R. Austin , Jens Biegert

We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For…

Atomic Physics · Physics 2016-12-28 V. V. Strelkov

This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…

High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…

Optics · Physics 2024-12-10 Qi Zeng , Yimin Deng , Xinyue Yang , Wei Cao , Peixiang Lu

Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a…

We present a method of producing single attosecond pulses by high-order harmonic generation with multi-cycle nonlinear chirped driver laser pulses. The symmetry of the laser feld in several optical cycles near the pulse center is…

Optics · Physics 2009-06-12 Yang Xiang , Yueping Niu , Yihong Qi , Shangqing Gong

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

One of the main difficulties to efficiently generating high-order harmonics in long neutral-gas targets is to reach the phase-matching conditions. One issue is that the medium cannot be sufficiently ionized by the driving laser due to…