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A joint theoretical approach, combining macroscopic symmetry analysis with microscopic methods (density functional theory and model cluster Hamiltonian), is employed to shed light on magnetoelectricity in Ba2CoGe2O7. We show that the…

Strongly Correlated Electrons · Physics 2015-05-27 Kunihiko Yamauchi , Paolo Barone , Silvia Picozzi

Type-II multiferroics, in which the magnetic order breaks inversion symmetry, are appealing for both fundamental and applied research due their intrinsic coupling between magnetic and electrical orders. Using first-principles calculations…

Materials Science · Physics 2023-11-20 Urmimala Dey , Mark S. Senn , Nicholas C. Bristowe

We performed high-magnetic-field magnetization, polarization, and ultrasonic measurements in Ba$_2$CuGe$_2$O$_7$ to investigate field-induced multiferroic properties arising from a cross-correlation between electric dipoles and electric…

Strongly Correlated Electrons · Physics 2024-03-20 R. Kurihara , Y. Sato , A. Miyake , M. Akaki , K. Mitsumoto , M. Hagiwara , H. Kuwahara , M. Tokunaga

We investigate the spin-induced polarization in the multiferroic compound Ba2CuGe2O7 using variarional and finite temperature mean field approaches. The compound is described by a spin-3/2 Heisenberg model extended with easy plane…

Strongly Correlated Electrons · Physics 2012-02-21 Judit Romhanyi , Miklos Lajko , Karlo Penc

We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be…

Strongly Correlated Electrons · Physics 2015-05-19 H. Murakawa , Y. Onose , S. Miyahara , N. Furukawa , Y. Tokura

We report results of joint experimental and theoretical studies on magnetoelectric (ME) compounds Co4Nb2O9 and Co4Ta2O9. On the experimental side, we present results of the magnetization and dielectric permittivity measurements in the…

Materials Science · Physics 2016-09-23 I. V. Solovyev , T. V. Kolodiazhnyi

Magnetic structure of the multiferroic Ca$_{2}$CoSi$_{2}$O$_{7}$ was determined by neutron diffraction techniques. Combination of the polycrystalline and single-crystal samples experiments revealed a collinear antiferromagnetic structure…

The unusual magnetoelectric effects observed in the multiferroic phase arising below TN=6.7K in Ba2CoGe2O7 (BCG) are related to the spontaneous toroidal moment existing in this compound. The transition to the multiferroic state, which…

Materials Science · Physics 2010-12-06 Pierre Toledano , Dmitry D. Khalyavin , Laurent C. Chapon

The magnetoelectric behavior of BiFeO$_3$ has been explored on the basis of accurate density functional calculations. The structural, electronic, magnetic, and ferroelectric properties of BiFeO$_3$ are predicted correctly without including…

Materials Science · Physics 2007-05-23 P. Ravindran , R. Vidya , A. Kjekshus , H. Fjellvåg , O. Eriksson

We report electric polarization and magnetization measurements in single crystals of double perovskite Lu2MnCoO6 using pulsed magnetic fields and optical second harmonic generation (SHG) in DC magnetic fields. we observe well-resolved…

Materials Science · Physics 2016-06-22 S. Chikara , J. Singleton , J. Bowlan , D. A. Yarotski , N. Lee , H. Y. Choi , Y. J. Choi , V. S. Zapf

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution…

Strongly Correlated Electrons · Physics 2019-07-31 G. H. Wang , C. Y. Xu , H. B. Cao , T. Hong , Q. Huang , Q. Y. Ren , J. Q. Xu , H. D. Zhou , W. D. Luo , D. Qian , J. Ma

Our results describe an unprecedented example of change in the mechanism of magnetically-induced electric polarization from spin current to spin-dependent p-d hybridization model. We have followed the evolution of the magnetic structures of…

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

The structural, electronic, magnetic and ferroelectric properties of Pb free double perovskite multiferroic Bi2FeTiO6 are investigated using density functional theory within the general gradient approximation (GGA) method. Our structural…

Materials Science · Physics 2018-05-23 Lokanath Patra , P. Ravindran

It was recently observed that materials showing most striking multiferroic phenomena are frustrated spin-density-wave magnets. We present a simple phenomenological theory, which describes the orientation of the induced electric polarization…

Strongly Correlated Electrons · Physics 2009-11-11 Maxim Mostovoy

The question of how ferroelectric polarization is coupled to magnetism in magnetoelectric multiferroics, in which both types of order are simultaneously present, is of considerable scientific and practical interest. A recent Letter…

Materials Science · Physics 2009-07-13 Rogerio de Sousa , Joel E. Moore

The fundamental principles of electrodynamics allow an electron carrying both electric monopole (charge) and magnetic dipole (spin) but prohibit its magnetic counterpart. Recently it was predicted that the magnetic "monopoles" carrying…

Strongly Correlated Electrons · Physics 2020-03-04 Feng Jin , Changle Liu , Anmin Zhang , Xiaoqun Wang , Gang Chen , Xuefeng Sun , Qingming Zhang

Density functional based simulations are employed to explore magnetoelectric effects in iron-based oxides, showing a unique layered structure. We theoretically predict CaFeO2 to be a promising magnetoelectric, showing…

Strongly Correlated Electrons · Physics 2015-06-15 Kunihiko Yamauchi , Tamio Oguchi , Silvia Picozzi

Despite remarkable progress in developing multifunctional materials, spin-driven ferroelectrics featuring both spontaneous magnetization and electric polarization are still rare. Among such ferromagnetic ferroelectrics are conical spin…

Strongly Correlated Electrons · Physics 2017-06-09 T. Honda , J. S. White , A. B. Harris , L. C. Chapon , A. Fennell , B. Roessli , O. Zaharko , Y. Murakami , M. Kenzelmann , T. Kimura

We present a phenomenological model for magnetoelectricity in multiferroic materials. The distinctive feature of the model is a two-component complex order parameter that encodes the electric polarization, along with a direct coupling…

Materials Science · Physics 2024-04-11 Pei Wang , You-Quan Li
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