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We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

Strongly Correlated Electrons · Physics 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa

Information about the physical properties of astrophysical objects cannot be measured directly but is inferred by interpreting spectroscopic observations in the context of atomic physics calculations. Ratios of emission lines, for example,…

Two-phonon contributions to meV-resolved inelastic x-ray scattering spectra of MgB2 at 300K are identified, in good agreement, in both intensity and energy, with a harmonic calculation using the force constant matrix from ab-inito LDA…

Superconductivity · Physics 2007-05-23 A. Q. R. Baron , H. Uchiyama , R. Heid , K. -P. Bohnen , Y. Tanaka , S. Tsutsui , D. Ishikawa , S. Lee , S. Tajima

We present an implementation of a damped response framework for calculating resonant inelastic X-ray scattering (RIXS) at the equation-of-motion coupled cluster singles and doubles (CCSD) and second-order approximate coupled cluster singles…

Orbital degrees of freedom play a major role in the physics of many strongly correlated transition metal compounds. However, they are still very difficult to access experimentally, in particular by neutron scattering. We propose here how to…

Strongly Correlated Electrons · Physics 2015-04-28 Pasquale Marra

Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitations of these materials hold great promise for understanding and…

Strongly Correlated Electrons · Physics 2019-04-02 Y. Cao , D. G. Mazzone , D. Meyers , J. P. Hill , X. Liu , S. Wall , M. P. M. Dean

A spherical tensor expansion is carried out to express the resonant inelastic scattering cross-section as a sum of products of fundamental spectra with tensors involving wavevectors and polarization vectors of incident and scattered…

Strongly Correlated Electrons · Physics 2014-05-20 Amélie Juhin , Christian Brouder , Frank De Groot

We present a method for including inelastic scattering in a first-principles density-functional computational scheme for molecular electronics. As an application, we study two geometries of four-atom gold wires corresponding to two…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Thomas Frederiksen , Mads Brandbyge , Nicolas Lorente , Antti-Pekka Jauho

Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

Strongly Correlated Electrons · Physics 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

The study of the interstellar medium (ISM) in the X-rays has entered a golden age with the advent of the X-ray observatories XMM-Newton and Chandra. High-energy resolution allowed to study dust spectroscopic features with unprecedented…

Astrophysics of Galaxies · Physics 2023-04-05 Elisa Costantini , Lia Corrales

Recent experiments on La$_2$CuO$_4$ suggest that indirect resonant inelastic X-ray scattering (RIXS) might provide a probe for transversal spin dynamics. We present in detail a systematic expansion of the relevant magnetic RIXS cross…

Strongly Correlated Electrons · Physics 2011-07-22 Filomena Forte , Luuk J. P. Ament , Jeroen van den Brink

Nuclear resonant forward scattering (NFS) and nuclear inelastic scattering (NIS) of synchrotron radiation are fairly recent spectroscopic methods for the investigation of complexes containing M\"ossbauer-active transition metal ions. NFS,…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Volker Schünemann , Alfred Xaver Trautwein , Heiner Winkler

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane.…

We provide a semiquantitative explanation of a recent experiment on the resonant inelastic x-ray scattering (RIXS) in insulating cuprate La2CuO4 (Y.J. Kim et al., Phys. Rev. Lett. 89, 177003 (2002).). We show theoretically that there are…

Strongly Correlated Electrons · Physics 2009-11-10 Takuji Nomura , Jun-ichi Igarashi

Small-Angle Scattering (SAS) investigates structures in samples that generally range from approximately 0.5 nm to a few 100 nm. This can both be done for isotropic samples such as blends and liquids, as well as anisotropic samples such as…

Instrumentation and Detectors · Physics 2023-09-22 Sebastian Jaksch

Despite significant progress in resonant inelastic x-ray scattering (RIXS) experiments on cuprates at the Cu L-edge, a theoretical understanding of the cross-section remains incomplete in terms of elementary excitations and the connection…

Strongly Correlated Electrons · Physics 2016-05-16 Chunjing Jia , Krzysztof Wohlfeld , Yao Wang , Brian Moritz , Thomas P. Devereaux

This work formally investigates the differential evolution indicators as a tool for ultrasonic tracking of elastic transformation and fracturing in randomly heterogeneous solids. Within the framework of periodic sensing, it is assumed that…

Analysis of PDEs · Mathematics 2023-03-29 Fatemeh Pourahmadian , Houssem Haddar

An unparalleled resolution is reported with an inelastic x-ray scattering instrument at the Cu K-edge. Based on a segmented concave analyzer, featuring single crystal quartz (SiO_{2}) pixels, the spectrometer delivers a resolution near 25…

A recent and unexpected discrepancy between \textit{ab initio} simulations and the interpretation of a laser shock experiment on aluminum, probed by X-ray Thomson scattering (XRTS), is addressed. The ion-ion structure factor deduced from…

Plasma Physics · Physics 2020-11-19 J. Clerouin , P. Arnault , G. Robert , C. Ticknor , J. Kress , L. Collins

X-ray Photon Correlation Spectroscopy (XPCS) has emerged as a unique technique allowing the measurement of dynamics in materials on mesoscopic lengthscales. In particular, applications in soft matter physics cover a broad range of topics…

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