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This paper reviews non-resonant meV-resolved inelastic x-ray scattering (IXS) as a complementary method to inelastic neutron scattering (INS). Two aspects of IXS that are notable in this context are (1) that IXS allows straightforward…

Soft Condensed Matter · Physics 2024-06-18 Alfred Q. R. Baron

Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and…

The use of inelastic x-ray scattering (IXS) to investigate phonons and phonon dispersion in crystals opens the field of phonon spectroscopy, allowing measurements on tiny samples: micrograms of material, or single crystals ~10 to 100 micron…

Materials Science · Physics 2009-11-02 Alfred Q. R. Baron

Excitons in a complex organic molecular crystal were studied by inelastic x-ray scattering (IXS) for the first time. The dynamic dielectric response function is measured over a large momentum transfer region, from which an exciton…

Other Condensed Matter · Physics 2007-05-23 K. Yang , L. P. Chen , Y. Q. Cai , N. Hiraoka , S. Li , J. F. Zhao , D. W. Shen , H. F. Song , H. Tian , L. H. Bai , Z. H. Chen , Z. G. Shuai , D. L. Feng

We describe how improvements in methodology and instrumentation for meV-resolved inelastic x-ray scattering (IXS), coupled with a fresh examination of older theory, allow identification of interaction between the quasi-elastic and acoustic…

Soft Condensed Matter · Physics 2022-05-18 Alfred Q. R. Baron , Daisuke Ishikawa

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

Strongly Correlated Electrons · Physics 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and…

Instrumentation and Detectors · Physics 2017-09-11 Jungho Kim , D. Casa , Ayman Said , Richard Krakora , B. J. Kim , Elina Kasman , Xianrong Huang , T. Gog

X-ray echo spectroscopy, a space-domain counterpart of neutron spin echo, is a recently proposed inelastic x-ray scattering (IXS) technique. X-ray echo spectroscopy relies on imaging IXS spectra, and does not require x-ray…

Optics · Physics 2017-08-04 Yuri Shvyd'ko

Inelastic x-ray scattering (IXS) now a widely used technique for studying the dynamics of electrons in condensed matter. We previously posed a solution to the phase problem for IXS [P. Abbamonte, et. al., Phys. Rev. Lett. {\bf 92}, 237401…

Strongly Correlated Electrons · Physics 2013-05-29 P. Abbamonte , J. P. Reed , Y. I. Joe , Yu Gan , D. Casa

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Thomas P. Devereaux , John P. Hill , Jeroen van den Brink

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

We describe a new method for imaging ultrafast dynamics in condensed matter using inelastic x-ray scattering (IXS). We use the concepts of causality and irreversibility to construct a general solution to the inverse scattering problem (or…

Other Condensed Matter · Physics 2009-06-12 P. Abbamonte , G. C. L. Wong , D. Cahill , J. P. Reed , R. H. Coridan , N. W. Schmidt , G. H. Lai , Y. I. Joe , D. Casa

We study conditions for aberration-free imaging of inelastic x-ray scattering (IXS) spectra with x-ray echo spectrometers. Aberration-free imaging is essential for achieving instrumental functions with high resolution and high contrast.…

Instrumentation and Detectors · Physics 2019-05-29 Manuel Sánchez del Río , Yuri Shvyd'ko

The state-resolved differential cross sections for both the 1s2 1S0 - 1s2s 1S0 monopolar transition and the 1s2 1S0 - 1s2p 1P1 dipolar transition of atomic helium have been measured over a large momentum transfer region by the…

Atomic Physics · Physics 2015-05-13 B. P. Xie , L. F. Zhu , K. Yang , B. Zhou , N. Hiraoka , Y. Q. Cai , Y. Yao , C. Q. Wu , E. L. Wang , D. L. Feng

Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

We compare several different ways of measuring the energy resolution for meV-resolved inelastic x-ray scattering (IXS): using scattering from poly(methyl methacrylate), PMMA, using scattering from borosilicate glass (Tempax), and using…

Materials Science · Physics 2021-03-17 Daisuke Ishikawa , Alfred Q. R. Baron

We propose a method for realizing true, real-space imaging of charge dynamics in a periodic system, with angstrom spatial resolution and attosecond time resolution. In this method, inelastic x-ray scattering (IXS) is carried out with a…

Strongly Correlated Electrons · Physics 2015-06-05 Yu Gan , Anshul Kogar , Peter Abbamonte

The development of medium-energy inelastic X-ray scattering (IXS) optics with meV and sub-meV resolution has attracted considerable efforts in recent years. Meanwhile, there are also concerns or debates about the fundamental and feasibility…

Optics · Physics 2011-09-12 Xian-Rong Huang

Understanding quantum materials -- solids in which quantum-mechanical interactions among constituent electrons yield a great variety of novel emergent phenomena -- is a forefront challenge in modern condensed matter physics. This goal has…

Strongly Correlated Electrons · Physics 2026-03-13 M. Mitrano , S. Johnston , Young-June Kim , M. P. M. Dean

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink
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