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Related papers: Dynamical Jahn--Teller instability in metallic ful…

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The Jahn-Teller distortion and the resulting orbital order usually cause some fascinating correlated electronic behaviors, and generally lead to antiferromagnetism in perovskite bulks. Here we demonstrate that the Jahn-Teller distortion…

Materials Science · Physics 2023-05-03 Ke Ji , Zongshuo Wu , Xiaofan Shen , Jianli Wang , Junting Zhang

Mott-Hubbard metal-insulator transitions in $N$-fold degenerate Hubbard models are studied within the Gutzwiller approximation. For any rational filling with $x$ (integer) electrons per site it is found that metal-insulator transition…

Condensed Matter · Physics 2009-10-22 Jian Ping Lu

Charge-state transitions of a single Cu-phthalocyanine molecule adsorbed on an insulating layer of NaCl on Cu(111) are probed by means of alternate charging scanning tunneling microscopy. Real-space imaging of the electronic transitions…

The electronic properties of many transition metal oxide systems require new ideas concerning the behaviour of electrons in solids for their explanation. A recent example, subsequent to that of cuprate superconductors, is of rare earth…

Strongly Correlated Electrons · Physics 2007-05-23 T. V. Ramakrishnan , H. R. Krishnamurthy , S. R. Hassan , G. Venketeswara Pai

It is shown that the d8 electron system occurring in the Ni2+ ion can have the non-magnetic ground state in the atomic scale formed by the Jahn-Teller effect. The tetragonal/trigonal off-cubic lattice distortion for the octahedral site…

Strongly Correlated Electrons · Physics 2007-05-23 Z. Ropka , R. J. Radwanski

The Jahn-Teller effect used semi-theoretically to analyse UV-visible spectra of the diamond like-carbon films on Si substrates. By deconvolution of UV-visible absorption spectra of the typical films, different absorption lines found. For…

Materials Science · Physics 2007-05-23 M. A. Vesaghi , A. Shafiekhani

By constructing an effective model based on recently calculated \emph{ab }initio bare interaction parameters, we study the phase diagram of alkali doped fullerides as a function of temperature and internal pressure. We use a slave-rotor…

Strongly Correlated Electrons · Physics 2019-10-08 Theja N. De Silva

The quadratic Jahn-Teller effect of C$_{60}^{n-}$ ($n=$ 1-5) is investigated from the first principles. Employing the density functional theory calculations with hybrid functional, the quadratic vibronic coupling constants of C$_{60}^-$…

Strongly Correlated Electrons · Physics 2018-07-03 Dan Liu , Yasuyuki Niwa , Naoya Iwahara , Tohru Sato , Liviu F. Chibotaru

It is shown that the layered antiferromagnetic order in stoechiometric LaMnO_3 cannot be understood purely from electronic interactions. On the contrary, it mainly results from strong cooperative Jahn-Teller deformations. Those involve a…

Strongly Correlated Electrons · Physics 2009-10-31 M. Capone , D. Feinberg , M. Grilli

We study the unconventional insulating state in A_4C_{60} with a variety of approaches, including density functional calculations and dynamical mean-field theory. While the former predicts a metallic state, in disagreement with experiment,…

Strongly Correlated Electrons · Physics 2007-08-07 M. Capone , M. Fabrizio , P. Giannozzi , E. Tosatti

The trivalent alkali fullerides A$_3$C$_{60}$, where C$_{60}$ are a well established family of molecular superconductors. The electron pairing has s-wave symmetry and is due to standard electron-phonon coupling, in particular by Jahn-Teller…

Superconductivity · Physics 2009-06-24 M. Capone , M. Fabrizio , C. Castellani , E. Tosatti

We study the electronic structure and magnetic interactions in methylamine-intercalated orthorhombic alkali-doped fullerene (CH3NH2)K3C60 within the density functional theory. As in the simpler ammonia intercalated compound (NH3)K3C60, the…

Strongly Correlated Electrons · Physics 2015-06-05 Anton Potočnik , Nicola Manini , Matej Komelj , Erio Tosatti , Denis Arčon

The Jahn-Teller (JT) distortion that can remove electronic degeneracies in partially occupied states and results in systematic atomic displacements is a common underlying feature to many of the intriguing phenomena observed in 3d…

Materials Science · Physics 2019-12-04 Julien Varignon , Manuel Bibes , Alex Zunger

Using elastic and inelastic neutron scattering, we investigated the evolution of the local atomic structure and lattice dynamics of La(1-x)Sr(x)CoO3 (x=0-0.5) as it crosses over with x from an insulator to a ferromagnetic metal (FMM). Our…

Strongly Correlated Electrons · Physics 2007-05-23 Despina Louca , J. L. Sarrao

The interplay between the band Jahn-Teller distortion and the superconductivity is studied for the system whose Fermi level lies in two-fold degenerate band. Assuming that the lattice distortion is coupled to the orbital electron density…

Superconductivity · Physics 2009-10-28 Haranath Ghosh , S. N. Behera , S. K. Ghatak , D. K. Ray

Perovskite oxides are already widely used in industry and have huge potential for novel device applications thanks to the rich physical behaviour displayed in these materials. The key to the functional electronic properties exhibited by…

Materials Science · Physics 2017-05-08 Julien Varignon , Nicholas C. Bristowe , Eric Bousquet , Philippe Ghosez

Magnetic and orbital structures in KCuF$_{3}$ are revisited by the cluster self-consistent field approach developed recently. We clearly showed that due to the inherent frustration, the ground state of the system with the superexchange and…

Strongly Correlated Electrons · Physics 2007-05-23 Dong-Meng Chen , Liang-Jian Zou

Alkali-doped fullerides exhibit a wealth of unusual phases that remain controversial by nature. Here we report a cryogenic scanning tunneling microscopy study of the sub-molecular structural and electronic properties of expanded fullerene…

Superconductivity · Physics 2020-02-26 Sha Han , Meng-Xue Guan , Can-Li Song , Yi-Lin Wang , Ming-Qiang Ren , Sheng Meng , Xu-Cun Ma , Qi-Kun Xue

For the first time, magnetic properties of fullerides have been studied using a torque technique. Rb3C60 single crystal has been investigated in these experiments. It was shown that this method is sensitive to the structural phase…

Superconductivity · Physics 2010-07-01 J. Chigvinadze , V. Buntar , S. Ashimov , T. Machaidze , G. Donadze

The mechanisms of localization of Jahn-Teller deformations and vibronic wavefunctions in isotope substituted dynamical Jahn-Teller systems are elucidated. It is found that the localization in the trough is of potential type in the case of…

Chemical Physics · Physics 2017-05-30 Naoya Iwahara , Tohru Sato , Kazuyoshi Tanaka , Liviu F. Chibotaru