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We successfully synthesized the zinc-verdazyl complex [Zn(hfac)$_2$]$\cdot$($o$-Py-V) [hfac = 1,1,1,5,5,5-hexafluoroacetylacetonate; $o$-Py-V = 3-(2-pyridyl)-1,5-diphenylverdazyl], which is an ideal model compound with an $S$ = 1/2…

We have succeeded in synthesizing single crystals of the verdazyl radical beta-2,6-Cl2-V [= beta-3-(2,6-dichlorophenyl)-1,5-diphenylverdazyl]. The ab initio MO calculation indicated the formation of an S = 1/2 Heisenberg antiferromagnetic…

Strongly Correlated Electrons · Physics 2013-11-20 H. Yamaguchi , T. Okubo , K. Iwase , T. Ono , Y. Kono , S. Kittaka , T. Sakakibara , A. Matsuo , K. Kindo , Y. Hosokoshi

A possibility of the uniform antiferromagnetic order is pointed out in an S=1/2 ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain compound: (CH_3)_2 CHNH_3 Cu(Cl_x Br_{1-x})_3. The system possesses…

Statistical Mechanics · Physics 2009-11-07 Tota Nakamura

A structural and thermodynamic study of the newly synthesized single crystal Sr5Rh4O12 is reported. Sr5Rh4O12 consists of a triangular lattice of spin chains running along the c-axis. It is antiferromagnetically ordered below 23 K with the…

Strongly Correlated Electrons · Physics 2015-06-25 G. Cao , S. Parkin , P. Schlottmann

The anisotropic s=1/2 anti-ferromagnetic Heisenberg chain in the presence of an external magnetic field is studied by using the standard quantum renormalization group. We obtain the critical line of the transition from partially magnetized…

Strongly Correlated Electrons · Physics 2009-10-31 A. Langari

The magnetization process of the one-dimensional antiferromagnetic Heisenberg model with the Ising-like anisotropic exchange interaction is studied by the exact diagonalization technique. It results in the evidence of the first-order spin…

Statistical Mechanics · Physics 2009-10-31 Toru Sakai , Minoru Takahashi

The ground state phase diagram of the alternating spin-1/2 chains with anisotropic ferromagnetic coupling under the influence of a symmetry breaking transverse magnetic field is studied. We have used the exact diagonalization technique. In…

Strongly Correlated Electrons · Physics 2008-03-31 Saeed Mahdavifar , Alireza Akbari

The low energy behavior of the S=1/2 antiferromagnetic XY-like XXZ chains with precious mean quasiperiodic exchange modulation is studied by the density matrix renormalization group method. It is found that the energy gap of the chain with…

Strongly Correlated Electrons · Physics 2009-10-31 Kazuo Hida

An $S=1/2$ ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain model is investigated in connection to its realization compound: (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$. The exchange interaction…

Disordered Systems and Neural Networks · Physics 2009-11-10 Tota Nakamura

Large single crystals of the new compound SrMn$_2$V$_2$O$_8$ have been grown by the floating-zone method. This transition-metal based oxide is isostructural to SrNi$_2$V$_2$O$_8$, described by the tetragonal space group $I4_1cd$. Magnetic…

Strongly Correlated Electrons · Physics 2011-07-28 Sandra K. Niesen , Oliver Heyer , Thomas Lorenz , Martin Valldor

The effect of anisotropy in the nearest-neighbor spin interactions that couple $N\geq 2$ consecutive spin-1/2 antiferromagnetic chains is studied theoretically by considering the limit where the coupling is purely of the Ising type. An…

Condensed Matter · Physics 2009-10-30 J. P. Rodriguez , P. D. Sacramento , V. R. Vieira

We present a model compound for the $S$=1/2 ferromagnetic Heisenberg chain composed of the verdazyl-based complex $[$Zn(hfac)$_2]$$[$4-Cl-$o$-Py-V-(4-F)$_2]$. $Ab$ $initio$ MO calculations indicate a predominant ferromagnetic interaction…

Strongly Correlated Electrons · Physics 2019-03-19 N. Uemoto , Y. Kono , S. Kittaka , T. Sakakibara , T. Yajima , Y. Iwasaki , S. Miyamoto , Y. Hosokoshi , H. Yamaguchi

The new antiferromagnetic (AF) compound BaCu_2Si_2O_7 is studied by magnetic susceptibility and neutron scattering techniques. The observed behavior is dominated by the presence of loosely coupled S=1/2 chains with the intrachain AF…

Strongly Correlated Electrons · Physics 2007-05-23 I. Tsukada , Y. Sasago , K. Uchinokura , A. Zheludev , S. Maslov , G. Shirane , K. Kakurai , E. Ressouche

The ground state magnetization process of the S=1 antiferromagnetic chain with the easy-axis single-ion anisotropy described by negative $D$ is investigated. It is numerically found that a phase transition between two different gapless…

Statistical Mechanics · Physics 2009-10-31 Toru Sakai

The anisotropy of magnetic properties commonly is introduced in textbooks using the case of an antiferromagnetic system with Ising type anisotropy. This model presents huge anisotropic magnetization and a pronounced metamagnetic transition…

Strongly Correlated Electrons · Physics 2017-04-12 K. Kliemt , M. Hofmann-Kliemt , K. Kummer , F. Yakhou-Harris , C. Krellner , C. Geibel

Complementary nature of coercivity enhancement and exchange bias is generalized from the layered systems to ferro-antiferromagnet (F-AF) exchange coupled systems with arbitrary configurations and is proved based on the coherent rotation of…

Materials Science · Physics 2009-11-11 Congxiao Liu , Min Sun , Hideo Fujiwara

The parent phases of the Fe-arsenide superconductors harbor an antiferromagnetic ground state. Significantly, the N\'eel transition is either preceded or accompanied by a structural transition that breaks the four fold symmetry of the…

Superconductivity · Physics 2011-09-30 I. R. Fisher , L. Degiorgi , Z. X. Shen

Competing magnetic interactions in low-dimensional quantum magnets can lead to the exotic ground state with fractionalized excitations. Herein, we present our results on an S = 5/2 quasi-one-dimensional spin system Bi3FeMo2O12. The…

We simulate the switching behavior of nanoscale synthetic antiferromagnets (SAFs), inspired by recent experimental progress in spin-orbit-torque switching of crystal antiferromagnets. The SAF consists of two ferromagnetic thin films with…

Mesoscale and Nanoscale Physics · Physics 2019-02-04 Michael S. Ackermann , Satoru Emori

We report on the magnetic properties of the supra-molecular compound iron(II) phthalocyanine in its alpha-form. dc- and ac-susceptometry measurements and Mossbauer experiments show that the iron atoms are strongly magnetically coupled into…

Condensed Matter · Physics 2007-05-23 M. Evangelisti , J. Bartolome , L. J. de Jongh , G. Filoti
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