English

GdRh$_2$Si$_2$: An exemplary tetragonal system for antiferromagnetic order with weak in-plane anisotropy

Strongly Correlated Electrons 2017-04-12 v1

Abstract

The anisotropy of magnetic properties commonly is introduced in textbooks using the case of an antiferromagnetic system with Ising type anisotropy. This model presents huge anisotropic magnetization and a pronounced metamagnetic transition and is well-known and well-documented both, in experiments and theory. In contrast, the case of an antiferromagnetic XX-YY system with weak in-plane anisotropy is only poorly documented. We studied the anisotropic magnetization of the compound GdRh2_2Si2_2 and found that it is a perfect model system for such a weak-anisotropy setting because the Gd3+^{3+} ions in GdRh2_2Si2_2 have a pure spin moment of S=7/2 which orders in a simple AFM structure with Q=(001){\bf Q} = (001). We observed experimentally in M(B)M(B) a continuous spin-flop transition and domain effects for field applied along the [100][100]- and the [110][110]-direction, respectively. We applied a mean field model for the free energy to describe our data and combine it with an Ising chain model to account for domain effects. Our calculations reproduce the experimental data very well. In addition, we performed magnetic X-ray scattering and X-ray magnetic circular dichroism measurements, which confirm the AFM propagation vector to be Q=(001){\bf Q} = (001) and indicate the absence of polarization on the rhodium atoms.

Keywords

Cite

@article{arxiv.1703.04114,
  title  = {GdRh$_2$Si$_2$: An exemplary tetragonal system for antiferromagnetic order with weak in-plane anisotropy},
  author = {K. Kliemt and M. Hofmann-Kliemt and K. Kummer and F. Yakhou-Harris and C. Krellner and C. Geibel},
  journal= {arXiv preprint arXiv:1703.04114},
  year   = {2017}
}