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The "trilobite" type of molecule, predicted in 2000 and observed experimentally in 2015, arises when a Rydberg electron exerts a weak attractive force on a neutral ground state atom. Such molecules have bond lengths exceeding 100 nm. The…

Atomic Physics · Physics 2018-10-02 Matthew T. Eiles , Zhengjia Tong , Chris H. Greene

A static electric field of a few V/cm shifts the energy levels of ultracold Rydberg atoms in a magneto-optical trap. For a given principle quantum number, most of the energy levels are nearly degenerate at zero field and fan out with…

When atoms are excited to high-lying Rydberg states they interact strongly with dipolar forces. The resulting state-dependent level shifts allow to study many-body systems displaying intriguing nonequilibrium phenomena, such as constrained…

Quantum Physics · Physics 2024-09-04 Chris Nill , Kay Brandner , Beatriz Olmos , Federico Carollo , Igor Lesanovsky

Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of…

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…

Atomic Physics · Physics 2021-07-14 Frederic Hummel , Matthew T. Eiles , Peter Schmelcher

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

Atomic Physics · Physics 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative…

We observe that when an ultracold ground state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit, ultralong-range molecules with giant (kilo-Debye) permanent electric dipole moments form. Large…

Atomic Physics · Physics 2015-06-23 Donald Booth , Seth Rittenhouse , Jin Yang , Hossein Sadeghpour , James Shaffer

We investigate the dynamical formation of crystalline states with systems of polar molecules or Rydberg atoms loaded into a deep optical lattice. External fields in these systems can be used to couple the atoms or molecules between two…

Quantum Gases · Physics 2015-03-13 J. Schachenmayer , I. Lesanovsky , A. Micheli , A. J. Daley

Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies.…

The laser-excitation of Rydberg atoms in ultracold gases is often described assuming that the atomic motion is frozen during the excitation time. We show that this frozen gas approximation can break down for atoms that are held in optical…

Atomic Physics · Physics 2013-05-23 W. Li , C. Ates , I. Lesanovsky

We present photo-excitation of ultra-long-range Rydberg molecules as a probe of spatial correlations in quantum gases. Rydberg molecules can be created with well-defined internuclear spacing, set by the radius of the outer lobe of the…

We calculate vibrational spectra of ultralong-range Cs(32p) Rydberg molecules which form in an ultracold gas of Cs atoms. We account for the partial-wave scattering of the Rydberg electrons from the ground Cs perturber atoms by including…

We investigate a hybrid system composed of ultracold Rydberg atoms immersed in an atomic Bose-Einstein condensate (BEC). The coupling between the Rydberg electrons and BEC atoms leads to the excitation of phonons, the exchange of which…

Quantum Gases · Physics 2015-06-24 Jia Wang , Marko Gacesa , Robin Côté

We investigate polyatomic ultralong-range Rydberg molecules consisting of three ground state atoms bound to a Rydberg atom via $s$- and $p$-wave interactions. By employing the finite basis set representation of the unperturbed Rydberg…

Atomic Physics · Physics 2016-08-03 Christian Fey , Markus Kurz , Peter Schmelcher

We consider the two-band Hubbard model, where electrons from different bands interact through an on-site one- and two-particle hybridization. The proposed Hamiltonian makes it possible to construct an effective theory and answer the…

Strongly Correlated Electrons · Physics 2026-01-07 Igor N. Karnaukhov

Circular Rydberg states offer advantages for quantum information and quantum simulation platforms due to their long lifetimes and strong dipole-dipole interactions. Unfortunately, current techniques for the production of these states remain…

Atomic Physics · Physics 2025-11-26 H. S. Parker , S. L. Sims , D. J. Lamphere , A. L. Harris

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

We develop a self-consistent approach that provides an explicit potential for a Rydberg electron whose ionic core consists of a polarizable medium, typically realized with superfluid droplets. The electron's motion remains separable in…

Atomic Physics · Physics 2026-02-23 Juan Carlos Acosta Matos , P. Giannakeas , Jan M. Rost

We review here the studies performed about interactions in an assembly of cold Rydberg atoms. We focus more specially the review on the dipole-dipole interactions and on the effect of the dipole blockade in the laser Rydberg excitation,…

Atomic Physics · Physics 2010-06-07 Daniel Comparat , Pierre Pillet
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