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Thermal properties in the metal/graphene (Gr) systems are analyzed by using an atomistic phonon transport model based on Landauer formalism and first-principles calculations. The specific structures under investigation include chemisorbed…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 R. Mao , B. D. Kong , C. Gong , S. Xu , T. Jayasekera , K. Cho , K. W. Kim

The half-Heusler (hH) compounds are currently considered promising thermoelectric (TE) materials due to their favorable thermopower and electrical conductivity. Accurate estimates of these properties are therefore highly desirable and…

Materials Science · Physics 2026-04-07 Vinod Kumar Solet , Sudhir K. Pandey

Density functional theory (DFT) based ab-initio calculations of electronic, phononic, and superconducting properties of 1T MoS2 are reported. The phonon dispersions are computed within density-functional-perturbation-theory (DFPT). We have…

Superconductivity · Physics 2021-07-08 Jagdish Kumar , Harkirat Singh

We predict high thermoelectric efficiency in the layered perovskite La$_2$Ti$_2$O$_7$, based on calculations (mostly ab-initio) of the electronic structure, transport coefficients, and thermal conductivity in a wide temperature range. The…

Materials Science · Physics 2019-03-06 Vincenzo Fiorentini , Roberta Farris , Edoardo Argiolas , Maria Barbara Maccioni

Critical thermoelectric parameters including Seebeck coefficient, electrical conductivity, thermal conductivity and figure of merit ZT of one-dimensional coaxial Bi2Te3/Sb2Te3 nanocomposite were modeled by following the single carrier…

Materials Science · Physics 2011-01-31 Qilin Gu

Dislocations can greatly enhance the figure of merit of thermoelectric materials by prominently reducing thermal conductivity. However, the evolution of phonon modes with different energies when they propagate through a single dislocation…

Applied Physics · Physics 2019-10-07 Yandong Sun , Yanguang Zhou , Jian Han , Wei Liu , Cewen Nan , Yuanhua Lin , Ming Hu , Ben Xu

Using Green's function equation of motion within Lacroix decoupling scheme, we examine the thermoelectric transport features of a strongly interacting quantum dot coupled between metallic leads. We demonstrate that a qualitative description…

Mesoscale and Nanoscale Physics · Physics 2023-08-22 Sachin Verma , B. S. Tewari , A. Dhyani , Ajay

We have investigated charge transport in ZnTPPdT-Pyr molecular junctions using the lithographic MCBJ technique at room temperature and cryogenic temperature (6K). We combined low-bias statistical measurements with spectroscopy of the…

The use of an asymmetric broadening in the transport distribution, a characteristic of resonant structures, is proposed as a route to engineer a decrease in electronic thermal conductivity thereby enhancing the electronic figure of merit in…

Mesoscale and Nanoscale Physics · Physics 2016-08-17 Urvesh Patil , Bhaskaran Muralidharan

Two-dimensional group IV transition-metal dichalcogenides have encouraging thermoelectric applications since their electronic and lattice properties can be manipulated with strain. In this paper, we report the thermoelectric parameters such…

Materials Science · Physics 2020-01-29 Ransell D'Souza , Sugata Mukherjee , Sohail Ahmad

We investigate phonon thermal transport of fullerene-based single-molecule junctions by employing classical molecular dynamics simulations. The thermal conductances of fullerene monomers, dimers, and trimers are computed through three…

Mesoscale and Nanoscale Physics · Physics 2024-02-12 Joanna Li , Jonathan J. Wang , Dvira Segal

This tutorial outlines the basic theoretical concepts and tools which underpin the fundamentals of phase-coherent electron transport through single molecules. The key quantity of interest is the transmission coefficient T(E), which yields…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 C J Lambert

The calculation of the nonlinear conductance of a single-molecule junction is revisited. The self energy on the junction resulting from the electron-phonon interaction has at low temperatures logarithmic singularities (in the real part) and…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 O. Entin-Wohlman , Y. Imry , A. Aharony

Within the Coulomb blockade regime, our study delves into the charge, spin, and thermoelectric transport characteristics in a benzene-based molecular nano-junction using the Pauli master equation and linear response theory. The charge- and…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Parbati Senapati , Prakash Parida

In order to improve the thermoelectric performance of TiCoSb we have substituted 50% of Ti equally with Zr and Hf at Ti site and Sb with Sn and Se equally at Sb site. The electronic structure of Ti0.5Zr0.25Hf0.25CoSn0.5Se0.5 is investigated…

Materials Science · Physics 2018-05-09 Mukesh K. Choudhary , P Ravindran

In this work we present a detailed study and derivation of the thermopower and thermoelectric coefficient of nano-granular metals at large tunneling conductance between the grains, g_T>> 1. An important criterion for the performance of a…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Andreas Glatz , I. S. Beloborodov

The principal paradigm for determining the thermoelectric properties of materials is based on the Boltzmann transport equations (BTEs) or Landauer equivalent. These equations depend on the electron and phonon density of states (e-DOS and…

Computational Physics · Physics 2024-11-05 J. A. Worden , M. R. von Spakovsky , C. Hin

The characteristics of molecular electronic devices are critically determined by metal-organic interfaces, which influence the arrangement of the orbital levels that participate in charge transport. Studies on self-assembled monolayers…

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

Mesoscale and Nanoscale Physics · Physics 2011-03-15 R. Härtle , M. Thoss

Introducing hierarchical disorder from multiple defects into materials through nanostructuring is one of the most promising directions to achieve extremely low thermal conductivities and thus improve thermoelectric performance. The success…

Materials Science · Physics 2019-09-16 Laura de Sousa Oliveira , Vassilios Vargiamidis , Neophytos Neophytou
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