Related papers: $S$ = 1/2 ferromagnetic-antiferromagnetic alternat…
We present a model compound for the $S$=1/2 ferromagnetic Heisenberg chain composed of the verdazyl-based complex $[$Zn(hfac)$_2]$$[$4-Cl-$o$-Py-V-(4-F)$_2]$. $Ab$ $initio$ MO calculations indicate a predominant ferromagnetic interaction…
We present the first experimental realization of an $S=2$ ferromagnetic-antiferromagnetic (F-AF) alternating chain in a new Mn-verdazyl complex [Mn(hfac)$_2$]$\cdot$($o$-Py-V) [hfac=1,1,1,5,5,5-hexafluoroacetylacetonate;…
The thermodynamic properties of a spin S=1/2 tetrameric Heisenberg antiferromagnetic chain with alternating interactions AF1-AF2-AF1-F (AF and F denote the antiferromagnetic and ferromagnetic couplings, respectively) are studied by means of…
The $S=1$ antiferromagnetic Heisenberg chain both with and without single ion anisotropy is studied. Using the recently proposed density matrix renormalization group technique we calculate the energy gaps as well as several different…
We have succeeded in synthesizing single crystals of the verdazyl radical beta-2,6-Cl2-V [= beta-3-(2,6-dichlorophenyl)-1,5-diphenylverdazyl]. The ab initio MO calculation indicated the formation of an S = 1/2 Heisenberg antiferromagnetic…
We present a study of the spin-1/2 Heisenberg chain with alternating ferro- and antiferromagnetic exchange, focusing on the role of the exchange couplings to cover both, dimer and Haldane limit. Employing a complementary combination of…
Magnetic excitations of the quasi-1D S=1/2 Heisenberg antiferromagnet (HAF) Cs2CuCl4 have been measured as a function of magnetic field using neutron scattering. For T<0.62 K and B=0 T the weak inter-chain coupling produces 3D…
We successfully synthesize single crystals of the verdazyl radical $\alpha$-2,3,5-Cl$_3$-V. $Ab$ $initio$ molecular orbital calculations indicate that the two dominant antiferromagnetic interactions, $J_{\rm{1}}$ and $J_{\rm{2}}$ ($\alpha…
In this article, we study the one dimensional Heisenberg spin-1/2 alternating bond chain in which the nearest neighbor exchange couplings are ferromagnetic (FM) and antiferromagnetic (AF) alternatively. By using exact diagonalization and…
We successfully synthesized a verdazyl-based complex, ($p$-Py-V-$p$-CN)$_2$[Cu(hfac)$_2$]. Molecular orbital calculations reveal that three types of antiferromagnetic (AF) interactions are involved in the formation of a spin-1/2 distorted…
The ground-state properties of a spin $S=1/2$ tetrameric Heisenberg antiferromagnetic chain with alternating couplings AF$_{1}$-AF$_{2}$-AF$_{1}$% -F (AF and F denote antiferromagnetic and ferromagnetic couplings, respectively) are studied…
We study Heisenberg spin-1/2 and spin-1 chains with alternating ferromagnetic ($J_1^F$) and antiferromagnetic ($J_1^A$) nearest-neighbor interactions and a ferromagnetic next-nearest-neighbor interaction ($J_2^F$). In this model frustration…
Inelastic neutron scattering on deuterated single-crystal samples is used to study Haldane-gap excitations in the new S=1 one-dimensional quantum antiferromagnet NDMAP, that was recently recognized as an ideal model system for high-field…
We calculate the excitation spectrum and spectral weights of the alternating antiferromagnetic-ferromagnetic spin-half Heisenberg chain with exchange couplings $J$ and $-|\lambda|J$ as a power series in $\lambda$. For small $|\lambda|$, the…
Inelastic neutron scattering is employed to study transverse spin correlations of a Heisenberg $S=1/2$ chain compound in a magnetic field of 7.5 T. The target compound is the antiferromagnetic Heisenberg $S=1/2$ chain material…
By means of electron spin resonance investigations we revealed the crucial role of the interchain coupling in the spin dynamics of the spin-1/2 Heisenberg antiferromagnetic (AF) chain material copper-pyrazine-dinitrate,…
We study the spin-1/2 antiferromagnetic Heisenberg chain in both uniform and (perpendicular) staggered magnetic fields using the density-matrix renormalization-group method. This model has been shown earlier to describe the physics of the…
An $S=1/2$ ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain model is investigated in connection to its realization compound: (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$. The exchange interaction…
The magnetic susceptibility of the $S = 2$ quasi-linear chain Heisenberg antiferromagnet (2,$2'$-bipyridine)trichloromanganese(III), MnCl_{3}(bipy), has been measured from 1.8 to 300 K with the magnetic field, H, parallel and perpendicular…
The molecular coordination complex NiI$_2$(3,5-lut)$_4$ [where (3,5-lut) $=$ (3,5-lutidine) $=$ (C$_7$H$_9$N)] has been synthesized and characterized by several techniques including synchrotron X-ray diffraction, ESR, SQUID magnetometry,…