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Skins of water and ice share the same attribute of supersolidity characterized by the identical H-O vibration frequency of 3450 cm-1. Molecular undercoordination and inter-electron-pair repulsion shortens the H-O bond and lengthen the O:H…

Chemical Physics · Physics 2014-09-26 Xi Zhang , Yongli Huang , Zengsheng Ma , Yichun Zhou , Weitao Zheng , Ji Zhou , Chang Q. Sun

Because of the segmental specific-heat disparity of the hydrogen bond (O:H-O) and the Coulomb repulsion between oxygen ions, cooling elongates the O:H-O bond at freezing by stretching its containing angle and shortening the H-O bond with an…

Soft Condensed Matter · Physics 2015-01-20 Chang Q. Sun

Consistency between theory predictions and measurements and calculations revealed that the skin of ice, containing water molecules with fewer than four neighbours, forms a supersolid phase that is highly polarized, elastic, hydrophobic,…

Soft Condensed Matter · Physics 2013-10-04 Xi Zhang , Yongli Huang , a Zengsheng Ma , Yichun Zhou , Chang Q Sun

Unlike other unusual materials whose bonds contract under compression, the O:H nonbond undergoes contraction and the H-O bond elongation towards O:H and H-O length symmetry in water and ice. The energy drop of the H-O bond dictates the…

Soft Condensed Matter · Physics 2015-01-29 Chang Q Sun

Compression shortens the O:H nonbond and lengthens the H-O bond simultaneously via O:H-O Coulomb repulsion. The energy loss of the elongated H-O bond lowers the melting point.

Soft Condensed Matter · Physics 2015-09-22 Chang Q. Sun

Molecular undercoordination shortens and stiffens the H-O bond but lengthens and softens the O:H nonbond simultaneously associated with O 1s energy entrapment and nonbonding electron dual polarization, which dictates behavior of water and…

Soft Condensed Matter · Physics 2015-02-24 Chang Q. Sun

We examined O:H-O bond relaxation under compression,heating,molecular undercoordination and claimed a universal resolution to the best-known mysteries of water ice such as ice foating, ice slipperiness, relegation and warm water cools…

Soft Condensed Matter · Physics 2018-09-06 Yongli Huang , Xi Zhang , Chang Q Sun

Coulomb repulsion between the bonding electron pair in the H-O covalent bond (denoted by "-") and the nonbonding electron pair of O (":") and the specific-heat disparity between the O:H and the H-O segments of the entire hydrogen bond…

Chemical Physics · Physics 2013-10-08 Chang Q. Sun

The interplay between intra-molecular H-O covalent bond contraction, due to molecular under-coordination, and inter-molecular O:H expansion, due to inter-electron pair Coulomb repulsion, has been shown to be the source of the anomalous…

Chemical Physics · Physics 2013-10-08 Chang Q. Sun

Coulomb repulsion between the unevenly-bound bonding and nonbonding electron pairs in the O:H-O hydrogen-bond is shown to originate the anomalies of ice under compression. Consistency between experimental observations, density functional…

Chemical Physics · Physics 2013-10-08 Chang Q Sun , Xi Zhang , Weitao Zheng

The segmental specific heat ratio of the couple hydrogen bond defines not only the phase of Vapor, Liquid, Ice I and XI phase with a quasisolid phase that shows the negative thermal extensibility but uniquely the slope of density of water…

Chemical Physics · Physics 2020-12-03 Chang Q Sun

Hydrogen-bond forms a pair of asymmetric, coupled, H-bridged oscillators with ultra-short-range interactions and memory. hydrogen bond cooperative relaxation and the associated binding electron entrapment and nonbonding electron…

Soft Condensed Matter · Physics 2015-01-16 Chang Q Sun

Molecular undercoordination induced O:H-O bond relaxation and dual polarization dictates the supersolid behavior of water skins interacting with other substances such as flowing in nanochannels, dancing of water droplets, floating of…

Soft Condensed Matter · Physics 2015-02-27 Chang Q. Sun

The mysterious nature and functionality of water and ice skins remain baffling to the community since 1859 when Farady firstly proposed liquid skin lubricating ice. Here we show the presence of supersolid phase that covers both water and…

Soft Condensed Matter · Physics 2014-09-26 Chang Q Sun

A sequential of concepts developed in last decade has enabled a resolution to multiple anomalies of water ice and its low-dimensionality, particularly. Developed concepts include the coupled hydrogen bond oscillator pair, segmental specific…

Soft Condensed Matter · Physics 2020-06-17 Chang Q Sun

The low kinetic friction between ice and numerous counterbodies is commonly attributed to an interfacial water layer, which is believed to originate from pre-existing surface water or from melt water induced by high contact pressures or…

Soft Condensed Matter · Physics 2025-09-03 Achraf Atila , Sergey V. Sukhomlinov , Martin H. Müser

Super-cooled liquids are characterized by their fragility: the slowing down of the dynamics under cooling is more sudden and the jump of specific heat at the glass transition is generally larger in fragile liquids than in strong ones.…

Disordered Systems and Neural Networks · Physics 2014-01-14 Le Yan , Gustavo Düring , Matthieu Wyart

Coulomb repulsion between the unevenly-bounded bonding "-" and nonbonding ":" electron pairs in the "O2- : H+/p-O2-" hydrogen-bond is found to originate the anomalies of low-compressibility, phonon relaxation dynamics, proton symmetrization…

Other Condensed Matter · Physics 2011-10-13 Chang Q Sun , Xi Zhang , Weitao Zheng

The friction of a stationary moving skate on smooth ice is investigated, in particular in relation to the formation of a thin layer of water between skate and ice. It is found that the combination of ploughing and sliding gives a friction…

Other Condensed Matter · Physics 2018-01-22 J. M. J. van Leeuwen

Laboratory experiments revealed that CO$_{2}$ ice particles stick less efficiently than H$_{2}$O ice particles, and there is an order of magnitude difference in the threshold velocity for sticking. However, the surface energies and elastic…

Earth and Planetary Astrophysics · Physics 2021-04-14 Sota Arakawa , Sebastiaan Krijt
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