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Coulomb explosion imaging (CEI) is a powerful technique for capturing the real-time motion of individual atoms during ultrafast photochemical reactions. CEI generates high-dimensional data with naturally embedded correlations that allow…

Evaluating multi-center molecular integrals with Cartesian Gaussian-type basis sets has been a long-standing bottleneck in electronic structure theory calculation for solids and molecules. We have developed a vector-coupling and…

Quantum Physics · Physics 2024-05-17 Hang Hu , Gilles Peslherbe , Hsu Kiang Ooi , Anguang Hu

A molecule can be optically accelerated to rotate unidirectionally at a frequency of a few terahertzes which is many orders higher than the classical mechanical rotor. Such a photon-induced ultrafast molecular unidirectional rotation has…

We demonstrate a spatial-imaging thermometry technique for ions in a one-dimensional Coulomb crystal by relating their imaged spatial extent along the linear radiofrequency ion trap axis to normal modes of vibration of coupled oscillators…

Atomic Physics · Physics 2016-02-11 V. Rajagopal , J. P. Marler , M. G. Kokish , B. C. Odom

The previously applied independent atom model (IAM) for highly charged ion-molecule collisions which implemented the suppression of multiple ionization and capture on the basis of geometric overlaps of cross-sectional areas representing…

Atomic Physics · Physics 2025-09-15 Hans Jürgen Lüdde , Marko Horbatsch , Tom Kirchner

We present a thermal velocity sampling method for calculating Doppler-broadened atomic spectra, which more efficiently reaches a smooth limit than regular velocity weighted sampling. The method uses equal-population sampling of the 1-D…

Velocity map imaging inside an electrostatic quadrupole guide is demonstrated. By switching the voltages that are applied to the rods, the quadrupole can be used for guiding Stark decelerated molecules and for extracting the ions. The…

Chemical Physics · Physics 2017-08-23 Marina Quintero Pérez , Paul Jansen , Hendrick L. Bethlem

Traditionally, measuring the center-of-mass (c.m.) velocity of an atomic ensemble relies on measuring the Doppler shift of the absorption spectrum of single atoms in the ensemble. Mapping out the velocity distribution of the ensemble is…

Atomic Physics · Physics 2020-03-10 Zilong Chen , Hong Ming Lim , Chang Huang , Rainer Dumke , Shau-Yu Lan

A novel locally statistical active contour model (ACM) for image segmentation in the presence of intensity inhomogeneity is presented in this paper. The inhomogeneous objects are modeled as Gaussian distributions of different means and…

Computer Vision and Pattern Recognition · Computer Science 2013-05-31 Kaihua Zhang , Lei Zhang , Kin-Man Lam , David Zhang

We report on the design and performance of a double-sided coincidence velocity map imaging spectrometer optimized for electron-ion and ion-ion coincidence experiments studying inner-shell photoionization of gas-phase molecules with soft…

We present a novel approach to model ultrafast time-dependent nonlinear optical polarization sensitive signals emitted from randomly-oriented molecules. By projecting the laboratory-frame analyzer polarization axis into the molecular frame…

Chemical Physics · Physics 2025-07-17 R. L. Thurston , N. Shivaram , Th. Weber , L. Z. Tan , D. S. Slaughter

We propose a method to investigate the vibrational dynamics of single polyatomic molecular ions confined in a Paul trap. Quantum logic techniques are employed to detect the recoil of single photon absorption events in the molecule via a…

Quantum Physics · Physics 2019-08-27 Philipp Schindler

We present the design of a Velocity Map Imaging apparatus tailored to the demands of high-resolution crossed molecular beam experiments employing Stark or Zeeman decelerators. The key requirements for these experiments consist of the…

Atomic Physics · Physics 2021-11-09 Vikram Plomp , Zhi Gao , Sebastiaan Y. T. van de Meerakker

A novel electromagnetic quantitative inversion scheme for translationally moving targets via phase correlation registration of back-projection (BP) images is proposed. Based on a time division multiplexing multiple-input multiple-output…

Image and Video Processing · Electrical Eng. & Systems 2025-11-20 Yitao Lin , Dahai Dai , Shilong Sun , Yuchen Wu , Bo Pang

In indirect measurements, the measurand is determined by solving an inverse problem which requires a model of the measurement process. Such models are often approximations and introduce systematic errors leading to a bias of the posterior…

Methodology · Statistics 2025-09-22 Maren Casfor , Philipp Trunschke , Sebastian Heidenreich , Nando Hegemann

We propose and implement a fast, universally applicable method for extracting the angular power spectrum C_l from CMB temperature maps by first estimating the correlation function \xi(\theta). Our procedure recovers the C_l's using N^2 (but…

In this paper, we consider the intensity-based inversion method (IIM) for quantitative material parameter estimation in quasi-static elastography. In particular, we consider the problem of estimating the material parameters of a given…

Numerical Analysis · Mathematics 2026-01-19 Ekaterina Sherina , Simon Hubmer

Accurate diagnosis of breast cancer in histopathology images is challenging due to the heterogeneity of cancer cell growth as well as of a variety of benign breast tissue proliferative lesions. In this paper, we propose a practical and…

Computer Vision and Pattern Recognition · Computer Science 2020-05-06 Xingyu Li , Marko Radulovic , Ksenija Kanjer , Konstantinos N. Plataniotis

We consider electron systems in quantum dots and imaging of the confined charge density by the Coulomb blockade microscopy (CBM) with the scanning probe technique. We apply an exact diagonalization method to study the reaction of the…

Mesoscale and Nanoscale Physics · Physics 2014-06-27 E. Wach , D. P. Żebrowski , B. Szafran