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Frontier orbitals, i.e., the highest occupied and lowest unoccupied orbitals of a molecule, generally determine molecular properties, such as chemical bonding and reactivities. Consequently, there has been a lot of interest in measuring…

In superconducting linear accelerators (linacs), accurately monitoring beam dynamics is essential for minimizing beam losses and ensuring stable operations. However, destructive diagnostics must be avoided in superconducting sections to…

We solve analytically the out-of-equilibrium initial stage that follows the injection of a radially finite electron beam into a plasma at rest and test it against particle-in-cell simulations. For initial large beam edge gradients and not…

Plasma Physics · Physics 2009-11-11 M. -C. Firpo , A. F. Lifschitz , E. Lefebvre , C. Deutsch

Scanning Transmission Electron Microscopy (STEM) has become the main stay for materials characterization on atomic level, with applications ranging from visualization of localized and extended defects to mapping order parameter fields. In…

Instrumentation and Detectors · Physics 2019-01-15 Xin Li , Ondrej Dyck , Sergei V. Kalinin , Stephen Jesse

Time-resolved spectroscopy provides the main tool for analyzing the dynamics of excitonic energy transfer in light-harvesting complexes. To infer time-scales and effective coupling parameters from experimental data requires to develop…

Chemical Physics · Physics 2018-11-28 Tobias Kramer , Mirta Rodriguez , Yaroslav Zelinskyy

Recent advances in transmission electron microscopy (TEM) have opened the path toward spin resonance spectroscopy with single-spin sensitivity. To assess this potential, we investigate the quantum precision limits for sensing magnetic…

We introduce the construction of a orthogonal wavepacket basis set, using the concept of stroboscopic time propagation, tailored to the efficient description of non-equilibrium extended electronic systems. Thanks to three desirable…

Materials Science · Physics 2008-08-08 P. Bokes , F. Corsetti , R. W. Godby

The coaxial wire method is a common and appreciated technique to assess the beam coupling impedance of an accelerator element from scattering parameters. Nevertheless, the results obtained from wire measurements could be inaccurate due to…

Accelerator Physics · Physics 2024-06-17 Antuono Chiara , Zannini Carlo , Mostacci Andrea , Migliorati Mauro

Use of electron vortex beams (EVB), that is convergent electron beams carrying an orbital angular momentum (OAM), is a novel development in the field of transmission electron microscopy. They should allow measurement of element-specific…

Materials Science · Physics 2015-06-19 Jan Rusz , Somnath Bhowmick , Mattias Eriksson , Nikolaj Karlsson

We present an experimental demonstration of closed-loop quantum parameter estimation in which real-time feedback is used to achieve robustness to modeling uncertainty. By performing broadband estimation of a magnetic field acting on…

Quantum Physics · Physics 2007-05-23 JM Geremia , John K. Stockton , Hideo Mabuchi

The electron beam propagation in a plasma medium is susceptible to several instabilities. In the relativistic regime typically the weibel instability leading to the current separation dominates. The linear instability analysis is carried…

Plasma Physics · Physics 2015-09-11 Chandrasekhar Shukla , Amita Das , Kartik Patel

Tracking the kinematics of fast-moving objects is an important diagnostic tool for science and engineering. Existing optical methods include high-speed CCD/CMOS imaging, streak cameras, lidar, serial time-encoded imaging and sequentially…

The concept of compressive sensing was recently proposed to significantly reduce the electron dose in scanning transmission electron microscopy (STEM) while still maintaining the main features in the image. Here, an experimental setup based…

Instrumentation and Detectors · Physics 2016-03-23 Armand Béché , Bart Goris , Bert Freitag , Jo Verbeeck

Precession of a converged beam during acquisition of a 4D-STEM dataset improves strain, orientation, and phase mapping accuracy by averaging over continuous angles of illumination. Precession experiments usually rely on integrated systems,…

Instrumentation and Detectors · Physics 2025-10-20 Stephanie M. Ribet , Rohan Dhall , Colin Ophus , Karen C. Bustillo

A resonance method of measuring the electric dipole moment (EDM) of nuclei in storage rings is described, based on two new ideas: (1) Oscillating particles' velocities in resonance with spin precession, and (2) alternately producing two…

High Energy Physics - Experiment · Physics 2009-11-11 Yuri F. Orlov , William M. Morse , Yannis K. Semertzidis

Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…

Mesoscale and Nanoscale Physics · Physics 2024-10-29 Rachel Gelfand , Matthew Pelton

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

One of the primary uses for transmission electron microscopy (TEM) is to measure diffraction pattern images in order to determine a crystal structure and orientation. In nanobeam electron diffraction (NBED) we scan a moderately converged…

We presented a new method for measuring the squares of the amplitudes and phases of partial vortex-beams in a complex beam array in real time. The method is based on measuring the high-order intensity moments and analyzing the solutions of…

Optics · Physics 2018-12-05 A. Volyar , M. Bretsko , Ya. Akimova , Yu. Egorov