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By many-body quantum-chemical calculations, we investigate the role of two structural effects - local ligand distortions and the anisotropic Cd-ion coordination - on the magnetic state of Cd2Os2O7, a spin S=3/2 pyrochlore. We find that…

Strongly Correlated Electrons · Physics 2013-03-28 Nikolay A. Bogdanov , Rémi Maurice , Ioannis Rousochatzakis , Jeroen van den Brink , Liviu Hozoi

We report structural and magnetic properties studies of large high quality single-crystals of the frustrated magnet, Nd$_2$Zr$_2$O$_7$. Powder x-ray diffraction analysis confirms that Nd$_2$Zr$_2$O$_7$ adopts the pyrochlore structure.…

Strongly Correlated Electrons · Physics 2015-05-18 M. Ciomaga Hatnean , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan , M. J. Gutmann , V. V. Klekovkina , B. Z. Malkin

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

Geometrical frustration and spin-orbit coupling effect together play vital role to influence properties in pyrochlore based iridium oxides. Here we have investigated detailed structural, magnetic, thermodynamic and transport properties of…

Strongly Correlated Electrons · Physics 2017-02-06 Harish Kumar , A. K. Pramanik

We report low-temperature susceptibility and magnetisation data for the cubic pyrochlore Er2Ti2O7. By performing the measurements on single crystals we are able to establish the degree of magnetic anisotropy present in this compound and to…

Strongly Correlated Electrons · Physics 2013-10-08 O. A. Petrenko , M. R. Lees , G. Balakrishnan

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

We have measured neutron diffraction patterns in a single crystal sample of the pyrochlore compound Er$_2$Ti$_2$O$_7$ in the antiferromagnetic phase (T=0.3\,K), as a function of the magnetic field, up to 6\,T, applied along the [110]…

Strongly Correlated Electrons · Physics 2015-05-19 H. B. Cao , I. Mirebeau , A. Gukasov , P. Bonville , C. Decorse

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…

Below $T_N = 1.1$K, the XY pyrochlore Er$_2$Ti$_2$O$_7$ orders into a $k=0$ non-collinear, antiferromagnetic structure referred to as the $\psi_2$ state. The magnetic order in Er$_2$Ti$_2$O$_7$ is known to obey conventional three…

Pronounced anisotropy of magnetic properties and complex magnetic order of a new oxi-halide compound Co7(TeO3)4Br6 has been investigated by powder and single crystal neutron diffraction, magnetization and ac susceptibility techniques.…

Materials Science · Physics 2013-05-29 M. Prester , I. Zivkovic , O. Zaharko , D. Pajic , P. Tregenna-Piggott , H. Berger

Magnetization (M) and magnetoresistance (MR) measurements on polycrystalline R2Mn3Si5 (R = Tb, Dy and Ho) compounds (tetragonal, space group P4/mnc) have been carried out in the temperature range of 2 K-300 K, in various applied fields.…

Materials Science · Physics 2009-11-11 R. Nirmala , S. K. Malik , A. V. Morozkin , Y. Yamamoto , H. Hori

We report magnetization data for several titanium pyrochlore systems measured down to 0.5 K. The measurements, performed on single crystal samples in fields of up to 7 T, have captured the essential elements of the previously reported phase…

Strongly Correlated Electrons · Physics 2014-08-18 O. A. Petrenko , M. R. Lees , G. Balakrishnan

We demonstrate the appearance of thermal order by disorder in Ising pyrochlores with staggered antiferromagnetic order frustrated by an applied magnetic field. We use a mean-field cluster variational method, a low-temperature expansion and…

A number of recent experiments exhibit electronic anisotropy in the iron pnictides, and there is a growing body of experimental evidence that its origin is related to orbital ordering in Fe d_{xz} and d_{yz} orbitals. We examine this…

Strongly Correlated Electrons · Physics 2011-04-12 Andriy H. Nevidomskyy

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. L. Cornelius , J. S. Gardner

Using Raman scattering spectroscopy, we uncover a complex magnetic behavior of Nd$_2$Ir$_2$O$_7$ , which stands out among magnetic pyrochlores by the lowest temperature of the all-in-all-out (AIAO) Ir moments ordering…

We study magnetic behaviour of the Yb$^{3+}$ ions on a frustrated pyrochlore lattice in the spinel {\CYS}. The crystal-electric field parameters deduced from high-energy inelastic neutron scattering reveal well-isolated ytterbium ground…

Strongly Correlated Electrons · Physics 2019-09-18 K. Guratinder , Jeffrey G. Rau , V. Tsurkan , C. Ritter , J. Embs , T. Fennell , H. C. Walker , M. Medarde , T. Shang , A. Cervellino , Ch. Rüegg , O. Zaharko

The pyrochlore magnet Tb$_{2}$Ti$_{2}$O$_{7}$ shows a lack of magnetic order to low temperatures and is considered to be a quantum spin liquid candidate. We perform time-domain THz spectroscopy on high quality Tb$_{2}$Ti$_{2}$O$_{7}$…

Strongly Correlated Electrons · Physics 2021-04-21 Xinshu Zhang , Yi Luo , T. Halloran , J. Gaudet , Huiyuan Man , S. M. Koohpayeh , N. P. Armitage

Temperature dependent Raman scattering measurements have been performed to explore unusual coupling between magnetism and crystal structure in doped pyrochlore iridate Y$_2$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ with $x$ = 0.0, 0.05 and 0.2. The…

Strongly Correlated Electrons · Physics 2019-02-20 Harish Kumar , V. G. Sathe , A. K. Pramanik

We present the results of susceptibility \chi(T) and magnetisation M(H) measurements performed on single crystal samples of the rare-earth oxides SrLn2O4 (Ln = Er, Dy and Ho). The measurements reveal the presence of magnetic ordering…

Strongly Correlated Electrons · Physics 2012-01-17 Thomas J. Hayes , Olga Young , Geetha Balakrishnan , Oleg A. Petrenko