English

Nonequilibrium low temperature phase in pyrochlore iridate Y$_2$Ir$_2$O$_7$: Possibility of glass-like dynamics

Strongly Correlated Electrons 2017-02-06 v1

Abstract

Geometrical frustration and spin-orbit coupling effect together play vital role to influence properties in pyrochlore based iridium oxides. Here we have investigated detailed structural, magnetic, thermodynamic and transport properties of pyrochlore iridate Y2_2Ir2_2O7_7. Magnetization data show onset of magnetic irreversibility around temperature TirrT_{irr} \sim 160 K, however, no sign of long-range type ferromagnetic ordering is observed below TirrT_{irr}. Specific heat data show no visible anomaly across TirrT_{irr}, and the analysis of data indicate sizable density of states across Fermi level. Temperature dependent x-ray diffraction measurements show no change in structural symmetry down to low temperature. The material, on the other hand, shows significant relaxation and aging behavior similar to glassy dynamics. The electronic charge transport in this highly insulating system is found to follow power law dependence with temperature. The material shows negative magnetoresistance which is explained with quantum interference effect.

Keywords

Cite

@article{arxiv.1512.00233,
  title  = {Nonequilibrium low temperature phase in pyrochlore iridate Y$_2$Ir$_2$O$_7$: Possibility of glass-like dynamics},
  author = {Harish Kumar and A. K. Pramanik},
  journal= {arXiv preprint arXiv:1512.00233},
  year   = {2017}
}