Related papers: Single molecule imaging with longer x-ray laser pu…
We report the initial demonstrations of the use of single crystals in indirect x-ray imaging for x-ray phase contrast imaging at the Washington University in St. Louis Computational Bioimaging Laboratory (CBL). Based on single Gaussian peak…
In this paper, we propose a new method to characterize the temporal structure of arbitrary optical laser pulses with low pulse energies. This approach is based on strong field photoelectron holography with the glory rescattering effect as…
The photoelectron momentum distribution in the strong-field ionization has a variety of structures that reveal the complicated dynamics of this process. Recently, we identified a low-energy interference structure in the case of a…
Time-resolved femtosecond x-ray diffraction patterns from laser-excited molecular iodine are used to create a movie of intramolecular motion with time and space resolution of $30~$fs and $0.3$ \AA . The high spatial fidelity is due to…
Glutaraldehyde (GA) reacts with amino groups in proteins, forming intermolecular cross-links that, at sufficiently high protein concentration, can transform a protein solution into a gel. Although GA has been used as a cross-linking reagent…
We solve the orientation recovery of a tumbling protein in the gas phase from single-event measurements of the spatial positions of its ions after an X-ray laser induced explosion. We simulate diffracted X-ray signal and ion dynamics under…
All-optical Compton sources are innovative, compact devices to produce high energy femtosecond X-rays. Here we present results on a single-pulse scheme that uses a plasma mirror to reflect the drive beam of a laser plasma accelerator and to…
We present a novel, highly versatile, and self-referenced arrival time monitor for measuring the femtosecond time delay between a hard X-ray pulse from a free-electron laser and an optical laser pulse, measured directly on the same sample…
We investigate parametric X-ray radiation (PXR) under condition of the extremely asymmetric diffraction, when the ultra-relativistic electron bunch is moving in \textit{vacuum} parallel to the crystal-vacuum interface, close to the crystal…
The first numerical simulation of the process of ionization of an atom adsorbed on a metal surface by the subfemtosecond pulse is presented. The streaking scheme is considered, when a weak sub-femtosecond pulse comes together with a strong…
Tuneable ultrafast laser pulses are a powerful tool for measuring difficult-to-access degrees of freedom in materials science. In general these experiments require the ability to address resonances and excitations both above and below the…
Emerging coherent X-ray scattering patterns of single particles have shown dominant morphological signatures in agreement with predictions of the scattering model used for conventional protein crystallography. The key question is if and to…
We report the experimental demonstration of femtosecond electron diffraction using high-brightness MeV electron beams. High-quality, single-shot electron diffraction patterns for both polycrystalline aluminum and single-crystal 1T-TaS2 are…
We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…
Ultrahigh peak power femtosecond laser pulses create extreme states of matter that are currently being probed with great interest. Plasma optics have been proposed for shaping and amplifying high-power pulses, but they are subject to huge…
Obtaining 3D information from a single X-ray exposure at high-brilliance sources, such as X-ray free-electron lasers (XFELs) [1] or diffraction-limited storage rings [2], allows the study of fast dynamical processes in their native…
Self-action nonlinearity is a key aspect -- either as a foundational element or a detrimental factor -- of several optical spectroscopies and photonic devices. Supercontinuum generation, wavelength converters and chirped pulse amplification…
We present the first fundamental simulation method for the determination of crater morphology due to femtosecond-pulse laser damage. To this end we have adapted the particle-in-cell (PIC) method commonly used in plasma physics for use in…
We study the possibility of efficient self-compression of femtosecond laser pulses in nonlinear media with anomalous dispersion of group velocity during the self-focusing of wave packets with a power several times greater than the critical…
Although ultrafast laser materials processing has advanced at a breakneck pace over the last two decades, most applications have been developed with laser pulses at near-IR or visible wavelengths. Recent progress in mid-infrared (MIR)…