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The hyperfine structure of 5snd ^1D_2 states in ^{87}Sr was studied for principal quantum numbers 11 <= n <= 25 by Doppler-free two-photon excitation combined with thermionic detection. Based on the more accurate data, compared to previous…

Atomic Physics · Physics 2009-10-30 J. Guedde , A. Klinkmueller , P. J. West , E. Matthias

Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals).…

Atomic Physics · Physics 2016-06-01 V. A. Dzuba , V. V. Flambaum

We investigate the microwave spectra of ultracold alkali metal dimers in magnetic, electric and combined fields, taking account of the hyperfine structure due to the nuclear spins. We consider the molecules 41K87Rb and 7Li133Cs, which are…

Chemical Physics · Physics 2015-05-14 Hong Ran , J. Aldegunde , Jeremy M. Hutson

In the framework of the multiconfiguration Dirac-Hartree-Fock method, we investigate the transition properties of four excited states in the $2p^53s$ configuration of neutral neon. The electron correlation effects are taken into account…

Atomic Physics · Physics 2015-06-12 Jiguang Li , Per Jönsson , Michel Godefroid , Gediminas Gaigalas

We consider the proximity effect in multiterminal ferromagnet superconductor (FSF) hybrid structures in which two or three electrodes are connected to a superconductor. We show that two competing effects take place in these systems: (i)…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 H. Jirari , R. Mélin , N. Stefanakis

We present state-of-the-art configuration interaction and coupled cluster calculations of the electron electric dipole moment, the nucleon-electron scalar-pseudoscalar, and the magnetic hyperfine interaction constants ($\alpha_{d_e},…

Atomic Physics · Physics 2019-10-28 Timo Fleig , Leonid V. Skripnikov

We report first ab initio relativistic correlation calculations of potential curves for ten low-lying electronic states, effective electric field on the electron and hyperfine constants for the ^3\Delta_1 state of cation of a heavy…

Atomic Physics · Physics 2013-05-29 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov

Because molecules can have their orientation locked when embedded into a solid rare-gas matrix, their hyperfine structure is strongly perturbed relative to the freely rotating molecule. The addition of an electric field further perturbs the…

Atomic Physics · Physics 2018-10-03 A. C. Vutha , M. Horbatsch , E. A. Hessels

Strong electron-electron interactions are known to significantly modify the electron-phonon coupling relative to the predictions of density functional theory, but this effect is challenging to calculate with realistic theories of strongly…

Strongly Correlated Electrons · Physics 2025-07-21 David J. Abramovitch , Jennifer Coulter , Sophie Beck , Andrew Millis

A method and codes for two-step correlation calculation of heavy-atom molecules have been developed, employing the generalized relativistic effective core potential and relativistic coupled cluster (RCC) methods at the first step, followed…

Chemical Physics · Physics 2009-11-07 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov , V. F. Ezhov , E. Eliav , U. Kaldor

We report on high-resolution laser spectroscopy of $^{255}$Fm ($T_{1/2} = 20$h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4~nm and…

Large-scale self-consistent multiconfiguration Dirac--Hartree--Fock and relativistic configuration interaction calculations are reported for the $n \leq 6$ levels in Be-like ions from B II to Ne VII. Effects from electron correlation are…

A precise theoretical study of the electronic structure of heavy atom diatomic molecules is of key importance to interpret the experiments in the search for violation of time-reversal (T) and spatial-parity (P) symmetries of fundamental…

Atomic Physics · Physics 2016-12-02 L. V. Skripnikov

This work presents accurate ab initio determination of the hyperfine splitting for the ground state and few low-lying excited states of 113Cd+; important candidates for the frequency standard in the microwave region, using coupled-cluster…

Atomic Physics · Physics 2009-11-13 Gopal Dixit , H. S. Nataraj , B. K. Sahoo , R. K. Chaudhuri , Sonjoy Majumder

The dipole moment is a crucial molecular property linked to a molecular system's bond polarity and overall electronic structure. To that end, the electronic dipole moment, which results from the electron density of a system, is often used…

Ab initio calculation of the hyperfine, P-odd, and P,T-odd constants for the YbF molecule was performed with the help of the recently developed technique, which allows to take into account correlations and polarization in the outercore…

Atomic Physics · Physics 2015-06-26 N. S. Mosyagin , M. G. Kozlov , A. V. Titov

We investigate the energy levels of heteronuclear alkali metal dimers in levels correlating with the lowest rotational level of the ground electronic state, which are important in efforts to produce ground-state ultracold molecules. We use…

Atomic Physics · Physics 2009-11-13 J. Aldegunde , Ben A. Rivington , Piotr S. Żuchowski , Jeremy M. Hutson

We investigate the parity ($\mathcal{P}$) and time-reversal ($\mathcal{T}$) symmetry violating effects in the CdH molecule and perform the relativistic coupled-cluster calculation of the molecular parameters- $E_\text{eff}$, $W_\text{s}$…

Chemical Physics · Physics 2020-03-11 Kaushik Talukdar , Malaya K. Nayak , Nayana Vaval , Sourav Pal

Parity and time-reversal violating electric dipole moment (EDM) of $^{171}$Yb is calculated accounting for the electron correlation effects over the Dirac-Hartree-Fock (DHF) method in the relativistic Rayleigh-Schr\"odinger many-body…

Atomic Physics · Physics 2017-07-05 B. K. Sahoo , Yashpal Singh

We carry out first-principle calculations of scalar and tensor components of the static electric dipole polarizabilities of six low-lying states of lithium (Li), sodium (Na) and potassium (K) alkali atoms in the linear response approach.…

Atomic Physics · Physics 2025-04-22 A. Chakraborty , B. K. Sahoo
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