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We explore structural correlations of strongly asymmetric mixtures of binary charged colloids within the primitive model of electrolytes considering large charge and size ratios of 10 and higher. Using computer simulations with explicit…

Soft Condensed Matter · Physics 2022-07-13 Elshad Allahyarov , Hartmut Löwen , Alan Denton

The interaction between charged objects in solution is generally expected to recapitulate two central principles of electromagnetics: (i) like-charged objects repel, and (ii) they do so regardless of the sign of their electrical charge.…

Soft Condensed Matter · Physics 2022-12-27 Sida Wang , Rowan Walker-Gibbons , Bethany Watkins , Melissa Flynn , Madhavi Krishnan

In this work, we study the synergistic correlated states in two distinct types of interacting electronic systems coupled by interlayer Coulomb interactions. We propose that this scenario can be realized in a type of Coulomb-coupled…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Xin Lu , Shihao Zhang , Yaning Wang , Xiang Gao , Kaining Yang , Zhongqing Guo , Yuchen Gao , Yu Ye , Zheng Vitto Han , Jianpeng Liu

Shapes of colloids matter at liquid interfaces. We explore the interactions between rough-surfaced nanocolloids at the air--water interface through the compaction of monolayers experimentally and numerically. Sufficiently rough systems…

Soft Condensed Matter · Physics 2023-05-17 Airi N. Kato , Yujie Jiang , Wei Chen , Ryohei Seto , Tao Li

We study thermal equilibrium of classical pointlike counterions confined between symmetrically charged walls at distance $d$. At very large couplings when the counterion system is in its crystal phase, a harmonic expansion of particle…

Soft Condensed Matter · Physics 2019-01-21 L. Samaj , M. Trulsson , E. Trizac

The charge state of dielectric surfaces in aqueous environments is of fundamental and technological importance. Here, we study the influence of dissolved molecular CO$_2$ on the charging of three, chemically different surfaces (SiO$_2$,…

Using molecular dynamics simulations we examine the effective interactions between two like-charged rods as a function of angle and separation. In particular, we determine how the competing electrostatic repulsions and…

Soft Condensed Matter · Physics 2009-11-10 Kun-Chun Lee , Itamar Borukhov , William M. Gelbart , Andrea J. Liu , Mark J. Stevens

We study the interactions between two negatively charged macroscopic surfaces confining positive counterions. A density-functional approach is introduced which, besides the usual mean-field interactions, takes into account the correlations…

Soft Condensed Matter · Physics 2015-06-25 A. Diehl , M. N. Tamashiro , Marcia C. Barbosa , Yan Levin

Properties of the "electron gas" - in which conduction electrons interact by means of Coulomb forces but ionic potentials are neglected - change dramatically depending on the balance between kinetic energy and Coulomb repulsion. The limits…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Amit Ghosal , A. D. Guclu , C. J. Umrigar , Denis Ullmo , Harold U. Baranger

The screened Coulomb interaction between uniformly charged flat plates is considered at very small plate separations for which the Debye layers are strongly overlapped, in the limit of small electrical potentials. If the plates are of…

Soft Condensed Matter · Physics 2017-02-06 Sandip Ghosal , John D. Sherwood

Long-ranged attractions across water between two surfaces that are randomly covered with (mobile) positive and negative charge domains have been attributed to induced correlation of the charges (positive lining up with negative) as the…

Soft Condensed Matter · Physics 2012-10-30 Gilad Silbert , Dan Ben-Yaakov , Yael Dror , Susan Perkin , Nir Kampf , Jacob Klein

In the present work, we study an electrolyte solution confined between planar surfaces with nonopatterned charged domains, which has been connected to a bulk ionic reservoir. The system is investigated through an improved Monte Carlo (MC)…

Soft Condensed Matter · Physics 2020-09-29 Amin Bakhshandeh , Maximiliano Segala , Thiago Colla

We have directly observed reversal of the polarity of charged surfaces in water upon the addition of tri- and quadrivalent ions using atomic force microscopy. The bulk concentration of multivalent ions at which charge inversion reversibly…

Statistical Mechanics · Physics 2009-11-10 K. Besteman , M. A. G. Zevenbergen , H. A. Heering , S. G. Lemay

In this work we study the competition or coexistence between charge density wave (CDW) and superconductivity (SC) in a two-band model system in a square lattice. One of the bands has a net attractive interaction ($J_d$) that is responsible…

Strongly Correlated Electrons · Physics 2021-06-02 Nei Lopes , Daniel Reyes , Mucio A. Continentino , Christopher Thomas

The mutual influence of two layers with strongly loclized electrons is exercised through the random Coulomb shifts of site energies in one layer caused by electron hops in the other layer. We trace how these shifts give rise to a voltage…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 M. E. Raikh , Felix von Oppen

We present a theoretical description of the effect of polyvalent ions on the interaction between titratable macro-ions. The model system consists of two point-like macro-ions with dissociable sites, immersed in an asymmetric ionic mixture…

Biological Physics · Physics 2016-06-22 Natasa Adzic , Rudolf Podgornik

Due to the strong correlations between multivalent counterions condensed on a macroion, the net macroion charge changes sign at some critical counterion concentration. This effect is known as the charge inversion. Near this critical…

Soft Condensed Matter · Physics 2009-11-07 T. T. Nguyen , B. I. Shklovskii

Attaining accurate average structural properties in a molecular simulation should be considered a prerequisite if one aims to elicit meaningful insights into a system's behavior. For charged surfaces in contact with an electrolyte solution,…

Materials Science · Physics 2021-03-25 Thomas Sayer , Stephen J. Cox

A variational theory is developed to study electrolyte solutions, composed of interacting point-like ions in a solvent, in the presence of dielectric discontinuities and charges at the boundaries. Three important and non-linear…

Soft Condensed Matter · Physics 2013-05-29 Sahin Buyukdagli , Manoel Manghi , John Palmeri

We study the influence of airborne CO2 on the charge state of carboxylate stabilized polymer latex particles suspended in aqueous electrolytes. We combine conductometric experiments interpreted in terms of Hessinger's conductivity model…

Soft Condensed Matter · Physics 2024-11-19 Peter Vogel , David Beyer , Christian Holm , Thomas Palberg