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High resolution neutron scattering measurements on a single crystal of SrCu(2-x)Mgx(BO3)2 with x=0.05 reveal the presence of new spin excitations within the gap of this quasi-two dimensional, singlet ground state system. Application of a…

Strongly Correlated Electrons · Physics 2009-11-11 S. Haravifard , S. R. Dunsiger , S. El Shawish , B. D. Gaulin , H. A. Dabkowska , M. T. F. Telling , J. Bonca

Macroscopic assemblies of interacting spins give rise to a broad spectrum of behaviors determined by the spatial arrangement of the magnetic sites and the electronic interactions between them. Compounds of copper (II), in which each copper…

Strongly Correlated Electrons · Physics 2021-04-22 Pavel Pokhilko , Dmitry S. Bezrukov , Anna I. Krylov

Using Random Phase Approximation, we show that a crossed-chains model of a spin-1/2 Heisenberg spins, with frustrated interchain couplings, has a non-dimerized spin-liquid ground state in 2D, with deconfined spinons as the elementary…

Strongly Correlated Electrons · Physics 2009-11-07 Oleg A. Starykh , Rajiv R. P. Singh , Gregory C. Levine

We present an effective dipolar-spin model based on the strong coupling analysis, which may explain the possible origin of the "spin liquid Mott insulator". The issue is related to the dimer Mott insulator reminiscent of the organic…

Strongly Correlated Electrons · Physics 2010-08-27 Chisa Hotta

Azurite, a natural mineral made up of CuO chains, is also an intriguing spin-1/2 quantum magnet. There has been much debate as to the 1-dimensional (1D) nature of this material by theorists and experimentalists alike. The focus of this…

Strongly Correlated Electrons · Physics 2012-07-23 K. C. Rule , D. A. Tennant , J. -S. Caux , M. C. R. Gibson , M. T. F. Telling , S. Gerischer , S. Süllow , M. Lang

Strongly correlated Fermi systems are among the most intriguing and fundamental systems in physics. We show that the herbertsmithite ZnCu3(OH)6Cl2 can be viewed as a new type of strongly correlated electrical insulator that possesses…

Strongly Correlated Electrons · Physics 2013-06-24 V. R. Shaginyan , K. G. Popov , V. A. Khodel

We present a microscopic model of the spin-gap quantum magnet (CuCl)LaNb2O7 that was previously suggested as a realization of the spin-1/2 frustrated square lattice. Taking advantage of the precise atomic positions from recent crystal…

Strongly Correlated Electrons · Physics 2010-08-30 Alexander A. Tsirlin , Helge Rosner

In quantum magnetism spin dimers are typically associated with spin-singlet states. To date, $triplet$ $dimerization$ has not been observed in any 3D or quasi-2D material. With this in mind we here discuss the electronic structure of the…

Inelastic neutron scattering measurements on the itinerant antiferromagnet (AFM) CaCo$_{\mathrm{2}-y}$As$_{2}$ at a temperature of 8 K reveal two orthogonal planes of scattering perpendicular to the Co square lattice in reciprocal space,…

We have studied the excitation spectrum of the $S=1/2$ quantum spin ladder with staggered dimerization by dimer series expansions, diagrammatic analysis of an effective interacting Bose gas of local triplets, and exact diagonalization of…

Strongly Correlated Electrons · Physics 2009-10-31 V. N. Kotov , J. Oitmaa , Zheng Weihong

Spin excitations are explored in the electron-doped spin-orbit Mott insulator (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$. As this bilayer square lattice system is doped into the metallic regime, long-range antiferromagnetism vanishes, yet a…

Strongly Correlated Electrons · Physics 2016-09-14 Tom Hogan , Rebecca Dally , Mary Upton , J. P. Clancy , Kenneth Finkelstein , Young-June Kim , M. J. Graf , Stephen D. Wilson

By measuring the THz electron spin resonance (ESR) transmission spectra and high-field magnetization on the spin-gapped system CuTe$_2$O$_5$, we identified the singlet-triplet excitations in the dimerized non-magnetic ground state. The…

Strongly Correlated Electrons · Physics 2011-11-22 Zhe Wang , M. Schmidt , Y. Goncharov , Y. Skourski , J. Wosnitza , H. Berger , H. -A. Krug von Nidda , A. Loidl , J. Deisenhofer

The ground-state spin arrangement and the bipartite entanglement within Cu$^{2+}$-Cu$^{2+}$ dimers across the magnetization process of the 4f-3d heterometallic coordination polymer [{Dy(hfac)$_2$(CH$_3$OH)}$_2${Cu(dmg)(Hdmg)}$_2$]$_n$…

Statistical Mechanics · Physics 2022-07-28 Lucia Gálisová

To reveal the structure-property relationship in quasi-one-dimensional (1D) spin-chain system Ca$_3$ZnMnO$_6$, we present comprehensive results, combining basic physical characterizations such as muon spin relaxation/rotation ($\mu$SR),…

The site- and bond-dilution effects of the nonmagnetic ground state of a two-dimensional $S=1/2$ antiferromagnetic Heisenberg model, coupled with the lattice distortions on a square lattice, are investigated by performing quantum Monte…

Strongly Correlated Electrons · Physics 2019-01-25 Chitoshi Yasuda , Shouta Miyara

The magnetic excitation spectrum of copper pyrimidine dinitrate, a material containing S=1/2 antiferromagnetic chains with alternating g-tensor and the Dzyaloshinskii-Moriya interaction, and exhibiting a field-induced spin gap, is probed…

Strongly Correlated Electrons · Physics 2009-11-10 S. A. Zvyagin , A. K. Kolezhuk , J. Krzystek , R. Feyerherm

Below about 150 K, the spin arrangement in the chain arrays of Sr14Cu24O41 is shown to develop in two dimensions (2D). Both the correlations and the dispersion of the observed elementary excitations agree well with a model of interacting…

Strongly Correlated Electrons · Physics 2009-10-31 L. P. Regnault , J. P. Boucher , H. Moudden , J. E. Lorenzo , A. Hiess , U. Ammerahl , G. Dhalenne , A. Revcolevschi

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Strongly Correlated Electrons · Physics 2024-07-18 Tao Xie , Jie Xing , S. E. Nikitin , S. Nishimoto , M. Brando , P. Khanenko , J. Sichelschmidt , L. D. Sanjeewa , Athena S. Sefat , A. Podlesnyak

We present a specific heat and inelastic neutron scattering study in magnetic fields up into the 1/3 magnetization plateau phase of the diamond chain compound azurite Cu$_3$(CO$_3$)$_2$(OH)$_2$. We establish that the magnetization plateau…

Statistical Mechanics · Physics 2009-11-13 K. C. Rule , A. U. B. Wolter , S. Süllow , D. A. Tennant , A. Brühl , S. Köhler , B. Wolf , M. Lang , J. Schreuer

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee