Related papers: Transmission-line decelerators for atoms in high R…
Beams of helium atoms in Rydberg-Stark states with principal quantum number $n=48$ and electric dipole moments of 4600~D have been decelerated from a mean initial longitudinal speed of 2000~m/s to zero velocity in the laboratory-fixed…
The large electric dipole moments associated with highly excited Rydberg states of atoms and molecules make gas-phase samples in these states very well suited to deceleration and trapping using inhomogeneous electric fields. The methods of…
Inhomogeneous electric fields generated above two-dimensional electrode structures have been used to transversely split beams of helium Rydberg atoms into pairs of spatially separated components. The atomic beams had initial longitudinal…
Metastable (1s)(2s) $^3{\rm S}_1$ helium atoms produced in a supersonic beam were excited to Rydberg-Stark states (with $n$ in the $27-30$ range) in a cryogenic environment and subsequently decelerated by, and trapped above, a…
Tunnel ionization rates of triplet Rydberg states in helium with principal quantum numbers close to 37 have been measured in electric fields at the classical ionization threshold of $\sim197$ V/cm. The measurements were performed in the…
Helium atoms in high- and low-field-seeking Rydberg states with linear and quadratic Stark shifts have been confined in two dimensions and guided over a distance of 150 mm using time-varying inhomogeneous electric fields. This was achieved…
Supersonic beams of hydrogen atoms, prepared selectively in Rydberg-Stark states of principal quantum number $n$ in the range between 25 and 35, have been deflected by 90$^\circ$, decelerated and loaded into off-axis electric traps at…
We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of…
Nitric oxide (NO) molecules initially traveling at 795 m/s in pulsed supersonic beams have been photoexcited to long-lived hydrogenic Rydberg-Stark states, decelerated and electrostatically trapped in a cryogenically cooled, chip-based…
Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number $n=53$ and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been…
Helium atoms have been prepared in the circular $|n=55,\ell=54,m_{\ell}=+54\rangle$ Rydberg state using the crossed electric and magnetic fields method. The atoms, initially travelling in pulsed supersonic beams, were photoexcited from the…
Helium atoms in Rydberg states have been manipulated coherently with microwave radiation pulses near a gold surface and near a superconducting NbTiN surface at a temperature of $3 \text{K}$. The experiments were carried out with a skimmed…
N$_2$ molecules traveling in pulsed supersonic beams have been excited from their ${\mathrm{X\,^1\Sigma_{\mathrm{g}}^+}}$ ground electronic state to long-lived Rydberg states with principal quantum numbers between 39 and 48 using a…
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit…
We present experimental results that demonstrate - for the first time - the Zeeman deceleration of helium atoms in the metastable 2^3S_1state. A more than 40% decrease of the kinetic energy of the beam is achieved for deceleration from 490…
The resonant transfer of energy from the inversion sublevels in NH$_3$ to He atoms in triplet Rydberg states with principal quantum number $n=38$ has been controlled using electric fields below 15 V/cm in intrabeam collisions at…
Tommey and Hogan [Phys. Rev. A, 104, 033305 (2021)] have reported a matter-wave interference experiment using Rydberg atoms traveling through inhomogeneous electric fields at approximately 2000 m/s. Using a simplified model containing the…
Rydberg atoms have shown significant promise as the basis for highly sensitive detectors of continuous radio-frequency (RF) E-fields. Here, we study their time-dependent response to pulse-modulated RF E-fields at 19.4 GHz using a cesium…
Rydberg alkaline earth atoms are promising tools for quantum simulation and metrology. When one of the two valence electrons is promoted to long-lived circular states, the second valence electron can be optically manipulated without…
We study two ions confined in a Penning trap. We show that electronically highly excited states exist in which an electron is delocalized among the two ions forming a giant molecule of several micrometer size. At energies close to the top…