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Related papers: Excited states from range-separated density-functi…

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A strictly truncated (weak-coupling) perturbation theory is applied to the attractive Holstein and Hubbard models in infinite dimensions. These results are qualified by comparison with essentially exact Monte Carlo results. The second order…

Condensed Matter · Physics 2009-10-22 J. K. Freericks , Mark Jarrell

Fractional occupation numbers can produce open-shell degeneracy in density functional theory. We develop the corresponding perturbation theory by requiring that a differentiable map connects the initial and perturbed states. The degenerate…

Materials Science · Physics 2016-07-22 Mark C. Palenik , Brett I. Dunlap

By combining extrapolated selected configuration interaction (sCI) energies obtained with the CIPSI (Configuration Interaction using a Perturbative Selection made Iteratively) algorithm with the recently proposed short-range…

Chemical Physics · Physics 2020-06-05 Emmanuel Giner , Anthony Scemama , Julien Toulouse , Pierre-François Loos

Model Hamiltonians with long-range interaction yield energies that are corrected taking into account the universal behavior of the electron-electron interaction at short range. Although the intention of the paper is to explore the…

Chemical Physics · Physics 2020-10-28 Andreas Savin

We investigate the use of perturbation theory in finite sized frustrated spin systems by calculating the effect of quantum fluctuations on coherent states derived from the classical ground state. We first calculate the ground and first…

Strongly Correlated Electrons · Physics 2009-10-31 N. P. Konstantinidis , D. Coffey

In this study, we extend the multicomponent heat-bath configuration interaction (HCI) method to excited states. Previous multicomponent HCI studies have been performed using only the variational stage of the HCI algorithm as they have…

Chemical Physics · Physics 2022-01-12 Naresh Alaal , Kurt R. Brorsen

The \textit{ab initio} approach is used to evaluate the excitation energies of the $2s2p \, ^{2S+1}P_J$ states from the ground state as well as the $2s2p \, ^3P_1 \rightarrow 2s2p \, ^3P_0$ and $2s2p \, ^3P_2 \rightarrow 2s2p \, ^3P_1$…

Atomic Physics · Physics 2024-11-05 A. V. Malyshev , Y. S. Kozhedub , V. M. Shabaev , I. I. Tupitsyn

Determining quantum excited states is crucial across physics and chemistry but presents significant challenges for variational methods, primarily due to the need to enforce orthogonality to lower-energy states, often requiring…

Quantum Physics · Physics 2025-05-01 Shi-Xin Zhang , Lei Wang

We consider first order perturbation theory for a non-minimally coupled inflaton field without assuming an adiabatic equation of state. In general perturbations in non-minimally coupled theory may be non-adiabatic. However under the…

High Energy Physics - Phenomenology · Physics 2013-01-10 Abhishek Basak , Jitesh R. Bhatt

To describe excited states, the electron density alone being insufficient, we use the noninteracting reference density matrix $\gamma_{s}({\bf x},{\bf x}')$ based on the recently established foundation for the $\Delta SCF$ theory, in which…

Chemical Physics · Physics 2024-08-20 Weitao Yang , Yichen Fan

We study second-order electromagnetic perturbations in the Schwarzschild background and derive the effective source terms for Regge-Wheeler equation which are quadratic in first-order gravitational and electromagnetic perturbations. In…

General Relativity and Quantum Cosmology · Physics 2025-11-19 Fawzi Aly , Mahmoud A. Mansour , Dejan Stojkovic

An exact diagonalization technique is used to investigate the low-lying excited polaron states in the Holstein model for the infinite one-dimensional lattice. For moderate values of the adiabatic ratio, a new and comprehensive picture,…

Condensed Matter · Physics 2009-11-07 Osor S. Barisic

We develop an analytical expression for the self-energy of the infinite-dimensional Hubbard model that is correct in a number of different limits. The approach represents a generalization of the iterative perturbation theory to arbitrary…

Strongly Correlated Electrons · Physics 2009-10-30 M. Potthoff , T. Wegner , W. Nolting

The calculation of excited state energies of electronic structure Hamiltonians has many important applications, such as the calculation of optical spectra and reaction rates. While low-depth quantum algorithms, such as the variational…

Quantum Physics · Physics 2019-07-03 Oscar Higgott , Daochen Wang , Stephen Brierley

We present a method for finding individual excited states' energy stationary points in complete active space self-consistent field theory that is compatible with standard optimization methods and highly effective at overcoming difficulties…

Strongly Correlated Electrons · Physics 2019-04-12 Lan Nguyen Tran , Jacqueline A. R. Shea , Eric Neuscamman

We calculate accurate potential energy curves for a ground-state He$^+$ ion interacting with a He atom in the lowest-energy metastable $^3\!S$ electronic state. We employ the full configuration interaction method, equivalent to exact…

Atomic Physics · Physics 2023-11-30 Jacek Gȩbala , Michał Przybytek , Marcin Gronowski , Michał Tomza

We calculate the one-photon exchange contribution to the interatomic interaction potential between electrically neutral, identical atoms, one of which is assumed to be in an excited state, by matching the scattering matrix (S matrix)…

Atomic Physics · Physics 2025-09-12 U. D. Jentschura , C. M. Adhikari

We present a new perturbation theory for quantum mechanical energy eigenstates when the potential equals the sum of two localized, but not necessarily weak potentials $V_{1}(\vec{r})$ and $V_{2}(\vec{r})$, with the distance $L$ between the…

Quantum Physics · Physics 2007-05-23 Seok Kim , Choonkyu Lee

We derive the second-order approximation (PT2) to the ensemble correlation energy functional by applying the G\"{o}rling-Levy perturbation theory on the ensemble density-functional theory (EDFT). Its performance is checked by calculating…

Computational Physics · Physics 2021-11-17 Zeng-hui Yang

Relativistic calculations for the $g$ factor of the lowest excited states $2p_{1/2}$ and $2p_{3/2}$ of lithium-like ions over a wide range of the nuclear charge numbers $Z=10-92$ are presented. Interelectronic interaction is considered…