Related papers: High-order harmonic spectroscopy for molecular ima…
Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…
High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…
We present the experimental and theoretical details of our recent published letter [Phys. Rev. Lett. 115. 123002] on synchronized high-harmonic and terahertz-wave spectroscopy (HATS) from nonadiabatically aligned nitrogen molecules in…
Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…
We study high-order harmonic generation by optically driven one- and two-dimensional hydrogenlike atoms formed by Coulomb imurities in graphene. The time-dependent Dirac equations with Coulomb plus time-periodic monochromatic field…
Structured light carrying orbital angular momentum enables new regimes of nonlinear light-matter interaction. Here we develop a molecular quantum electrodynamics description of third-harmonic generation (THG) driven by focused…
Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…
Sub-femtosecond x-ray burst is powerful tool for probing and imaging electronic and concomitant atomic motion in attosecond physics. For years, x-ray source (above 2 keV) had mainly been obtained from X-ray free electron laser (XFEL) or…
Geometric moments and moment invariants of image artifacts have many uses in computer vision applications, e.g. shape classification or object position and orientation. Higher order moments are of interest to provide additional feature…
We investigate the use of light beams carrying orbital angular momentum (OAM) in the context of high harmonic generation (HHG) within semiconductor crystals. Our contribution deals with the transfer and conservation of OAM in the…
We present a theoretical study of high-order harmonic generation (HHG) and propagation driven by an infrared field carrying orbital angular momentum (OAM). Our calculations unveil the following relevant phenomena: extreme-ultraviolet…
We theoretically demonstrate a scheme for tomographic reconstruction of asymmetric molecular orbitals based on high-order harmonic generation with a two-color multicycle laser field. It is shown that by adjusting the relative phase of the…
We propose a real-time time-dependent ab__initio approach within a configuration-interaction-singles ansatz to decompose the high-harmonic generation (HHG) signal of molecules in terms of individual molecular-orbital (MO) contributions.…
We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…
Measuring the three-dimensional (3D) distribution of chemistry in nanoscale matter is a longstanding challenge for metrological science. The inelastic scattering events required for 3D chemical imaging are too rare, requiring high beam…
Graph generation techniques are increasingly being adopted for drug discovery. Previous graph generation approaches have utilized relatively small molecular building blocks such as atoms or simple cycles, limiting their effectiveness to…
Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…
Atomic-resolution imaging with scanning transmission electron microscopy is a powerful tool for characterizing the nanoscale structure of materials, in particular features such as defects, local strains, and symmetry-breaking distortions.…
We investigate the spatial characteristics of high-order harmonic radiation generated in argon, and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these…
Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…