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Multiple exciton generation solar cells exhibit a low power conversion efficiency owing to nonradiative recombination even if numerous electron and hole pairs are generated per incident photon. This paper elucidates the non-idealities of…

Applied Physics · Physics 2021-04-14 Jongwon Lee

Colloidal semiconductor nanoplatelets, in which carriers are strongly confined only along one dimension, present fundamentally different excitonic properties than quantum dots, which support strong confinement in all three dimensions. In…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Daniel Amgar , Gaoling Yang , Ron Tenne , Dan Oron

Semiconductor quantum dots host a rich manifold of excitonic complexes, including neutral excitons that emit anti-bunched single photons and charged exciton complexes capable of producing super-bunched photons via cascade emission.…

Energy-time entangled photons provide new opportunities for controlling multiphoton absorption beyond classical limits. Here, we investigate biexciton generation in nanocrystal quantum dots driven by energy-time-entangled quantum light…

Chemical Physics · Physics 2026-05-27 Kaiyue Peng , Chieh Tsao , Hendrik Utzat , Eran Rabani

We consider theoretically the formation and stability of quasi-one dimensional many-body excitons in GaAs quantum wire structures under external photoexcitation conditions by solving the dynamically screened Bethe-Salpeter equation for…

Strongly Correlated Electrons · Physics 2009-10-31 S. Das Sarma , D. W. Wang

Unique properties of lead chalcogenides have enabled multiple exciton generation (MEG) in their nanocrystals that can be beneficial in enhancing the efficiency of the third generation solar cells. Although the intrinsic electric field plays…

Atomic and Molecular Clusters · Physics 2017-09-07 Mahdi Gordi , Mohammad Kazem Moravvej-Farshi , Hamidreza Ramezani

The two-dimensional semiconductor MoS2 in its mono- and few-layer form is expected to have a significant exciton binding energy of several 100 meV, leading to the consensus that excitons are the primary photoexcited species. Nevertheless,…

Electroluminescence (EL) of colloidal nanocrystals promises a new generation of high-performance and solution-processable light-emitting diodes (LEDs). The operation of nanocrystal-based LEDs relies on the recombination of…

The quasiparticle band structure and optical properties of single-walled zigzag and armchair SiC nanotubes (SiC-NTs) as well as single SiC sheet are investigated by ab initio many-body calculations using the GW and the GW plus…

Mesoscale and Nanoscale Physics · Physics 2011-08-23 H. C. Hsueh , G. Y. Guo , Steven G. Louie

Electron-phonon and exciton-phonon interactions in nanoclusters are formulated and computed under the framework of GW-BSE (Bethe-Salpeter equation) approach. The phonon effect is modeled with the two-particle representation for the first…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Taofang Zeng , Yi He

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

We report absorption and photoluminescence spectra of Si and SnO$_2$ polycrystalline nanofilms in the UV-Vis-NIR range, featuring discrete bands resulting from transverse quantum confinement. The film thickness ranged 3.9 nm to 12.2 nm,…

Mesoscale and Nanoscale Physics · Physics 2014-05-21 Vladimir I. Makarov , Igor Khmelinskii

Singlet fission (SF), an exciton multiplication process occurring in organic semiconductors, offers a way to break the Shockley-Queisser limit in single-bandgap photovoltaics (PV). If the triplet excitons generated by SF can be transferred…

Transition metal dichalcogenides (TMDCs) have demonstrated significant potential as versatile quantum materials for light absorption and emission. Their unique properties are primarily governed by exciton-photon interactions, which can be…

We study carrier interaction induced many-body effects on the excitonic optical properties of highly photoexcited one-dimensional semiconductor quantum wire systems by solving the dynamically screened Bethe-Salpeter equation using realistic…

Strongly Correlated Electrons · Physics 2009-11-07 D. W. Wang , S. Das Sarma

The electrons and excitons multiple exciton generation dynamics in two silicon clusters, or more specifically the inelastic scattering rates of electronic and excitonic states in the two silicon clusters, Si26 and Si46, are calculated using…

Mesoscale and Nanoscale Physics · Physics 2020-07-14 Taofang Zeng , Yi He

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

Exciton many-body interaction bear great implication for application in advanced photonic devices and quantum science and technology such as quantum computing, but the fundamental understanding about exciton many-body interaction is very…

Materials Science · Physics 2020-09-17 Yiling Yu , Guoqing Li , Linyou Cao

Excitons -- quasiparticles formed by the binding of an electron and a hole through electrostatic attraction -- hold promise in the fields of quantum light confinement and optoelectronic sensing. Atomically thin transition metal…

Optical properties of single-wall carbon nanotubes (SWCNTs) for light polarized parallel to the nanotube axis have been extensively studied, whereas their response to light polarized perpendicular to the nanotube axis has not been well…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fumiya Katsutani , Weilu Gao , Xinwei Li , Yota Ichinose , Yohei Yomogida , Kazuhiro Yanagi , Junichiro Kono