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As narrow optical bandgap materials, semiconducting single-walled carbon nanotubes (SWCNTs) are rarely regarded as charge donors in photoinduced charge-transfer (PCT) reactions. However, the unique band structure and unusual exciton…

The controlled introduction of covalent sp$^{3}$ defects into semiconducting single-walled carbon nanotubes (SWCNTs) gives rise to exciton localization and red-shifted near-infrared luminescence. The single-photon emission characteristics…

Materials Science · Physics 2022-06-22 Wenhao Zheng , Nicolas F. Zorn , Mischa Bonn , Jana Zaumseil , Hai I. Wang

Photophysics of single-wall carbon nanotubes (SWCNTs) is intensively studied due to their potential application in light harvesting and optoelectronics. Excited states of SWCNTs form strongly bound electron-hole pairs, excitons, of which…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 J. Palotas , M. Negyedi , S. Kollarics , A. Bojtor , P. Rohringer , Th. Pichler , F. Simon

We have studied the electronic structure and charge-carrier dynamics of individual single-wall carbon nanotubes (SWNTs) and nanotube ropes using optical and electron-spectroscopic techniques. The electronic structure of semiconducting SWNTs…

Materials Science · Physics 2009-11-10 A. Hagen , G. Moos , V. Talalaev , J. W. Tomm , T. Hertel

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

Excitons play major roles in optical processes in modern semiconductors, such as single-wall carbon nanotubes (SWCNTs), transition metal dichalcogenides, and 2D perovskite quantum wells. They possess extremely large binding energies…

Single walled carbon nanotubes (SWNT) have displayed a wealth of quantum transport phenomena thus far. Defect free, unperturbed SWNTs with wellbehaved or tunable metal contacts are important to probing the intrinsic electrical properties of…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Jien Cao , Qian Wang , Hongjie Dai

The nature of the primary photoexcitations in semiconducting single-walled carbon nanotubes (S-SWCNTs) is of strong current interest. We have studied the emission spectra of S-SWCNTs and two different $\pi$-conjugated polymers in solutions…

Materials Science · Physics 2007-05-23 H. Zhao , S. Mazumdar , C. -X. Sheng , Z. V. Vardeny

One-dimensional nanoscale devices, such as semiconductor nanowires (NWs) and single- walled carbon nanotubes (SWNTs), have been intensively investigated because of their potential application of future high-speed electronic, optoelectronic,…

Instrumentation and Detectors · Physics 2014-10-27 B. H. Son , Jae-Ku Park , J. T. Hong , Ji-Yong. Park , Soonil. Lee , Y. H. Ahn

Through ultrafast pump-probe spectroscopy with intense pump pulses and a wide continuum probe, we show that interband exciton peaks in single-walled carbon nanotubes (SWNTs) are extremely stable under high laser excitations. Estimates of…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 G. N. Ostojic , S. Zaric , J. Kono , V. C. Moore , R. H. Hauge , R. E. Smalley

A detailed understanding of energy transduction is crucial for achieving precise control of energy flow in complex, integrated systems. In this context, carbon nanotubes (CNTs) are intriguing model systems due to their rich,…

Mesoscale and Nanoscale Physics · Physics 2011-02-16 Eyal Shafran , Benjamin D. Mangum , Jordan M. Gerton

The recent development of efficient chirality sorting techniques has opened the way to the use of single-walled carbon nanotubes (SWCNTs) in a plethora of nanoelectronic, photovoltaic, and optoelectronic applications. However, to understand…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 María Rosa Preciado-Rivas , Victor Alexander Torres-Sánchez , Duncan J. Mowbray

Solution-processed networks of semiconducting, single-walled carbon nanotubes (SWCNTs) have attracted considerable attention as materials for next-generation electronic devices and circuits. However, the impact of the SWCNT network…

We report a femtosecond mid-infrared study of the broadband low-energy response of individually separated (6,5) and (7,5) single-walled carbon nanotubes. Strong photoinduced absorption is observed around 200 meV, whose transition energy,…

Mesoscale and Nanoscale Physics · Physics 2010-07-16 Jigang Wang , Matt W. Graham , Yingzhong Ma , Graham R. Fleming , Robert A. Kaindl

We study quantum optical properties of the single-walled carbon nanotube (SWCNT) by introducing the effective interaction between the quantized electromagnetic field and the confined electrons in the SWCNT. Our purpose is to explore the…

Mesoscale and Nanoscale Physics · Physics 2009-04-30 Z. L. Guo , Z. R. Gong , C. P. Sun

A method is introduced to isolate and measure the electrical transport properties of individual single-walled carbon nanotubes (SWNTs) aligned on an ST-cut quartz, from room temperature down to 2 K. The diameter and chirality of the…

Mesoscale and Nanoscale Physics · Physics 2014-08-26 Tohru Watanabe , El-Hadi S. Sadki , Takahide Yamaguchi , Yoshihiko Takano

Light emission from nanostructures exhibits rich quantum effects and has broad applications. Single-walled carbon nanotubes (SWNTs) are one-dimensional (1D) metals or semiconductors, in which large number of electronic states in a narrow…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 David Mann , Y. K. Kato , Anika Kinkhabwala , Eric Pop , Jien Cao , Xinran Wang , Li Zhang , Qian Wang , Jing Guo , Hongjie Dai

The properties of excitons in semiconducting single-walled carbon nanotubes (SWCNTs), isolated in vacuum or a medium, and their contributions to the optical spectra of nanotubes are studied within the elementary potential model, in which an…

Materials Science · Physics 2010-12-15 Oleksii A. Smyrnov

A theoretical model for the calculation of the phonon-drag thermopower, $S^{g}$, in degenerately doped semiconducting single-wall carbon nanotubes (SWCNTs) is proposed. Detailed calculations of $S^{g}$ are performed as a function of…

Mesoscale and Nanoscale Physics · Physics 2011-03-03 Margarita Tsaousidou

At cryogenic temperature and at the single emitter level, the optical properties of single-wall carbon nanotubes depart drastically from that of a one-dimensional (1D) object. In fact, the (usually unintentional) localization of excitons in…

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