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We demonstrate a spin-precession method to observe and analyze multi-level coherence between all hyperfine levels in the $X ^2\Sigma^+,N=0$ ground state of barium monofluoride ($^{138}$Ba$^{19}$F). The signal is sensitive to the…

We report the coherent manipulation of electron spins in a double quantum dot integrated with a micro-magnet. We performed electric dipole spin resonance experiments in the continuous wave (CW) and pump-and-probe modes. We observed two…

Different approaches have improved the sensitivity of either electron or nuclear magnetic resonance to the single spin level. For optical detection it has essentially become routine to observe a single electron spin or nuclear spin.…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Jörg Wrachtrup , Amit Finkler

Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial,…

The effect of dipolar and exchange interactions within pairs of paramagnetic electronic states on Pauli-blockade-controlled spin-dependent transport and recombination rates during magnetic resonant spin excitation is studied numerically…

Materials Science · Physics 2013-04-24 M. E. Limes , J. Wang , W. J. Baker , S. -Y. Lee , B. Saam , C. Boehme

We describe the first precision measurement of the electron's electric dipole moment (eEDM, $d_e$) using trapped molecular ions, demonstrating the application of spin interrogation times over 700 ms to achieve high sensitivity and stringent…

We report on a novel dynamical phenomenon in electron spin resonance experiments of phosphorus donors. When strongly coupling the paramagnetic ensemble to a superconducting lumped element resonator, the coherent exchange between these two…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 Stefan Weichselbaumer , Matthias Zens , Christoph W. Zollitsch , Martin S. Brandt , Stefan Rotter , Rudolf Gross , Hans Huebl

We study a scheme for electrical detection of the spin resonance (ESR) of a single electron trapped near a Field Effect Transistor (FET) conduction channel. In this scheme, the resonant Rabi oscillations of the trapped electron spin cause a…

Materials Science · Physics 2007-05-23 I. Martin , D. Mozyrsky , H. W. Jiang

We discuss procedures for error-tolerant spin control in environments that permit transient, large-angle reorientation of magnetic bias field. Short sequences of pulsed, non-resonant magnetic field pulses in a laboratory-frame meridional…

Chemical Physics · Physics 2022-11-17 Sven Bodenstedt , Morgan W. Mitchell , Michael C. D. Tayler

Paramagnetic centers in a solid-state environment usually give rise to inhomogenously broadened electron paramagnetic resonance (EPR) lines, making conventionally detected free induction decay (FID) signals disappear within the spectrometer…

Quantum dots patterned by atomically precise placement of phosphorus donors in single crystal silicon have long spin lifetimes, advantages in addressability, large exchange tunability, and are readily available few-electron systems. To be…

Mesoscale and Nanoscale Physics · Physics 2016-07-06 Yu Wang , Chin-Yi Chen , Gerhard Klimeck , Michelle Y. Simmons , Rajib Rahman

Spin resonance of single spin centers bears great potential for chemical structure analysis, quantum sensing and quantum coherent manipulation. Essential for these experiments is the presence of a two-level spin system whose energy…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Philip Willke , Aparajita Singha , Xue Zhang , Taner Esat , Christopher P. Lutz , Andreas J. Heinrich , Taeyoung Choi

In recent years, a variety of solid-state qubits has been realized, including quantum dots, superconducting tunnel junctions and point defects. Due to its potential compatibility with existing microelectronics, the proposal by Kane based on…

Quantum Physics · Physics 2007-05-23 A. R. Stegner , C. Boehme , H. Huebl , M. Stutzmann , K. Lips , M. S. Brandt

Electric dipole spin resonance (EDSR) is a commonly used tool for manipulation and spectroscopy of quantum-dot-based spin qubits. When an EDSR experiment is embedded in a transport setup and Pauli spin blockade is used as means for…

Mesoscale and Nanoscale Physics · Physics 2021-08-23 Arnau Sala , Jeroen Danon

The electrical detection of spin echoes via echo tomography is used to observe decoherence processes associated with the electrical readout of the spin state of phosphorus donor electrons in silicon near a SiO$_2$ interface. Using the…

Quantum Physics · Physics 2008-05-06 Hans Huebl , Felix Hoehne , Benno Grolik , Andre R. Stegner , Martin Stutzmann , Martin S. Brandt

Motivated by the recent progress of phonon-mediated control in quantum spin devices, we propose a possibility of hybrid measurement using electron paramagnetic resonance (EPR) and a surface acoustic wave (SAW). Considering quadrupole-strain…

Strongly Correlated Electrons · Physics 2020-11-04 Mikito Koga , Masashige Matsumoto

Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with…

Strongly Correlated Electrons · Physics 2009-08-04 L. M. Holanda , J. M. Vargas , C. Rettori , S. Nakatsuji , K. Kuga , Z. Fisk , S. B. Oseroff , P. G. Pagliuso

The rapidly rising fields of spintronics and quantum information science have led to a strong interest in developing the ability to coherently manipulate electron spins. Electron spin resonance (ESR) is a powerful technique to manipulate…

Materials Science · Physics 2009-11-13 M. Pioro-Ladriere , T. Obata , Y. Tokura , Y. -S. Shin , T. Kubo , K. Yoshida , T. Taniyama , S. Tarucha

The phenomenon of spin resonance has had far reaching influence since its discovery nearly 70 years ago. Electron spin resonance (ESR) driven by high frequency magnetic fields has informed our understanding of quantum mechanics, and finds…

Mesoscale and Nanoscale Physics · Physics 2009-10-27 S. M. Frolov , S. Luscher , W. Yu , Y. Ren , J. A. Folk , W. Wegscheider

Spin-dependent relaxation and recombination processes in $\gamma$-irradiated $n$-type Czochralski-grown silicon are studied using continuous wave (cw) and pulsed electrically detected magnetic resonance (EDMR). Two processes involving the…

Materials Science · Physics 2014-07-22 David P. Franke , Felix Hoehne , Leonid S. Vlasenko , Kohei M. Itoh , Martin S. Brandt