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Synchrotron-based x-ray reflectivity is increasingly employed as an \textit{in situ} probe of surface morphology during thin film growth, but complete interpretation of the results requires modeling the growth process. Many models have been…

Materials Science · Physics 2013-05-29 Arthur R. Woll , Tushar V. Desai , James R. Engstrom

Thin films are usually obtained by depositing atoms with a continuous flux. We show that using a chopped flux changes the growth and the morphology of the film. A simple scaling analysis predicts how the island densities change as a…

Materials Science · Physics 2016-08-16 Pablo Jensen , Bernd Niemeyer

In the electrochemical deposition of thin films the measurement of the current-time curve does not allow for a direct determination of the nucleus growth law, electrode surface coverage and mean film thickness. In this work we present a…

Soft Condensed Matter · Physics 2018-03-07 S. Politi , M. Tomellini

Atomic-scale smooth thin films are keys to successful integration and proper function of many multilayer-structured devices. However, the intrinsic island-like growth mode prevents human being from realizing such ultrasmooth films of many…

Applied Physics · Physics 2021-10-04 Rongjing Guo , Tai-Chang Chiang , Huan-hua Wang

A model of submonolayer thin film growth is studied, where the attachment of atoms to island edges is hindered by an energy barrier. A novel behavior of the density of islands, N_s, is predicted as a function of flux F and temperature T.…

Materials Science · Physics 2009-10-31 Daniel Kandel

Thin films formed from small molecules rapidly gain importance in different technological fields. To explain their growth, methods developed for zero--dimensional atoms as the film forming particles are applied. However, in organic thin…

Materials Science · Physics 2013-03-14 Gregor Hlawacek , Christian Teichert

Using in situ grazing-incidence x-ray scattering, we have measured the diffuse scattering from islands that form during layer-by-layer growth of GaN by metal-organic vapor phase epitaxy on the (1010) m-plane surface. The diffuse scattering…

Effect of an anisotropic detachment on a heteroepitaxial island shape is studied by means of a kinetic Monte Carlo simulation of a square lattice gas model. Only with molecular deposition followed by surface diffusion, islands grow in a…

Materials Science · Physics 2007-07-20 Yukio Saito , Ryo Kawasaki

The stability of interfaces and the mechanisms of thin film growth on semiconductors are issues of central importance in electronic devices. These issues can only be understood through detailed study of the relevant microscopic processes.…

mtrl-th · Physics 2016-09-07 Efthimios Kaxiras

Blended organic thin films have been studied during the last decades due to their applicability in organic solar cells. Although their optical and electronic features have been examined intensively, there is still lack of detailed knowledge…

Square lattice gas models for heteroepitaxial growth are studied by means of kinetic Monte Carlo simulations, in order to find a possible origin of anisotropic island shape observed in growth experiments of long organic molecules. When…

Materials Science · Physics 2009-11-13 Yukio Saito , Ryo Kawasaki

The shape evolution of two-dimensional islands through periphery diffusion biased by an electromigration force is studied numerically using a continuum approach. We show that the introduction of crystal anisotropy in the mobility of edge…

Materials Science · Physics 2009-11-10 Philipp Kuhn , Joachim Krug , Frank Hausser , Axel Voigt

Organic semiconductors tend to self-assemble into highly ordered and oriented morphologies with anisotropic optical properties. Studying these optical anisotropies provides insight into processing-dependent structural properties and informs…

Materials Science · Physics 2016-11-03 Steven J. Brown , Ruth A. Schlitz , Michael L. Chabinyc , Jon A. Schuller

We investigate the formation and the coarsening dynamics of islands in a strained epitaxial semi-conductor film. These islands are commonly observed in thin films undergoing a morphological instability due to the presence of the elasto…

Materials Science · Physics 2016-11-02 Guido Schifani , Thomas Frisch , Mederic Argentina , Jean-Noël Aqua

We have performed Kinetic Monte Carlo simulation work to study the effect of diffusion anisotropy, bonding anisotropy and edge diffusion on island formation at different temperatures during the sub-monolayer film growth in Molecular Beam…

Materials Science · Physics 2019-12-13 Jagannath Devkota , Shankar P. Shrestha

Desorption of deposited species plays a role in determining the evolution of surface morphology during crystal growth when the desorption time constant is short compared to the time to diffuse to a defect site, step edge or kink. However,…

In this work we investigate influence of substrate temperature on the surface morphology for substrate coverage below one monolayer. The model of film growth is based on random deposition enriched by limited surface diffusion. Also…

Condensed Matter · Physics 2007-05-23 K. Malarz

Thin film deposition on weakly interacting substrates exhibits a unique growth mode characterized by initially strong island formation and rapidly increasing roughness, which reaches a maximum and subsequently decreases as the film returns…

Pentacene is known to grow on isotropic silicon oxide surfaces in a substrate-induced phase with fiber textured crystallites. This growth study reports on the growth of pentacene crystallites on uniaxially oriented surfaces. Silica…

Materials Science · Physics 2022-07-12 Stefan Pachmajer , Oliver Werzer , Carlo Mennucci , Francesco Buatier de Mongeot , R. Resel

The crystal growth of isotactic polystyrene (it-PS) is investigated in very thin, 11 nm thick films. The it-PS crystals grown in the thin films show quite different morphology from that in the bulk. With decreasing crystallization…

Soft Condensed Matter · Physics 2016-08-31 Ken Taguch , Hideki Miyaji , Kunihide Izumi , Akitaka Hoshino , Yoshihisa Miyamoto , Ryohei Kokawa
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