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Combining insights from quantum chemistry calculations with master equations, we discuss a mechanism for negative differential resistance (NDR) in molecular junctions, operated in the regime of weak tunnel coupling. The NDR originates from…

Mesoscale and Nanoscale Physics · Physics 2013-01-10 Martin Leijnse , Wei Sun , Mogens Brøndsted Nielsen , Per Hedegård , Karsten Flensberg

A new mechanism is proposed to explain the origin of negative differential resistance (NDR) in a strongly coupled single molecule-metal junction. A first-principles quantum transport calculation in a Fe-terpyridine linker molecule…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ranjit Pati , Mike McClain , Anirban Bandyopadhyay

Negative differential resistance (NDR) is tuned at junctions of electronically different dimer and trimer of Rose Bengal on an atomic flat gold (111) surface. Isolated molecule did not show any NDR. But it was induced to show double NDR…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Anirban Bandyopadhyay , Y. Wakayama

Using self-consistent calculations based on Non-Equilibrium Green's Function (NEGF) formalism, the origin of negative differential resistance (NDR) in molecular junctions and quantum wires is investigated. Coupling of the molecule to…

Mesoscale and Nanoscale Physics · Physics 2008-08-21 Hosein Cheraghchi , Keivan Esfarjani

Nonlinear electrical properties, such as negative differential resistance (NDR), are essential in numerous electrical circuits, including memristors. Several physical origins have been proposed to lead to the NDR phenomena in semiconductor…

In this work, we clarify the physical mechanism for the phenomenon of negative output differential resistance (NDR) in short-channel graphene FETs (GFETs) through non-equilibrium Green's function (NEGF) simulations and a simpler…

Mesoscale and Nanoscale Physics · Physics 2012-12-27 Roberto Grassi , Tony Low , Antonio Gnudi , Giorgio Baccarani

A negative differential resistance (NDR) in the nanotransport is often ascribed to electron correlations. We present a simple example which demonstrates that finite electrode bandwidths and energy dependent electrode density of states are…

Mesoscale and Nanoscale Physics · Physics 2010-05-12 Ioan Baldea , Horst Koppel

We unravel the critical role of vibrational mode softening in single-molecule electronic devices at high bias. Our theoretical analysis is carried out with a minimal model for molecular junctions, with mode softening arising due to…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Junjie Liu , Dvira Segal

Reaction currents in chemical networks usually increase when increasing their driving affinities. But far from equilibrium the opposite can also happen. We find that such negative differential response (NDR) occurs in reaction schemes of…

Statistical Mechanics · Physics 2019-07-24 Gianmaria Falasco , Tommaso Cossetto , Emanuele Penocchio , Massimiliano Esposito

We have observed tunable negative differential resistance (NDR) in scanning tunneling spectroscopy measurements of a double layer of C60 molecules on a metallic surface. Using a simple model we show that the observed NDR behavior is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Grobis , A. Wachowiak , R. Yamachika , M. F. Crommie

The effect of electric field, applied on systems in the nanoscale regime has attracted a lot of research in recent times. We highlight some of the recent results in the field of single molecule electronics and then move on to focus on some…

Materials Science · Physics 2008-10-11 S. Lakshmi , Sudipta Dutta , Swapan K. Pati

The negative differential resistance (NDR) response of Nb/NbOx/Pt cross-point devices is shown to have a polarity dependence due to the effect of the metal/oxide Schottky barriers on the contact resistance. Three distinct responses are…

We present the multilevel fabrication and measurement of a Coulomb-blockade device displaying tunable negative differential resistance (NDR). Applications for devices displaying NDR include amplification, logic, and memory circuits. Our…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 C. P. Heij , D. C. Dixon , P. Hadley , J. E. Mooij

We demonstrate that the different magnetic states of a Mn12 molecule can be distinguished in a two-probe transport experiment from a complete knowledge of the current-voltage curve. Our results, obtained with state-of-the-art…

Materials Science · Physics 2009-05-05 C. D. Pemmaraju , I. Rungger , S. Sanvito

Current-controlled (also known as "S-type") negative differential resistance (NDR) is of crucial importance to many emerging applications including neuromorphic computing and high-density memristors integration. However, the experimental…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Miao Wang , Chengyu Wang , Chenchen Wu , Qiao Li , Chen Pan , Cong Wang , Shi-Jun Liang , Feng Miao

The conductance-voltage spectrum of molecular nanostructures measured by scanning tunneling spectroscopy (STS) is generally assumed to reflect the local density of states of the molecule. This excludes the possibility of observing negative…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Yongqiang Xue , Supriyo Datta , Seunghun Hong , R. Reifenberger , Jason I. Henderson , Cliff P. Kubiak

A negative differential resistance (NDR) in a one-dimensional band insulator attached to electrodes is investigated. We systematically examine the effects of an electrode bandwidth and a potential distribution inside the insulator on…

Strongly Correlated Electrons · Physics 2014-11-12 Yasuhiro Tanaka , Kenji Yonemitsu

We investigate the atomic-scale tunneling characteristics of bilayer graphene on silicon carbide using the scanning tunneling microscopy. The high-resolution tunneling spectroscopy reveals an unexpected negative differential resistance…

We determine the conditions in which negative differential resistance (NDR) appears in the C$_{60}$-based molecular device of [Phys. Rev. Lett. {\bf 100}, 036807 (2008)] by means of ab-initio electron-transport simulations. Our calculations…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Frederico D. Novaes , Manuel Cobian , Alberto Garcia , Pablo Ordejon , Hiromu Ueba , Nicolas Lorente

We have studied the transport properties of a molecular device composed of donor and acceptor moieties between two electrodes on either side. The device is considered to be one-dimensional with different on-site energies and the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 S. Lakshmi , Swapan K. Pati
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