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We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…

Materials Science · Physics 2021-05-05 Dino Novko , Vito Despoja , Marcel Reutzel , Andi Li , Hrvoje Petek , Branko Gumhalter

Versatile quantum modes emerge for plasmon describing the collective oscillations of free electrons in metallic nanoparticles when the particle sizes are greatly reduced. Rather than traditional nanoscale study, the understanding of quantum…

We consider the effect of electromagnetic coupling between localized surface plasmons in a metallic nanoparticle (NP) and excitons or weakly interacting electron-hole pairs in a semiconductor matrix where the NP is embedded. An expression…

Mesoscale and Nanoscale Physics · Physics 2018-10-08 Rui M. S. Pereira , Joel Borges , Georgui V. Smirnov , Filipe Vaz , Mikhail I. Vasilevskiy

Scattering scanning near-field optical microscopy enables optical imaging and characterization of plasmonic devices with nanometer-scale resolution well below the diffraction limit. This technique enables developers to probe and understand…

By tuning the radiative coupling of localized surface plasmons to diffracted orders, we demonstrate how stop-gaps in plasmonic crystals of nanorods may be opened and tuned. The stop-gap arises from the mutual coupling of surface lattice…

The effect of smooth shape changes of metallic nanoparticles on localized surface plasmon resonances is assessed with a boundary integral equation method. The boundary integral equation method allows compact expressions of nanoparticle…

Mesoscale and Nanoscale Physics · Physics 2013-02-19 Titus Sandu

Silver nanocrystals made by a chemical reduction of silver salts (AgNO$_3$) by sodium borohydride (NaBH$_4$) were studied using Transmission Electron Microscopy (TEM) and light scattering simulations. For various AgNO$_3$/NaBH$_4$ molar…

Materials Science · Physics 2012-02-22 Annett Thøgersen , Jack Bonsak , Carl Huseby Fosli , Georg Muntingh

Shifting of the surface plasmon resonance wavelength induced by the variation of the thickness of insulating spacer between single layer graphene and Au nanoparticles is studied. The system demonstrates a blue shift of 29 nm as the…

Materials Science · Physics 2015-06-11 Jing Niu , Young Jun Shin , Jaesung Son , Youngbin Lee , Jong Hyun Ahn , Hyunsoo Yang

The surface-enhanced Raman scattering in graphene deposited on AlxGa1-xN/GaN axial heterostructure nanowires was investigated. The intensity of graphene Raman spectra was found not to be correlated with aluminium content. Analysis of…

It is an established understanding that the electromagnetic contribution (the plasmon-mediated enhancement of the laser and scattered local electromagnetic fields) is the main actor in Surface Enhanced Raman Scattering (SERS), with the…

As an interesting surface plasmon phenomenon discovered several years ago, electromagnetic field redistribution in nanoparticle dimer on film system provides a novel thought to enhance the light power on a plain film which could been widely…

Mesoscale and Nanoscale Physics · Physics 2015-11-24 Ting Liu , Jingjing Hao , Yingzhou Huang , Xun Su , Li Hu , Yurui Fang

Nanostructured metal surfaces comprised of periodically arranged spherical voids are grown by electrochemical deposition through a self-assembled template. Detailed measurements of the angle- and orientation-dependent reflectivity reveal…

Optics · Physics 2007-05-23 T. A. Kelf , Y. Sugawara , J. J. Baumberg , M. Abdelsalam , P. N. Bartlett

Ultrafast demagnetization in magnetic nanoparticles using pulsed laser has attracted considerable attention because of its potential applications in spintronics, such as data storage. In such applications, it is necessary to control…

Metal surfaces with disorder or with nanostructure modifications are studied, allowing for a localized charge layer (CL) in addition to continuous charges (CC) in the bulk, both charges having a compressional or diffusive non-local…

Mesoscale and Nanoscale Physics · Physics 2012-07-02 Baruch Horovitz , Carsten Henkel

Surface optical plasmons on metal-dielectric boundaries of various shapes are studied. The study features by the exploration of plasmons of the frequency that is larger than $\omega_{pl}/\sqrt{2}$ and approximately equal to $\omega _{pl}$.…

Optics · Physics 2007-06-13 V. S. Zuev , H. Ya. Zueva

This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Surface plasmons in a centrosymmetric metal nanocrystal have been perceived as achiral, based on the quantum-mechanical theory of molecular optical activity. The one-electron theory is insufficient to describe optical activity in crystals,…

Mesoscale and Nanoscale Physics · Physics 2018-03-02 Jong-Won Park

The long-range action of surface-enhanced Raman scattering (SERS) is probed via distance-dependent measurements of molecular Raman spectra. To this end, identical SERS substrates composed of irregular silver nanoisland arrays were covered…

Materials Science · Physics 2015-06-12 V. I. Kukushkin , A. B. Van'kov , I. V. Kukushkin

The fact that surface-induced damping rate of surface plasmon polaritons (SPPs) in metal nanoparticles increases with the decrease of particle size is well known. We show that this rate also increases with the degree of the mode…

Optics · Physics 2016-01-20 Jacob B Khurgin , Greg Sun

Understanding light-matter interaction at the nanoscale requires probing the optical properties of matter at the individual nano-absorber level. To this end, we have developed a nanomechanical photothermal sensing platform that can be used…

Optics · Physics 2024-06-07 Kostas Kanellopulos , Robert G. West , Silvan Schmid