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We present a theoretical framework to investigate spin chirality in molecular quantum systems. Focusing on a minimal three-spin-center model with antiferromagnetic exchange and symmetry breaking driven by an electric-field-induced…

Mesoscale and Nanoscale Physics · Physics 2025-04-25 Aman Ullah , Ziqi Hu , Juan Aragó , Alejandro Gaita-Ariño

Enantioselective interactions of chiral molecules include distinct absorptions to opposite-handed circularly polarized light, known as chiral absorption. Traditionally, chiral absorption has been primarily attributed to electric dipole and…

Optics · Physics 2024-06-03 Hanwei Wang , Yang Zhao

Photons with spin angular momentum possess intrinsic chirality which underpins many phenomena including nonlinear optics1, quantum optics2, topological photonics3 and chiroptics4. Intrinsic chirality is weak in natural materials, and recent…

We report on a universal topological dichroism of chiral three-dimensional systems in response to the chirality of light. We show that chiral topological invariants result in integer-quantized dichroic excitation rate differences. Moreover,…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 Wojciech J. Jankowski , Giandomenico Palumbo , Robert-Jan Slager

Chirality, a fundamental concept describing an object cannot superpose with its mirror image, is crucial in optics and photonics and leads to various exotic phenomena, such as circular dichroism, and optical activity. Recent findings reveal…

Optics · Physics 2025-01-13 Shijie Kang , Haitao Li , Jiayu Fan , Jiusi Yu , Boyang Qu , Peng Chen , Xiaoxiao Wu

Optical beams with a new and distinctive type of helicity have become the subject of much recent interest. While circularly polarised light comprises photons with spin angular momentum, these optically engineered 'twisted beams' (optical…

Optics · Physics 2015-06-26 David L. Andrews , Luciana C. Davila Romero , Mohamed Babiker

Optimally-chiral electromagnetic fields with maximized helicity density, recently introduced in [1], enable chirality characterization of optically small nanoparticles. Here, we demonstrate a technique to obtain optimally-chiral nearfields…

Applied Physics · Physics 2020-12-02 Mina Hanifeh , Mohammad Albooyeh , Filippo Capolino

In quantum optics, it is common to assume that atoms are point-like objects compared to the wavelength of the electromagnetic field they interact with. However, this dipole approximation is not always valid, e.g., if atoms couple to the…

Quantum Physics · Physics 2022-02-22 Ariadna Soro , Anton Frisk Kockum

It is well-known that many three-dimensional chiral material models become non-chiral when reduced to two dimensions. Chiral properties of the two-dimensional model can then be restored by adding appropriate two-dimensional chiral terms. In…

Mathematical Physics · Physics 2020-06-15 Christian G. Boehmer , Yongjo Lee , Patrizio Neff

Molecular chirality plays a crucial role in innumerable biological processes. The chirality of a molecule can typically be identified by its characteristic optical response, the circular dichroism (CD). CD signals have thus long been used…

Symmetry breaking together with strong spin-orbit interaction give rise to many exciting phenomena within condensed matter physics. A recent example is the existence of chiral spin textures, which are observed in magnetic systems lacking…

Mesoscale and Nanoscale Physics · Physics 2017-09-26 Wanjun Jiang , Gong Chen , Kai Liu , Jiadong Zang , Suzanne G. E. te Velthuis , Axel Hoffmann

We theoretically investigate light matter interactions for chiral molecules in the presence of non-chiral nanoantennas. Isotropic nanostructures supporting optical-frequency electric or magnetic dipoles are sufficient to locally enhance the…

Mesoscale and Nanoscale Physics · Physics 2013-06-14 Aitzol Garcia-Etxarri , Jennifer A. Dionne

We study incidence geometries that are thin and residually connected. These geometries generalise abstract polytopes. In this generalised setting, guided by the ideas from the polytopes theory, we introduce the concept of chirality, a…

Group Theory · Mathematics 2016-04-13 Maria Elisa Fernandes , Dimitri Leemans , Asia Ivić Weiss

Dipoles in triangular optical ladders constitute a flexible platform for the study of the interplay between geometric frustration and long-range anisotropic interactions, and in particular for the observation of the spontaneous onset of…

Chirality arises from the asymmetry of matters, where two counterparts are the mirror image of each other. The interaction between circular-polarization light and quantum materials is enhanced in chiral space groups due to the structural…

Mesoscale and Nanoscale Physics · Physics 2023-09-13 Chang Niu , Shouyuan Huang , Neil Ghosh , Pukun Tan , Mingyi Wang , Wenzhuo Wu , Xianfan Xu , Peide D. Ye

The spin-orbit interaction of light is a crucial concept for understanding the electromagnetic properties of a material and realizing the spin-controlled manipulation of optical fields. Achieving these goals requires a complete description…

Optics · Physics 2022-11-08 Longlong Feng , Qianfan Wu

We show that superconducting correlations in the presence of non-zero condensate velocity can mediate the peculiar interaction between localized spins that breaks the global inversion symmetry of magnetic moments. The proposed interaction…

Superconductivity · Physics 2018-11-26 D. S. Rabinovich , I. V. Bobkova , A. M. Bobkov , M. A. Silaev

Light scattering from chiral plasmonic structures can create near fields with an asymmetry greater than the equivalent circularly polarised light, a property sometimes referred to as superchirality. These near fields with enhanced chiral…

We perform a theoretical and numerical study of the optical properties of both direct and inverse three-dimensional (3D) chiral woodpile structures, and a corresponding chiral Bragg stack. We compute transmission spectra in the helical…

Explorations of symmetry and topology have led to important breakthroughs in quantum optics, but much richer behaviors arise from the non-Hermitian nature of light-matter interactions. A high-reflectivity, non-Hermitian optical mirror can…

Quantum Physics · Physics 2022-08-09 Yi-Cheng Wang , Jhih-Shih You , H. H. Jen