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The quest for mapping the femtosecond dynamics of the electronic band structure of complex materials via Time- and Angle-Resolved Photoelectron Spectroscopy (TR-ARPES) over their full First Brillouin Zone is pushing the development of…

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

Time- and angle-resolved photoelectron spectroscopy (trARPES) employing a 500 kHz extreme-ultravioled (XUV) light source operating at 21.7 eV probe photon energy is reported. Based on a high-power ytterbium laser, optical parametric chirped…

Instrumentation and Detectors · Physics 2019-02-14 M. Puppin , Y. Deng , C. W. Nicholson , J. Feldl , N. B. M. Schroeter , H. Vita , P. S. Kirchmann , C. Monney , L. Rettig , M. Wolf , R. Ernstorfer

We demonstrate a remarkably effective single-stage compression technique for ultrafast pulses in the visible electromagnetic spectrum using second-harmonic pulses at 515 nmderived from a 1030 nm Yb-based femtosecond regenerative amplifier.…

In this work the experimental realization of a tunable high photon flux extreme ultraviolet light source is presented. This is enabled by high harmonic generation of two temporally delayed driving pulses, resulting in a tuning range of 0.8…

A critical technology for high-volume manufacturing of nanoscale integrated circuits is a high-power extreme ultraviolet (EUV) light source. Over the past decades, laser-produced plasma (LPP) sources have been actively utilized in this…

Accelerator Physics · Physics 2025-01-27 Changchao He , Hanxiang Yang , Nanshun Huang , Bo Liu , Haixiao Deng

Extreme ultraviolet (XUV) light sources allow for the probing of bound electron dynamics on attosecond scales, interrogation of high-energy-density matter, and access to novel regimes of strong-field quantum electrodynamics. Despite the…

Time- and angle-resolved photoelectron spectroscopy (trARPES) is a powerful method to track the ultrafast dynamics of quasiparticles and electronic bands in energy and momentum space. We present a setup for trARPES with 22.3 eV…

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

With its direct correspondence to electronic structure, angle-resolved photoemission spectroscopy (ARPES) is a ubiquitous tool for the study of solids. When extended to the temporal domain, time-resolved (TR)-ARPES offers the potential to…

We report on spectroscopy and time-of-flight measurements using an 18 keV fast-pulsed photoelectron source of adjustable intensity, ranging from single photoelectrons per pulse to 5 photoelectrons per microsecond at pulse repetition rates…

Instrumentation and Detectors · Physics 2009-06-19 K. Valerius , M. Beck , H. Arlinghaus , J. Bonn , V. M. Hannen , H. Hein , B. Ostrick , S. Streubel , Ch. Weinheimer , M. Zboril

This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…

We demonstrate experimentally the full tunability of a coherent femtosecond source in the whole ultraviolet spectral region. The experiment relies on the technique of high-order harmonic generation driven by a near-infrared parametric laser…

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

Deep ultraviolet (DUV) laser pulses with tuneable wavelength and very short duration are a key enabling technology for next-generation technology and ultrafast science. Their generation has been the subject of extensive experimental effort,…

Optics · Physics 2023-01-10 Christian Brahms , John C. Travers

Recent progresses in femtosecond ytterbium-doped fiber laser technology areopening new perspectives in strong field physics and attosecond science. Highorder harmonic generation from these systems is particularly interesting because it…

We demonstrate a versatile technique for generating continuously wavelength-tunable laser waveforms, with mJ pulse energies and ultrashort pulse durations down to few-cycle in the ultraviolet C and visible spectral ranges. Using the…

Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet…

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

Optics · Physics 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

We report the generation of the 5th harmonic of Ti:sapphire, at 160 nm, with more than 4~$\mu$J of pulse energy, and a pulse length of 37 fs with a 1 kHz repetition rate. The VUV pulses are produced using Four-Wave Difference Frequency…

Optics · Physics 2024-04-01 Ruaridh Forbes , Paul Hockett , Quentin Leterrier , Rune Lausten