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While important for many industrial applications, chemical reactions responsible for charging of solids in water are often poorly understood. We theoretically investigate the charging kinetics of solid-liquid interfaces, and find that the…

Soft Condensed Matter · Physics 2023-02-08 Willem Boon , Marjolein Dijkstra , René van Roij

Two-dimensional ionic liquids with single site anion and cation-neutral dimer are studied by computer simulations and integral equation techniques, with the aim of characterizing differences with single site anion-cation mixtures, and also…

Chemical Physics · Physics 2018-10-17 Perera Aurélien , Urbic Tomaz

With recent experiments investigating the optical properties of progressively smaller plasmonic particles, quantum effects become increasingly more relevant, requiring a microscopic description. Using the density matrix formalism we analyze…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Alexandra Crai , Andreas Pusch , Doris E. Reiter , Lara Román Castellanos , Tilmann Kuhn , Ortwin Hess

We study the consequences of long-range Coulomb interactions at the critical points between integer/fractional quantum Hall states and an insulator. We use low energy theories for such transitions in anyon gases in the presence of an…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Jinwu Ye , Subir Sachdev

The free energy of ion solvation can be decomposed into enthalpic and entropic contributions. This helps to understand the connection between the dielectric properties and the underlying forces. We present a simple linear-response model of…

Soft Condensed Matter · Physics 2024-06-24 Alec Wills , Anthony Mannino , Isidro Losada , Sara G. Mayo , Jose M. Soler , Marivi Fernandez-Serra

We describe short-time kinetic and steady-state properties of the non--equilibrium phases, namely, solid, liquid and gas anisotropic phases in a driven Lennard-Jones fluid. This is a computationally-convenient two-dimensional model which…

Soft Condensed Matter · Physics 2009-11-11 J. Marro , P. L. Garrido , M. Diez-Minguito

Criticality in a fluid of dielectric constant D that exhibits Ising-type behavior is studied as additional electrostatic (i.e., ionic) interactions are turned on. An exploratory perturbative calculation is performed for small ionicity as…

Soft Condensed Matter · Physics 2009-10-31 A. G. Moreira , M. M. Telo da Gama , M. E. Fisher

The correlation functions of an ionic fluid with charge and size asymmetry are studied within the framework of the random phase approximation. The results obtained for the charge-charge correlation function demonstrate that the…

Statistical Mechanics · Physics 2016-08-31 Oksana Patsahan , Ihor Mryglod , Jean-Michel Caillol

The equilibrium phase diagram of a 1:1 symmetrical mixture composed of oppositely charged colloids is calculated using Monte Carlo simulations. We model the system by the DLVO effective interaction potential. The phase diagram is similar to…

Soft Condensed Matter · Physics 2007-05-23 José B. Caballero , Antonio M. Puertas

We analyze the critical gas-liquid phase behavior of arbitrary fluid mixtures in their coexistence region. We focus on the setting relevant for polydisperse colloids, where the overall density and composition of the system are being…

Soft Condensed Matter · Physics 2019-11-22 Pablo de Castro , Peter Sollich

We consider the system of particles with equal charges and nearest neighbour Coulomb interaction on the interval. We study local properties of this system, in particular the distribution of distances between neighbouring charges. For zero…

Mathematical Physics · Physics 2016-11-08 V. A. Malyshev , A. A. Zamyatin

The theory of first order density-driven phase transitions with frustration due to the long range Coulomb (LRC) interaction develop on paper I of this series is applied to the following physical systems: i) the low density electron gas ii)…

Strongly Correlated Electrons · Physics 2016-08-31 J. Lorenzana , C. Castellani , C. Di Castro

Despite the importance of the electron correlation in the first-principles description of the Li-ion cathode materials, the Coulomb interaction parameter, U is often treated as an ad hoc value. In practice, one usually relies on empirical…

Materials Science · Physics 2021-03-10 Bongjae Kim , Kyoo Kim , Sooran Kim

We have studied properties of quantum charge fluids interacting with random impurities or heavy polarons using a microscopic Hamiltonian with the full many-body Coulomb interaction with the use of variational many-body formalism. At zero…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Mikko Saarela , F V Kusmartsev

The pressure and internal energy of an ultracold plasma in a state of quasi-equilibrium are evaluated using classical molecular dynamics simulations. Coulomb collapse is avoided by modeling electron-ion interactions using an attractive…

Plasma Physics · Physics 2017-04-26 Sanat Kumar Tiwari , Nathaniel R. Shaffer , Scott D. Baalrud

Using {\it ab initio} approaches for extended Hubbard interactions coupled to phonons, we reveal that the intersite Coulomb interaction plays important roles in determining various distinctive phases of the paradigmatic charge ordered…

Strongly Correlated Electrons · Physics 2023-03-30 Bo Gyu Jang , Minjae Kim , Sang-Hoon Lee , Wooil Yang , Seung-Hoon Jhi , Young-Woo Son

We present a systematic study of the effect of the ion pairing on the gas-liquid phase transition of hard-core 1:1 electrolyte models. We study a class of dipolar dimer models that depend on a parameter R_c, the maximum separation between…

Statistical Mechanics · Physics 2009-11-07 J. M. Romero-Enrique , L. F. Rull , A. Z. Panagiotopoulos

We explore the possibility of a Berezinskii-Kosterlitz-Thouless-like critical phase for the charge degrees of freedom in the intermediate-temperature regime between the charge-ordered and disordered phases in two-dimensional systems with…

Strongly Correlated Electrons · Physics 2018-05-23 Ryui Kaneko , Yoshihiko Nonomura , Masanori Kohno

The time-dependent structure, interfacial tension, and evaporation of an oversaturated colloid-rich (liquid) phase in contact with an undersaturated colloid-poor (vapor) phase of a colloidal dispersion is investigated theoretically during…

Soft Condensed Matter · Physics 2014-05-08 Markus Bier , Daniel Arnold

We first explore the liquid-gas mixed phase in a bulk calculation, where two phases coexist without the geometrical structures. In the case of symmetric nuclear matter, the system behaves congruently, and the Maxwell construction becomes…

Nuclear Theory · Physics 2015-06-04 Toshiki Maruyama , Toshitaka Tatsumi