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We demonstrate a novel method to determine the longitudinal phase-space distribution of a cryogenic buffer gas beam of barium-fluoride molecules based on a two-step laser excitation scheme. The spatial resolution is achieved by a…

We report measurements of the dynamics of isolated $^{8}$Li$^{+}$ in single crystal rutile TiO$_{2}$ using $\beta$-detected NMR. From spin-lattice relaxation and motional narrowing, we find two sets of thermally activated dynamics: one…

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…

Atomic Physics · Physics 2019-07-24 L. Caldwell , J. A. Devlin , H. J. Williams , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We calculate the light-induced collisional loss of laser-cooled and trapped magnesium atoms for detunings up to 50 atomic linewidths to the red of the ^1S_0-^1P_1 cooling transition. We evaluate loss rate coefficients due to both radiative…

Atomic Physics · Physics 2009-11-07 M. Machholm , Paul S. Julienne , K. -A. Suominen

Atomic vapor of four different paramagnetic species: gold, silver, lithium, and rubidium, is produced and studied inside several buffer gases: helium, nitrogen, neon, and argon. The paramagnetic atoms are injected into the buffer gas using…

Atomic Physics · Physics 2009-11-13 A. O. Sushkov , D. Budker

Electronic instabilities in transition metal compounds often spontaneously form orbital molecules, which consist of orbital-coupled metal ions at low temperature. Recent local structural studies utilizing the pair distribution function…

A simple method to control molecular translation with a chemical reaction is demonstrated. Slow NO molecules have been produced by partially canceling the molecular beam velocity of NO$_2$ with the recoil velocity of the NO photofragment.…

Chemical Physics · Physics 2009-09-10 Bum Suk Zhao , So Eun Shin , Sung Tai Park , Xingnan Sun , Doo Soo Chung

Diatomic nitrogen is an archetypal molecular system known for its exceptional stability and complex behavior at high pressures and temperatures, including rich solid polymorphism, formation of energetic states, and an insulator-to-metal…

We report laser cooling of fermionic K-40 atoms, with temperatures down to (15 +/- 5) microK, for an enriched sample trapped in a MOT and additionaly cooled in optical molasses. This temperature is a factor of 10 below the Doppler-cooling…

Statistical Mechanics · Physics 2009-10-31 G. Modugno , C. Benko , P. Hannaford , G. Roati , M. Inguscio

In this paper laser cooling of atoms with a narrow-line optical transition, i.e. in regimes of quantum nature of laser-light interactions resulting in a significant recoil effect, is studied. It is demonstrated that a minimum laser cooling…

Atomic Physics · Physics 2019-03-06 O. N. Prudnikov , R. Ya Il'enkov , A. V. Taichenachev , V. I. Yudin

Highly stable laser sources based on narrow atomic transitions provide a promising platform for direct generation of stable and accurate optical frequencies. Here we investigate a simple system operating in the high-temperature regime of…

We have carried out extensive isokinetic {\it ab initio} molecular dynamic simulations to investigate the finite temperature properties of the impurity doped cluster Li$_6$Sn along with the host cluster Li$_7$. The data obtained from about…

Condensed Matter · Physics 2009-11-10 Kavita Joshi , D. G. Kanhere

We describe the realization of a magnetically guided beam of cold rubidium atoms, with a flux of $7\times 10^9$ atoms/s, a temperature of 400 $\mu$K and a mean velocity of 1 m/s. The rate of elastic collisions within the beam is sufficient…

Other Condensed Matter · Physics 2009-11-10 T. Lahaye , J. M. Vogels , K. Guenter , Z. Wang , J. Dalibard , D. Guery-Odelin

Magnetic trapping of bromine atoms at temperatures in the milliKelvin regime is demonstrated for the first time. The atoms are produced by photodissociation of Br$_2$ molecules in a molecular beam. The lab-frame velocity of Br atoms is…

Atomic Physics · Physics 2014-02-21 C. J. Rennick , J. Lam , W. G. Doherty , T. P. Softley

We report observation of sub-Doppler cooling of lithium using an irregular-tetrahedral laser beam arrangement, which is produced by a nanofabricated diffraction grating. We are able to capture 11(2) % of the lithium atoms from a grating…

Atomic Physics · Physics 2022-03-23 D. S. Barker , E. B. Norrgard , N. N. Klimov , J. A. Fedchak , J. Scherschligt , S. Eckel

In this work we study the diffusion mechanisms in lithium disilicate melt using molecular dynamics simulation, which has an edge over other simulation methods because it can track down actual atomic rearrangements in materials once a…

Materials Science · Physics 2014-05-30 Luis G. V. Gonçalves , José P. Rino

The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He$_2^*$ would enable a new generation of precision measurements to test quantum…

Atomic Physics · Physics 2025-05-22 Lucía Verdegay , Bingcheng Zeng , Daniel Y. Knapp , Jack C. Roth , Maximilian Beyer

The direct laser cooling of neutral diatomic molecules in molecular beams suggests that trapped molecular ions can also be laser cooled. The long storage time and spatial localization of trapped molecular ions provides the opportunity for…

We employ semiclassical theoretical analysis to study laser cooling of free atoms using three-level cascade transitions, where the upper transition is much weaker than the lower one. This represents an alternate cooling scheme, particularly…

Atomic Physics · Physics 2015-06-16 Flavio C. Cruz , Michael L. Sundheimer , Wictor C. Magno

Superconducting thin films have been prepared on Si-substrates, using pulsed laser deposition from a target composed of a mixture of Mg and MgB2 powders. The films were deposited at room temperature and post-annealed at 600 degrees C. The…