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Several thermodynamic properties of ice Ih, II, and III are studied by a quasi-harmonic approximation and compared to results of quantum path integral and classical simulations. This approximation allows to obtain thermodynamic information…

Chemical Physics · Physics 2012-09-24 R. Ramirez , N. Neuerburg , M. -V. Fernandez-Serra , C. P. Herrero

A mixture of solvent particles with short-range, directional interactions and solute particles with short-range, isotropic interactions that can bond multiple times is of fundamental interest in understanding liquids and colloidal mixtures.…

Soft Condensed Matter · Physics 2016-09-21 Artee Bansal , D. Asthagiri , Kenneth R. Cox , Walter G. Chapman

We perform the analysis of predictions of a classical density functional theory for associating fluids with different association strength concerned with wetting of solid surfaces. The four associating sites water-like models with…

Soft Condensed Matter · Physics 2024-04-01 A. Kozina , M. Aguilar , O. Pizio , S. Sokołowski

This work is an attempt to give a brief overview of the implementation of the statistical ther- modynamics to hadronic matter. The possibility to use the hydrodynamic approach for developing the physical model of the formation of exotic…

Nuclear Theory · Physics 2015-09-23 K. V. Cherevko , L. L. Jenkovszky , V. M. Sysoev , Feng-Shou Zhang

Thermodynamics (in concert with its sister discipline, statistical physics) can be regarded as a data reduction scheme based on partitioning a total system into a subsystem and a bath that weakly interact with each other. The ubiquity and…

Statistical Mechanics · Physics 2009-11-11 David Ford , Steven Huntsman

Dynamic heterogeneity as one of the most important properties in supercooled liquids has been found for several decades. However, its structural origin remains open for many systems. Here, we propose a new structural parameter to…

Disordered Systems and Neural Networks · Physics 2015-10-16 S. P. Pan , S. D. Feng , J. W. Qiao , W. M. Wang , J. Y. Qin

One dramatic feature of network liquids is the emergence at low temperatures and high pressures of polyamorphism, where multiple distinct liquid phases are accessed in a single material. Polyamorphism can arise from the competition between…

Soft Condensed Matter · Physics 2026-05-07 Max Hall-Brown , Peter Guy Wolynes

It has recently been shown that the TIP4P/Ice model of water can be studied numerically in metastable equilibrium at and below its liquid-liquid critical temperature. We report here simulations along a subcritical isotherm, for which two…

Soft Condensed Matter · Physics 2021-06-02 Riccardo Foffi , John Russo , Francesco Sciortino

A calculational approach in fluid turbulence is presented. Use is made of the attracting nature of the fluid-dynamic dynamical system. An approximate approach is offerred that effectively propagates the statistics in time. Loss of…

Fluid Dynamics · Physics 2007-05-23 Edsel A. Ammons

We regularize the potential distribution framework to calculate the excess free energy of liquid water simulated with the BLYP-D density functional. The calculated free energy is in fair agreement with experiments but the excess internal…

Chemical Physics · Physics 2015-05-19 Valéry Weber , D. Asthagiri

Water plays a fundamental role in the structure and function of proteins and other biomolecules. The thermodynamic profile of water molecules surrounding a protein are critical for ligand binding and recognition. Therefore, identifying the…

Biomolecules · Quantitative Biology 2024-11-26 Florian B. Hinz , Matthew R. Masters , Julia N. Kieu , Amr H. Mahmoud , Markus A. Lill

Quantitative prediction of thermodynamic properties in solution is essential for translating atomistic simulations into reliable chemical insight. As an exemplar system, the behaviour of CaCO$_3$ in water has been widely studied to…

Liquid water, besides being fundamental for life on Earth, has long fascinated scientists due to several anomalies. Different hypotheses have been put forward to explain these peculiarities. The most accredited one foresees the presence in…

Numerical Analysis · Mathematics 2022-10-26 Michele Benzi , Isabella Daidone , Chiara Faccio , Laura Zanetti-Polzi

Reactive chemistry of molecular hydrogen at surfaces, notably dissociative sticking and hydrogen evolution, plays a crucial role in energy storage and fuel cells. Theoretical studies can help to decipher underlying mechanisms and reaction…

Formalism based on equilibrium statistical thermodynamics is applied to communication networks of decision making individuals. It is shown that in statistical ensembles for choice models, properly defined disutility can play the same role…

Statistical Mechanics · Physics 2007-05-23 Arkadiusz Majka , Wojciech Wislicki

Last years, there has been a renewed interest in the utilization of statistical field theory methods for the description of systems at equilibrium both in the vicinity and away from critical points, in particular in the field of liquid…

Statistical Mechanics · Physics 2012-07-02 Vincent Russier , Jean-Michel Caillol

Thermodynamic and structural properties of the tangent diatomic fluid are studied in the framework provided by the Reference Interaction Site Model (RISM) theory, coupled with a Modified Hypernetted Chain closure. The enforcement of the…

Statistical Mechanics · Physics 2009-11-13 G. Munao' , D. Costa , C. Caccamo

Chemical equilibrium is fully characterized by thermodynamics, while the rates of chemical reactions can be calculated for ideal solutions by using mass-action equations. The evaluation of the rates of reactions in a non-ideal system is…

Chemical Physics · Physics 2025-01-20 Doriano Brogioli , Fabio La Mantia

An ensemble of classical subsystems interacting with surrounding particles has been considered. In general case, a phase volume of the subsystems ensemble was shown to be a function of time. The evolutional equations of the ensemble are…

Statistical Mechanics · Physics 2015-06-24 S. R. Sharov

Relevant and fundamental concepts of the statistical mechanical theory of classical liquids are ordinarily introduced in the context of the description of thermodynamic equilibrium states. This makes explicit reference to probability…

Statistical Mechanics · Physics 2024-01-30 O. Joaquín-Jaime , R. Peredo-Ortiz , M. Medina-Noyola , L. F. Elizondo-Aguilera