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Characterization of the molecular properties of surfaces under ambient or chemically reactive conditions is a fundamental scientific challenge. Moreover, many traditional analytical techniques used for probing surfaces often lack dynamic or…

We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

Nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) spectroscopy of bulk quantum materials have provided insight into phenomena such as quantum phase criticality, magnetism, and superconductivity. With the emergence of…

We present a novel approach to the detection of weak magnetic fields that takes advantage of recently developed techniques for the coherent control of solid-state electron spin quantum bits. Specifically, we investigate a magnetic sensor…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. M. Taylor , P. Cappellaro , L. Childress , L. Jiang , D. Budker , P. R. Hemmer , A. Yacoby , R. Walsworth , M. D. Lukin

Nitrogen-vacancy centers in diamond are a promising platform for nanoscale nuclear magnetic resonance sensing. Despite significant progress towards using NV centers to detect and localize nuclear spins down to the single spin level,…

The nitrogen-vacancy (NV) center is an emerging platform for constructing inertial sensors. Its native nitrogen spin can serve as a gyroscope using Ramsey interferometry protocols. The sensitivities of these nuclear-spin-based NV gyroscopes…

Quantum Physics · Physics 2025-02-03 Johnathan Kuan , Gregory D. Fuchs

We demonstrate a technique to nanofabricate nitrogen vacancy (NV) centers in diamond based on broad-beam nitrogen implantation through apertures in electron beam lithography resist. This method enables high-throughput nanofabrication of…

Mesoscale and Nanoscale Physics · Physics 2010-08-02 David M. Toyli , Christoph D. Weis , Gregory D. Fuchs , Thomas Schenkel , David D. Awschalom

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

The sensing capability of a single optically bright electronic spin in diamond can be enhanced by making use of proximal dark nuclei as ancillary spins. Such systems, so far only realized in bulk diamond, provide orders of magnitude higher…

Quantum Physics · Physics 2017-10-04 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Nuclear spins in the solid state environment of diamond are highly coherent, but difficult to rapidly control due to the small nuclear gyromagnetic ratio. Here we demonstrate a more than 50-fold enhancement of the effective nuclear…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 S. Sangtawesin , J. R. Petta

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

We present a technique that uses an ensemble of nitrogen-vacancy (NV) centers in diamond to image magnetic fields with high spatio-temporal resolution and sensitivity. A focused laser beam is raster-scanned using an acousto-optic deflector…

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

We present a method to directly detect the axion dark matter using nitrogen vacancy centers in diamonds. In particular, we use metrology leveraging the nuclear spin of nitrogen to detect axion-nucleus couplings. This is achieved through…

High Energy Physics - Phenomenology · Physics 2025-05-01 So Chigusa , Masashi Hazumi , Ernst David Herbschleb , Yuichiro Matsuzaki , Norikazu Mizuochi , Kazunori Nakayama

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

Quantum Physics · Physics 2024-11-12 Yuhang Ren , Susumu Takahashi

The negatively-charged nitrogen-vacancy center (NV) in diamond forms a versatile system for quantum sensing applications. Combining the advantageous properties of this atomic-sized defect with scanning probe techniques such as atomic force…

Mesoscale and Nanoscale Physics · Physics 2018-12-26 Philipp Fuchs , Michel Challier , Elke Neu

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…

Nitrogen-vacancy (NV) centers in diamond are a leading modality for magnetic sensing and imaging under ambient conditions. However, these sensors suffer from degraded performance due to paramagnetic impurities and regions of stress in the…

Quantum Physics · Physics 2024-04-22 Connor Roncaioli , Connor Hart , Ronald Walsworth , Donald P. Fahey

Single nitrogen-vacancy (NV) centers are widely used as nanoscale sensors for magnetic and electric fields, strain and temperature. Nanoscale magnetometry using NV centers allows for example to quantitatively measure local magnetic fields…

The negatively charged nitrogen-vacancy (NV$^-$) center in diamond is a model quantum system for university teaching labs due to its room-temperature compatibility and cost-effective operation. Based on the low-cost experimental setup that…