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We present and characterize a 2-D imaging spectrometer based on a virtually-imaged phased array (VIPA) disperser for rapid, high-resolution molecular detection using mid-infrared (MIR) frequency combs at 3.1 and 3.8 \mu m. We demonstrate…

We present quasi-real-time dual-comb spectroscopy (DCS) using two Yb:fiber combs with ~750 MHz repetition rates. A computational coherent averaging technique is employed to correct timing and phase fluctuations of the measured dual-comb…

We perform heterodyne spectroscopy at 1.56 micron with a tunable laser and thermal radiation from the Sun. The laser tuning is calibrated with a frequency comb, providing a simple spectrometer with absolute frequency tracebility and…

Instrumentation and Methods for Astrophysics · Physics 2020-11-17 Connor Fredrick , Freja Olsen , Ryan Terrien , Suvrath Mahadevan , Franklyn Quinlan , Scott Diddams

Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities…

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

A 12.5 GHz-spaced optical frequency comb locked to a Global Positioning disciplined oscillator for near-IR spectrograph calibration is presented. The comb is generated via filtering a 250 MHz-spaced comb. Subsequency nonlinear broadening of…

Optics · Physics 2015-05-18 F. Quinlan , G. Ycas , S. Osterman , S. Diddams

We describe a successful effort to produce a laser comb around 1.55 $\mu$m in the astronomical H band using a method based on a line-referenced, electro-optical-modulation frequency comb. We discuss the experimental setup, laboratory…

Instrumentation and Methods for Astrophysics · Physics 2016-06-08 X. Yi , K. Vahala , S. Diddams , G. Ycas , P. Plavchan , S. Leifer , J. Sandhu , G. Vasisht , P. Chen , P. Gao , J. Gagne , E. Furlan , M. Bottom , E. Martin , M. Fitzgerald , G. Doppmann , C. Beichman

Optical spectroscopic sensors are powerful tools for analysing gas mixtures in industrial and scientific applications. Whilst highly sensitive spectrometers tend to have a large footprint, miniaturized optical devices usually lack…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

The ability to detect and identify molecules at high sensitivity without the use of labels or capture agents is important for medical diagnostics, threat identification, environmental monitoring, and basic science. Microtoroid optical…

Optics · Physics 2022-10-17 Gwangho Choi , Adley Gin , Judith Su

High-resolution spectroscopy in the near-infrared could become the leading method for discovering extra-solar planets around very low-mass stars and brown dwarfs. To help to achieve an accuracy of ~m/s, we are developing a gas cell which…

Instrumentation and Methods for Astrophysics · Physics 2015-05-18 L. Valdivielso , P. Esparza , E. Martín

Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…

We report an approach for high-resolution spectroscopy using a widely tunable laser emitting in the molecular fingerprint region. The laser is based on difference-frequency generation (DFG) in a nonlinear orientation-patterned GaAs crystal.…

Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…

Quantum Physics · Physics 2023-03-30 Alexandre Belsley

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…

The remarkable precision of frequency comb (FC) lasers is transferred to the extreme ultraviolet (XUV, wavelengths shorter than 100 nm), a frequency region previously not accessable to these devices. A frequency comb at XUV wavelengths near…

We demonstrate a new simple technique to measure IR frequencies near 30 THz using a femtosecond (fs) laser optical comb and sum-frequency generation. The optical frequency is directly compared to the distance between two modes of the fs…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Intracavity laser absorption spectroscopy (ICLAS) with an evacuated Cr2+: ZnSe laser is performed with a high-resolution time-resolved Fourier transform interferometer with a minimum detectable absorption coefficient equal to 4 10-9 cm-1…

Noise-immune cavity-enhanced optical frequency comb spectroscopy (NICE-OFCS) is a recently developed technique that utilizes phase modulation to obtain immunity to frequency-to-amplitude noise conversion by the cavity modes and yields high…

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