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Increasing the sweep rate of mid-infrared (MIR) frequency-swept sources offers significant potential for various high-speed spectroscopy-based applications. While continuous-wave frequency-swept lasers have achieved sweep rates up to 1 MHz,…

Gas samples relevant to health and environment typically contain a plethora of molecular species that span a huge concentration dynamic range. High-concentration molecules impose a strong absorption background that hinders robust…

Optics · Physics 2024-06-07 Qizhong Liang , Apoorva Bisht , Andrew Scheck , Peter G. Schunemann , Jun Ye

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…

We report multipass broadband photoacoustic spectroscopy of trace gases in the mid-infrared. The measurement principle of the sensor relies on supercontinuum-based Fourier transform photoacoustic spectroscopy (FT-PAS), in which a scanning…

Instrumentation and Detectors · Physics 2022-08-31 Tommi Mikkonen , Tuomas Hieta , Goëry Genty , Juha Toivonen

Measuring low light absorption with combined uncertainty < 1 permille is crucial in a wide range of applications. Popular cavity ring-down spectroscopy can provide ultra-high precision, below 0.01 permille, but its accuracy is strongly…

Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne…

We demonstrate a high-accuracy dual-comb spectrometer centered at 3.4 \mu m. The amplitude and phase spectra of the P, Q, and partial R-branch of the methane {\nu}3 band are measured at 25 MHz to 100 MHz point spacing with ~kHz resolution…

Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…

Optics · Physics 2020-04-23 David Burghoff

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

Frequency combs based on nonlinear-optical phenomena in integrated photonics are a versatile light source that can explore new applications, including frequency metrology, optical communications, and sensing. We demonstrate robust…

We demonstrate a 0.95 GHz repetition rate fully stabilized Yb:fiber frequency comb without optical amplification. Benefitted from the high mode power and high coherence, this comb achieved 35 dB to 42 dB signal to noise ratio on the direct…

Optics · Physics 2019-10-02 Yuxuan Ma , Fei Meng , Yan Wang , Aimin Wang , Zhigang Zhang

High-resolution ultrasound based imaging techniques like photoacoustic (PA) imaging that require fast detection of acoustic waves, are often coupled with an opto-mechanical sensor like a Fabry-Perot cavity (FPC) for enhanced sensitivity at…

Harnessing the quantum interference of photon-pair generation processes, infrared quantum absorption spectroscopy (IRQAS) can extract the infrared optical properties of a sample through visible or near-infrared photon detection without the…

Optics · Physics 2022-06-22 Yu Mukai , Ryo Okamoto , Shigeki Takeuchi

A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…

Optics · Physics 2007-09-24 Julien Mandon , Guy Guelachvili , Nathalie Picqué

Supercontinua generated in highly non-linear fibers by ultrashort-pulse lasers can be used for high resolution Fourier transform absorption spectroscopy. The practical advantages of these bright ultrabroadband light sources for spectroscopy…

The discovery and characterization of exoplanets around nearby stars is driven by profound scientific questions about the uniqueness of Earth and our Solar System, and the conditions under which life could exist elsewhere in our Galaxy.…

Advances in high-resolution laser spectroscopy have enabled many scientific breakthroughs in physics, chemistry, biology and astronomy. Optical frequency combs have pushed measurement limits with ultrahigh-frequency accuracy and…

Optics · Physics 2023-03-27 Shuangyou Zhang , Toby Bi , Pascal Del'Haye

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…

Optics · Physics 2020-01-16 Noh Soo Han , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

A direct measurement of the universe's expansion history could be made by observing in real time the evolution of the cosmological redshift of distant objects. However, this would require measurements of Doppler velocity drifts of about 1…

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