Related papers: Laser induced ultrafast demagnetization: an \emph{…
Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…
The control of antiferromagnetic order can pave the way to large storage capacity as well as fast manipulation of stored data. Here achieving a steady-state of sublattice magnetization after switching is crucial to prevent loss of stored…
Synthetic ferrimagnets are composite magnetic structures formed from two or more anti- ferromagnetically coupled magnetic sublattices with different magnetic moments. Here we report on atomistic spin simulations of the laser-induced…
Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely-used three-temperature model (3TM). Here, we…
The magnetization of a non-magnetic semiconductor by femtosecond light pulses is crucial to achieve an all-optical control of the spin dynamics in materials and to develop faster memory devices. However, the conditions for its detection are…
Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…
The first principles momentum dependent local ansatz wavefunction method (MLA) has been extended to the ferromagnetic state by introducing spin-dependent variational parameters. The theory is applied to the ferromagnetic Fe, Co, and Ni. It…
Laser-induced femtosecond demagnetization, femtomagnetism, offers a potential route to develop faster magnetic storage devices. It is generally believed that the traditional spin-wave theory, which is developed for thermally driven slow…
Ultrafast magnetization dynamics in metallic heterostructures consists of a combination of local demagnetization in the ferromagnetic constituent and spin-dependent transport contributions within and in between the constituents. Separation…
Despite spin (SAM) and orbital (OAM) angular momentum dynamics are well-studied in demagnetization processes, their components receive less focus. Here, we utilize the non-collinear spin version of real-time time-dependent density…
We study the ultrafast demagnetization dynamics of LnRh$_2$Si$_2$ (Ln $=$ Pr, Nd, Sm, Gd, Tb, Dy, Ho) antiferromagnets (AFM) after excitation by a laser pulse, using a combination of density functional theory and atomistic spin and…
We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz…
We present an investigation of the electron spin dynamics in an ensemble of singly-charged quantum dots subject to an external magnetic field and laser pumping with circularly polarized light. The spectral laser width is tailored such that…
We present the first materials specific ab initio theory of the magnetization induced by circularly polarized laser light in metals. Our calculations are based on non-linear density matrix theory and include the effect of absorption. We…
A circularly polarized laser pulse can induce persistent intra-molecular currents by either exciting or ionizing molecules. These two cases are identified as electron currents and hole currents, respectively, and up to now they have been…
Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…
By correlating time- and angle-resolved photoemission and time-resolved transverse- magneto- optical Kerr effect measurements, both at extreme ultraviolet wavelengths, we uncover the universal nature of the ultrafast photoinduced magnetic…
The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…
We use a non-equilibrium many-body theory that engages the elements of transient coherence, correlation, and nonlinearity to describe changes in the magnetic and electronic phases of strongly correlated systems induced by femtosecond…
Since the discovery of ultrafast demagnetization in Ni thin films in 1996, laser-induced ultrafast spin dynamics have become a prominent research topic in the field of magnetism and spintronics. This development offers new possibilities for…