Related papers: Laser induced ultrafast demagnetization: an \emph{…
Using time-dependent density functional theory, applied to valence electrons, coupled non-adiabatically to molecular dynamics of the ions, we study the induced dynamics of ethylene subjected to the laser field. We demonstrate the reliable…
Optically-induced phase transitions of the manganite $\rm Pr_{1/3}Ca_{2/3}MnO_3$ have been simulated using a model Hamiltonian, that captures the dynamics of strongly correlated charge, orbital, lattice, and spin degrees of freedom. Its…
Microscopic origins of charge currents and electromagnetic (EM) radiation generated by them in spintronic THz emitters -- such as, femtosecond laser pulse-driven single magnetic layer or its heterostructures with a nonmagnetic layer hosting…
We study the non-equilibrium dynamics of driven spin lattices in the presence of decoherence caused by either laser phase noise or strong decay. In the first case, we discriminate between correlated and uncorrelated noise and explore their…
We present the time-dependent complete-active-space self-consistent-field (TD-CASSCF) method to simulate multielectron dynamics in ultrafast intense laser fields from the first principles. While based on multiconfiguration expansion, it…
Understanding the correlation between fast and ultrafast demagnetization processes is crucial for elucidating the microscopic mechanisms underlying ultrafast demagnetization, which is pivotal for various applications in spintronics. Initial…
Designing material properties on demand has important implications to potential future technological applications. While theoretically it is always possible to tune various intrinsic energy scales, there are fundamental limitations to this…
By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much…
Spin-controlled lasers are highly interesting photonic devices and have been shown to provide ultra-fast polarization dynamics in excess of 200 GHz. In contrast to conventional semiconductor lasers their temporal properties are not limited…
Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. Several microscopic mechanisms have been proposed to explain the observations, including the transport of ultrashort spin-polarized…
A novel method invented to measure the minute thermodynamic spin magnetization of dilute two dimensional fermions is applied to electrons in a silicon inversion layer. Interplay between the ferromagnetic interaction and disorder enhances…
Engineering and controlling heat and spin transport on the femtosecond time-scale in spintronic devices opens up new ways to manipulate magnetization with unprecedented speed. Yet the underlying reversal mechanisms remain poorly understood…
We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…
Electron spin dephasing in a singly charged semiconductor quantum dot can partially be suppressed by periodic laser pulsing. We propose a semi-classical approach describing the decoherence of the electron spin polarization governed by the…
We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…
Terahertz (THz) lasers provide a new research perspective for spin electronics applications due to their sub-picosecond time resolution and non-thermal ultrafast demagnetization, but the interaction between spin, charge and lattice dynamics…
The ability to controllably manipulate the laser-induced ultrafast magnetic dynamics is a prerequisite for future high speed spintronic devices. The optimization of devices requires the controllability of the ultrafast demagnetization time,…
In our previous work [J. Chem. Phys. \textbf{136}, 024502 (2012)], we reported a demixing phase transition of a two-dimensional, binary Heisenberg fluid mixture driven by the ferromagnetic interactions of the magnetic species. Here, we…
We describe an ab initio and non-perturbative $R$-matrix with time-dependence theory for ultrafast atomic processes in light fields of arbitrary polarization. The theory is applicable to complex, multielectron atoms and atomic ions subject…
We determine the localization threshold in a partially filled and orbitally degenerate model of correlated electrons. Particular emphasis is put on a non-integer band filling, when the system decomposes into the localized and the itinerant…