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Related papers: Laser induced ultrafast demagnetization: an \emph{…

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Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

We use transient absorption spectroscopy with circularly polarized x-rays to detect laser-excited hole states below the Fermi level and compare their dynamics with that of unoccupied states above the Fermi level in ferromagnetic [Co/Pd]…

Exploring ultrafast magnetization control in two-dimensional (2D) magnets through optically driven coherent phonons has been well-established. Yet, the microscopic interplay between spin dynamics and lattice degrees of freedom remains less…

Computational Physics · Physics 2024-03-25 Zhaobo Zhou , Min Li , Thomas Frauenheim , Junjie He

Demagnetization in ferromagnetic transition metals driven by a femtosecond laser pulse is a fundamental problem in solid state physics, and its understanding is essential to the development of spintronics devices. Ab initio calculation of…

Materials Science · Physics 2024-01-02 Mitsuko Murakami , G. P. Zhang

We propose a semi-classical model for femtosecond-laser induced demagnetization due to spin-polarized excited electron diffusion in the super-diffusive regime. Our approach treats the finite elapsed time and transport in space between…

Materials Science · Physics 2011-06-14 Marco Battiato , Karel Carva , Peter M. Oppeneer

We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr$_{2}$O$_{3}$. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast…

Strongly Correlated Electrons · Physics 2017-06-29 Feng Guo , Na Zhang , Wei Jin , Jun Chang

The dynamics of single laser-driven electrons and many particle systems with spin are investigated on the basis of a classical theory. We demonstrate that the spin forces can alter the electron dynamics in an ultra-relativistic laser field…

Plasma Physics · Physics 2014-06-17 Meng Wen , Heiko Bauke , Christoph H. Keitel

With the goal of pushing Spintronic devices towards faster and faster timescales, we demonstrate, using ab-intio time-dependent density functional theory simulations of bulk Heusler compounds subject to ultrashort intense laser pulses, that…

Materials Science · Physics 2016-03-18 P. Elliott , T. Müller , J. K. Dewhurst , S. Sharma , E. K. U. Gross

We report on {\it ab-initio} simulations of the quantum dynamics of electronic charge and spin when subjected to intense laser pulses. By performing separate calculations for a Ni thin film and bulk Ni, we conclude that surface effects have…

Materials Science · Physics 2017-05-24 K. Krieger , P. Elliott , T. Müller , N. Singh , J. K. Dewhurst , E. K. U. Gross , S. Sharma

Spin current flowing between femtosecond laser pulse (fsLP)-driven ferromagnetic metal and adjacent normal metal (NM) hosting strong spin-orbit coupling is invariably invoked to explain terahertz (THz) radiation believed to be emitted…

Mesoscale and Nanoscale Physics · Physics 2025-04-30 Ali Kefayati , Yafei Ren , M. Benjamin Jungfleisch , Lars Gundlach , John Q. Xiao , Branislav K. Nikolic

The ultra-fast demagnetization of small iron clusters initiated by an intense optical excitation is studied with time-dependent spin density functional theory (TDSDFT). In particular we investigate the effect of the spin-orbit interaction…

Mesoscale and Nanoscale Physics · Physics 2016-07-27 Maria Stamenova , Jacopo Simoni , Stefano Sanvito

Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

Materials Science · Physics 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

Materials Science · Physics 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

We apply the coupled dynamics of time-dependent density functional theory and Maxwell equations to the interaction of intense laser pulses with crystalline silicon. As a function of electromagnetic field intensity, we see several regions in…

Other Condensed Matter · Physics 2015-06-03 K. Yabana , T. Sugiyama , Y. Shinohara , T. Otobe , G. F. Bertsch

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

Materials Science · Physics 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby

Ultrafast magnetization dynamics are governed by energy flow between electronic, magnetic, and lattice degrees of freedom. A quantitative understanding of these dynamics must be based on a model that agrees with experimental results for all…

We report a computational theoretical investigation of electron spin-flip scattering induced by the electron-phonon interaction in the transition-metal ferromagnets bcc Fe, fcc Co and fcc Ni. The Elliott-Yafet electron-phonon spin-flip…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 K. Carva , M. Battiato , D. Legut , P. M. Oppeneer

Laser-induced ultrafast demagnetization is an important phenomenon that probes arguably ultimate limits of the angular momentum dynamics in solid. Unfortunately, many aspects of the dynamics remain unclear except that the demagnetization…

Materials Science · Physics 2023-07-03 Kyuhwe Kang , Hiroki Omura , Oukjae Lee , Kyung-Jin Lee , Hyun-Woo Lee , Tomoyasu Taniyama , Gyung-Min Choi

The ultrafast dynamics of magnetic order in a ferromagnet are governed by the interplay between electronic, magnetic and lattice degrees of freedom. In order to obtain a microscopic understanding of ultrafast demagnetization, information on…

We study the ultrafast demagnetization of Ni/NiMn and Co/NiMn ferromagnetic/antiferromagnetic bilayer systems after excitation by a laser pulse. We probe the ferromagnetic order of Ni and Co using magnetic circular dichroism in…