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We show that it is possible to realize significant nonlinear optical interactions at the few photon level in graphene nanostructures. Our approach takes advantage of the electric field enhancement associated with the strong confinement of…

Mesoscale and Nanoscale Physics · Physics 2014-08-11 M. Gullans , D. E. Chang , F. H. L. Koppens , F. J. García de Abajo , M. D. Lukin

The linear electronic dispersion relation of graphene endows the atomically thin carbon layer with a large intrinsic optical nonlinearity, with regard to both parametric and photothermal processes. While plasmons in graphene nanostructures…

Mesoscale and Nanoscale Physics · Physics 2026-02-05 Line Jelver , Joel D. Cox

Electrically tunable graphene plasmons are anticipated to enable strong light-matter interactions with resonant quantum emitters. However, plasmon resonances in graphene are typically limited to infrared frequencies, below those of optical…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Joel D. Cox , F. Javier García de Abajo

We analyze nonlinear optics schemes for generating pairs of quantum entangled plasmons in the terahertz-infrared range in graphene. We predict that high plasmonic field concentration and strong optical nonlinearity of monolayer graphene…

Mesoscale and Nanoscale Physics · Physics 2022-06-17 Zhiyuan Sun , D. N. Basov , M. M. Fogler

A distant-neighbor quantum-mechanical method is used to study the nonlinear optical wave mixing in graphene nanoflakes (GNFs), including sum- and difference-frequency generation, as well as four-wave mixing. Our analysis shows that…

Optics · Physics 2022-03-11 Hanying Deng , Changming Huang , Yingji He , Fangwei Ye

Graphene is known to possess strong optical nonlinearity. Its nonlinear response can be further enhanced by graphene plasmons. Here, we report a novel nonlinear electro-absorption effect observed in nanostructured graphene due to excitation…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 D. Kundys , B. Van Duppen , O. P. Marshall , F. Rodriguez , I. Torre , A. Tomadin , M. Polini , A. N. Grigorenko

We present a theoretical framework for nonlinear optics of graphene and other 2D materials in layered structures. We derive a key equation to find the effective electric field and the sheet current density in the 2D material for given…

Optics · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , N. Vermeulen , C. Guo

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

Nonlinear light-matter interactions are typically enhanced by increasing the local field and its interaction time with matter. Conventional methods to achieve these goals are based on resonances or slow-light effects. However, these methods…

The optical nonlinear effects can provide different advanced electromagnetic functionalities, such as wave mixing and phase conjugation, which can be applied in a variety of new applications. However, these effects usually suffer from…

Optics · Physics 2020-06-29 Boyuan Jin , Christos Argyropoulos

Nonlinear optical processes rely on the intrinsically weak interactions between photons enabled by their coupling with matter. Unfortunately, many applications in nonlinear optics are severely hindered by the small response of conventional…

Materials Science · Physics 2014-12-15 Joel D. Cox , F. J. Garcia de Abajo

Graphene has emerged as a promising platform to bring nonlinear quantum optics to the nanoscale, where a large intrinsic optical nonlinearity enables long-lived and actively tunable plasmon polaritons to strongly interact. Here we…

Second-order nonlinear optical processes are used to convert light from one wavelength to another and to generate quantum entanglement. Creating chip-scale devices to more efficiently realize and control these interactions greatly increases…

The ability of graphene to support long-lived, electrically tunable plasmons that interact strongly with light, combined with its highly nonlinear optical response, has generated great expectations for application of the atomically-thin…

Mesoscale and Nanoscale Physics · Physics 2017-04-12 Joel D. Cox , Iván Silveiro , F. Javier García de Abajo

Owing to its peculiar energy dispersion, the quantum capacitance property of graphene can be exploited in a two-dimensional layered capacitor configuration. Using graphene and boron nitride respectively as the electrodes and the insulating…

Quantum Physics · Physics 2017-05-19 Sina Khorasani , Akshay Koottandavida

We present the first experimental investigation of nonlinear optical properties of graphene flakes. We find that at near infrared frequencies a graphene monolayer exhibits a remarkably high third-order optical nonlinearity which is…

Materials Science · Physics 2011-01-13 E. Hendry , P. J. Hale , J. J. Moger , A. K. Savchenko , S. A. Mikhailov

Optomechanical systems provide a unique platform for observing quantum behavior of macroscopic objects. However, efforts towards realizing nonlinear behavior at the single photon level have been inhibited by the small size of the radiation…

Quantum Physics · Physics 2015-01-14 Xunnong Xu , Michael Gullans , Jacob M. Taylor

A non-perturbative model for graphene optical nonlinearity is developed for the study of ultrafast pulse propagation along a monolayer, as in the case of graphene-comprising nanophotonic integrated waveguides. This graphene `hot electron'…

Optics · Physics 2022-03-18 Alexandros Pitilakis , Emmanouil E. Kriezis

We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…

Materials Science · Physics 2017-01-25 Habib Rostami , Mikhail I. Katsnelson , Marco Polini

The observation and electrical manipulation of infrared surface plasmons in graphene have triggered a search for similar photonic capabilities in other atomically thin materials that enable electrical modulation of light at visible and…

Mesoscale and Nanoscale Physics · Physics 2017-02-08 F. Javier Garcia de Abajo , Alejandro Manjavacas
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