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Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

Frustrated systems exhibit remarkable properties due to the high degeneracy of their ground states. Stabilised by competing interactions, a rich diversity of typically nanometre-sized phase structures appear in polymer and colloidal…

We report an investigation on structure and magnetic properties of the $S=3/2$ zigzag spin chain compound BaCoTe$_2$O$_7$. Neutron diffraction measurements reveal BaCoTe$_2$O$_7$ crystallizes in the noncentrosymmetric space group $Ama2$…

Strongly Correlated Electrons · Physics 2021-07-06 Lisi Li , Xunwu Hu , Zengjia Liu , Jia Yu , Benyuan Cheng , Sihao Deng , Lunhua He , Kun Cao , Dao-Xin Yao , Meng Wang

We present an extensive numerical study of a new type of frustrated itinerant magnetism on the pyrochlore lattice. In this theory, the pyrochlore magnet can be viewed as a cross-linking network of Kondo or double-exchange chains. Contrary…

Strongly Correlated Electrons · Physics 2018-12-17 Jing Luo , Gia-Wei Chern

We report on x-ray diffraction, magnetic susceptibility, electron- spin resonance and heat- capacity studies of Co[Al_1-xCo_x]_2O_4 for Co concentrations 0<x<1. In this spinel system only the A-site Co^2+ cation is magnetic, while the…

Materials Science · Physics 2009-11-13 N. Tristan , V. Zestrea , G. Behr , R. Klingeler , B. Buechner , H. A. Krug von Nidda , A. Loidl , V. Tsurkan

The structural and magnetic properties of the geometrically frustrated spin-$1/2$ capped-kagome antiferromagnet (RbCl)Cu$_{5}$P$_{2}$O$_{10}$ are investigated via temperature dependent x-ray diffraction, magnetization, heat capacity, and…

Materials Science · Physics 2023-09-25 S. Mohanty , J. Babu , Y. Furukawa , R. Nath

We have synthesized single crystals of Na_2IrO_3 and studied their structure, transport, magnetic, and thermal properties using powder x-ray diffraction (PXRD), electrical resistivity, isothermal magnetization M versus magnetic field H,…

Strongly Correlated Electrons · Physics 2010-06-03 Yogesh Singh , P. Gegenwart

We study the magnetic properties of CaFeTi$_2$O$_6$ (CFTO) by high-field magnetization and specific heat measurements. While the magnetic susceptibility data yield a vanishingly small Curie-Weiss temperature, the magnetic moments are not…

Strongly Correlated Electrons · Physics 2021-05-11 Di Liu , Si Wu , Xuanyu Long , Yao Wang , Hai-Feng Li , Ming Yang , Junfeng Wang , Zheng Liu , Xiang Li , Yuan Wan , Shiliang Li

Crystal structure, electronic structure, and magnetic behavior of the spin-1/2 quantum magnet Na1.5VOPO4F0.5 are reported. The disorder of Na atoms leads to a sequence of structural phase transitions revealed by synchrotron x-ray powder…

A frustrated system is one whose symmetry precludes the possibility that every pairwise interaction (``bond'') in the system can be satisfied at the same time. Such systems are common in all areas of physical and biological science. In the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Steven T. Bramwell , Michel J. -P. Gingras

We have investigated the magnetic, dielectric and magnetodielectric (MDE) behavior of a geometrically frustrated spin-chain system, Ca3Co1.4Rh0.6O6, in the single crystalline form for different orientations. The results bring out that the…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kartik K. Iyer , Kiran Singh , K. Mukherjee , P. L. Paulose , E. V. Sampathkumaran

In an ideal classical pyrochlore antiferromagnet without perturbations, an infinite degeneracy at a ground state leads to absence of a magnetic order and spin-glass transition. Here we present Na$_3$Mn(CO$_3$)$_2$Cl as a new candidate…

Strongly Correlated Electrons · Physics 2018-10-19 Kazuhiro Nawa , Daisuke Okuyama , Maxim Avdeev , Hiroyuki Nojiri , Masahiro Yoshida , Daichi Ueta , Hideki Yoshizawa , Taku J. Sato

Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…

Strongly Correlated Electrons · Physics 2022-04-20 Sheetal , A. Elghandour , R. Klingeler , C. S. Yadav

Magnetization measurements and time-of-flight neutron powder-diffraction studies on the high-temperature (300--980 K) magnetism and crystal structure (321--1200 K) of a pulverized YCrO$_3$ single crystal have been performed.…

Strongly Correlated Electrons · Physics 2021-11-04 Yinghao Zhu , Si Wu , Bao Tu , Shangjian Jin , Ashfia Huq , Joerg Persson , Haoshi Gao , Defang Ouyang , Zhubing He , Dao-Xin Yao , Zikang Tang , Hai-Feng Li

Frustrated magnets provide a platform for exploring exotic phases beyond conventional ordering, with potential relevance to functional materials and information technologies. In this work, we use Monte Carlo simulations to map the…

Strongly Correlated Electrons · Physics 2025-12-16 Prakash Timsina , Andres Chappa , Deema Alyones , Igor Vasiliev , Ludi Miao

We report the synthesis of fine particles of a well-known geometrically frustrated spin-chain compound Ca3Co2O6 through a new route, namely, a pyrophoric method employing triathanolamine (TEA) and studied the magnetic behavior of such…

Strongly Correlated Electrons · Physics 2010-01-28 K. Mukherjee , E. V. Sampathkumaran

We report a random singlet ground state in the $S=\frac{1}{2}$ Heisenberg pyrochlore antiferromagnet NaCdCu$_2$F$_7$. Cationic Na$^+$/Cd$^{2+}$ disorder on the pyrochlore $A$ site generates a broad distribution of…

A new pyrochlore compound, NaCaNi$_2$F$_7$, was recently synthesized and has a single magnetic site with spin-1 Ni$^{2+}$. We present zero field (ZF) and longitudinal field (LF) muon spin rotation ($\mu$SR) measurements on this pyrochlore.…

Strongly Correlated Electrons · Physics 2018-09-26 Y. Cai , M. N. Wilson , A. M. Hallas , L. Liu , B. A. Frandsen , S. R. Dunsiger , J. W. Krizan , R. J. Cava , Y. J. Uemura , O. Rubel , G. M. Luke

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals