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We theoretically investigate an exciton transfer process in a donor domain of organic photovoltaic cells focusing on the roles of local and nonlocal electron-phonon interactions. Our model consists of a three-level system described by the…

Materials Science · Physics 2021-01-25 Mauro Cainelli , Yoshitaka Tanimura

The interplay between coherence and system-environment interactions is at the basis of a wide range of phenomena, from quantum information processing to charge and energy transfer in molecular systems, biomolecules, and photochemical…

Quantum Physics · Physics 2025-11-30 Diego Fallas Padilla , Visal So , Abhishek Menon , Roman Zhuravel , Han Pu , Guido Pagano

An asymptotic scaling theory is presented using the conceptual basis of trapping-free subspace (i.e., orthogonal subspace) to establish the generic mechanism of optimal efficiency of excitation energy transfer (EET) in light-harvesting…

Quantum Physics · Physics 2013-05-16 Jianlan Wu , Jianshu Cao , Robert J. Silbey

We introduce a classical potentiostatic feedback mechanism that attenuates the dissipation in a quantum system arising from coupling to the surrounding thermodynamic bath, preserving the inter-state interference in an electronic excitation…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Chaitanya Gupta , Aldo Peña Perez , Sean Fischer , Stephen Weinreich , Boris Murmann , Roger T. Howe

We review the latest progress in understanding the fundamental noise properties of a coherent single electron emitter known as the mesoscopic capacitor. The system consists of a sub-micron cavity connected to a two-dimensional electron gas…

Mesoscale and Nanoscale Physics · Physics 2011-02-14 Mathias Albert , Christian Flindt , Markus Büttiker

We investigate electron transfer processes in donor-acceptor systems with a coupling of the electronic degrees of freedom to a common bosonic bath. The model allows to study many-particle effects and the influence of the local Coulomb…

Strongly Correlated Electrons · Physics 2007-05-23 Sabine Tornow , Ning-Hua Tong , Ralf Bulla

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

Quantum Physics · Physics 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

Selectivity filter is a gate in ion channels which are responsible for the selection and fast conduction of particular ions across the membrane (with high throughput rates of $10^8$ ions/sec and a high 1:$10^4$ discrimination rate between…

Biological Physics · Physics 2018-09-24 Amir Jalalinejad , Hassan Bassereh , Vahid Salari , Tapio Ala-Nissila , Achille Giacometti

The role of noise in the transport properties of quantum excitations is a topic of great importance in many fields, from organic semiconductors for technological applications to light-harvesting complexes in photosynthesis. In this paper we…

Quantum Physics · Physics 2016-11-22 Stefano Iubini , Octavi Boada , Yasser Omar , Francesco Piazza

Using large-scale, real-time quantum dynamics calculations, we present a detailed analysis of electronic excitation transfer (EET) mechanisms in a multi-particle plasmonic nanoantenna system. Specifically, we utilize real-time,…

Mesoscale and Nanoscale Physics · Physics 2018-03-06 Niranjan V. Ilawe , M. Belén Oviedo , Bryan M. Wong

In this paper, we study the role of collective vibrational motion in the phenomenon of electronic energy transfer (EET) along a chain of coupled electronic dipoles with varying excitation frequencies. Previous experimental work on EET in…

Quantum Physics · Physics 2015-03-13 F. L. Semião , K. Furuya , G. J. Milburn

Excitation energy transfer (EET) is one of the most important processes in both natural and artificial chemical systems including, for example, photosynthetic complexes and organic solar cells. The EET rate, however, is strongly suppressed…

Chemical Physics · Physics 2018-02-27 Nguyen Thanh Phuc , Akihito Ishizaki

A generic and intuitive model for coherent energy transport in multiple minima systems coupled to a quantum mechanical bath is shown. Using a simple spin-boson system, we illustrate how a generic donor-acceptor system can be brought into…

Biological Physics · Physics 2014-06-24 Tristan Farrow , Vlatko Vedral

In this paper, we investigate the effect of noise and disorder on the efficiency of excitation energy transfer (EET) in a $N=5$ sites linear chain with "static" dipole-dipole couplings. In fact, here, the disordered chain is a toy model for…

Disordered Systems and Neural Networks · Physics 2014-12-25 Hassan Bassereh , Vahid Salari , Farhad Shahbazi

Dielectric constant and absorption measurements on boron doped silicon samples show that transitions between the acceptor energy levels can be induced by an applied resonant ac electric field and the Stark tuning of level spacing with an…

Quantum Physics · Physics 2015-05-20 Y. P. Song , B. Golding

A theory of electrical transport through molecular wires is used to estimate the electronic factor in the intramolecular electron transfer (ET) in porphyrin-nitrobenzene supermolecules, and to analyze its structure. The chosen molecules…

Soft Condensed Matter · Physics 2007-05-23 Natalya Zimbovskaya , Godfrey Gumbs

Quantum simulation offers a route to study open-system molecular dynamics in non-perturbative regimes by programming the interactions among electronic, vibrational, and environmental degrees of freedom on similar energy scales. Trapped-ion…

We study cooperative effects in energy transfer (ET) from an ensemble of donors to an acceptor near a plasmonic nanostructure. We demonstrate that in cooperative regime ET takes place from plasmonic superradiant and subradiant states rather…

Mesoscale and Nanoscale Physics · Physics 2019-04-15 Vitaliy N. Pustovit , Augustine M. Urbas , Tigran V. Shahbazyan

Resonant energy transfer mechanisms have been observed in the sensitized luminescence of solids, in quantum dots and in molecular nanostructures, and they also play a central role in light harvesting processes in photosynthetic organisms.…

Quantum Physics · Physics 2009-11-07 Brendon Lovett , John H. Reina , Ahsan Nazir , Beeneet Kothari , Andrew Briggs

A collective electron transfer (ET) process was discovered by studying the current noise in a field effect transistor with light-sensitive gate formed by nanocrystals linked by organic molecules to its surface. Fluctuations in the ET…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Y. Paltiel , G. Jung , T. Aqua , D. Mocatta , U. Banin , R. Naaman