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The response of a model micro-electrochemical system to a time-dependent applied voltage is analyzed. The article begins with a fresh historical review including electrochemistry, colloidal science, and microfluidics. The model problem…

Soft Condensed Matter · Physics 2009-11-10 Martin Z. Bazant , Katsuyo Thornton , Armand Ajdari

Three models for nonlocal electron thermal transport are here compared against Vlasov-Fokker-Planck (VFP) codes to assess their accuracy in situations relevant to both inertial fusion hohlraums and tokamak scrape-off layers. The models…

The DFN (Doyle-Fuller-Newman) model is well know for being accurate and computationally expensive. In situations where temperature gradients are important (eg fast charging) it is desirable to couple the temperature dynamics within a…

Chemical Physics · Physics 2022-08-11 Matthew Hunt , Florian Theil , Ferran Brosa Planella , W. Dhammika Widanage

A Poisson-Nernst-Planck-Fermi (PNPF) theory is developed for studying ionic transport through biological ion channels. Our goal is to deal with the finite size of particle using a Fermi like distribution without calculating the forces…

Biological Physics · Physics 2015-06-23 Jinn-Liang Liu , Bob Eisenberg

A Fokker-Planck model for the interaction of fast ions with the thermal electrons in a quasi-neutral plasma is developed. When the fast ion population has a net flux (i.e. the distribution of the fast ions is anisotropic in velocity space)…

Plasma Physics · Physics 2020-01-08 Brian Appelbe , Mark Sherlock , Omar El-Amiri , Chris Walsh , Jeremy Chittenden

We present and analyze two mathematical models for the self consistent quantum transport of electrons in a graphene layer. We treat two situations. First, when the particles can move in all the plane $\RR^2$, the model takes the form of a…

Analysis of PDEs · Mathematics 2013-10-28 Raymond El Hajj , Florian Méhats

Room temperature ionic liquids are attractive to numerous applications and particularly, to renewable energy devices. As solvent free electrolytes, they demonstrate a paramount connection between the material morphology and Coulombic…

Chemical Physics · Physics 2016-03-15 Nir Gavish , Arik Yochelis

Three analytic results are proposed for a linear form of the modified Poisson-Boltzmann equation in the theory of bulk electrolytes. Comparison is also made with the mean spherical approximation results. The linear theories predict a…

Statistical Mechanics · Physics 2019-06-28 C. W. Outhwaite , L. B. Bhuiyan

Electrostatic correlation effects in inhomogeneous symmetric electrolytes are investigated within a previously developed electrostatic self-consistent (SC) theory (R.R. Netz and H. Orland, Eur. Phys.J. E 11, 301 (2003)). To this aim, we…

Soft Condensed Matter · Physics 2015-06-05 Sahin Buyukdagli , Cristian Achim , Tapio Ala-Nissila

In this work, we have computed electrical conductivities at ambient conditions of aqueous NaCl and KCl solutions by using the Einstein-Helfand equation. Common force fields (charge q = 1 e) do not reproduce the experimental values of…

Chemical Physics · Physics 2024-01-25 S. Blazquez , J. L. F. Abascal , J. Lagerweij , P. Habibi , P. Dey , T. J. H. Vlugt , O. A. Moultos , C. Vega

In this paper, we design, analyze, and numerically validate positive and energy-dissipating schemes for solving the time-dependent multi-dimensional system of Poisson-Nernst-Planck (PNP) equations, which has found much use in the modeling…

Numerical Analysis · Mathematics 2020-02-24 Hailiang Liu , Wumaier Maimaitiyiming

Thermodynamic quantities of Coulomb plasmas consisting of point-like ions immersed in a compressible, polarizable electron background are calculated for ion charges Z=1 to 26 and for a wide domain of plasma parameters ranging from the…

Plasma Physics · Physics 2016-09-08 G. Chabrier , A. Y. Potekhin

We study the electro-diffusion properties of a domain containing a cusp-shaped structure in three dimensions when one ionic specie is dominant. The mathematical problem consists in solving the steady-state Poisson-Nernst-Planck (PNP)…

Neurons and Cognition · Quantitative Biology 2017-10-09 J. Cartailler , D. Holcman

The transport approach is a useful tool to study dynamics of non-equilibrium systems. For heavy-ion collisions at intermediate energies, where both the smooth nucleon potential and the hard-core nucleon-nucleon collision are important, the…

Nuclear Theory · Physics 2019-04-02 Jun Xu

The optical properties of molecules close to plasmonic nanostructures greatly differ from their isolated molecule counterparts. To theoretically investigate such systems in a Quantum Chemistry perspective, one has to take into account that…

Mesoscale and Nanoscale Physics · Physics 2016-12-26 Silvio Pipolo , Stefano Corni

We consider numerical methods for the Poisson-Nernst-Planck-Cahn-Hilliard (PNPCH) equations with steric interactions. We propose a novel energy stable numerical scheme that respects mass conservation and positivity at the discrete level.…

Numerical Analysis · Mathematics 2021-02-03 Yiran Qian , Cheng Wang , Shenggao Zhou

The model reduction of a mesoscopic kinetic dynamics to a macroscopic continuum dynamics has been one of the fundamental questions in mathematical physics since Hilbert's time. In this paper, we consider a diagram of the diffusion limit…

Numerical Analysis · Mathematics 2020-09-29 Jae Yong Lee , Jin Woo Jang , Hyung Ju Hwang

We consider the singular electron-electron interaction corrections to the transport coefficients in disordered metals to test the validity of the Wiedemann-Franz law. We develop a local, quantum kinetic equation approach in which the charge…

Disordered Systems and Neural Networks · Physics 2008-09-25 G. Catelani , I. L. Aleiner

The equilibrium density profiles in a classical multicomponent plasma near a hard wall made with a dielectric material characterized by a relative dielectric constant $\ew$ are studied from the first Born-Green-Yvon equation combined with…

Statistical Mechanics · Physics 2007-05-23 Jean-Noel Aqua , Francoise Cornu

In this paper, based on geometric singular perturbation analysis of a quasi-one dimensional Poisson-Nernst-Planck model for ionic flows, we study the problem of zero current condition for ionic flows through membrane channels with a simple…

Dynamical Systems · Mathematics 2020-09-22 Hamid Mofidi , Weishi Liu