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Related papers: H2+ and HD+: candidates for a molecular clock

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We identify laser-accessible transitions in group 16-like highly charged ions as candidates for high-accuracy optical clocks, including S-, Se-, and Te-like systems. For this class of ions, the ground $^{3}P_{J}$ fine structure manifold…

Atomic Physics · Physics 2022-10-06 Saleh O. Allehabi , S. M. Brewer , V. A. Dzuba , V. V. Flambaum , K. Beloy

Accurate $EF{}^1\Sigma^+_g-X{}^1\Sigma^+_g$ transition energies in molecular hydrogen were determined for transitions originating from levels with highly-excited vibrational quantum number, $v=11$, in the ground electronic state.…

Atomic Physics · Physics 2016-09-23 T. Madhu Trivikram , M. L. Niu , P. Wcisło , W. Ubachs , E. J. Salumbides

The hyperfine structure of the S1/2-D5/2 quadrupole transition at 729 nm in 43Ca+ has been investigated by laser spectroscopy using a single trapped 43Ca+ ion. We determine the hyperfine structure constants of the metastable level as…

Atomic Physics · Physics 2015-06-26 J. Benhelm , G. Kirchmair , U. Rapol , T. Koerber , C. F. Roos , R. Blatt

We propose here a few selective highly charged ions (HCIs), namely Ni$^{12+}$ and Cu$^{13+}$, Pd$^{12+}$ and Ag$^{13+}$, that not only promise to be very high accurate optical clocks below $10^{-19}$ uncertainties, but also offer quality…

Atomic Physics · Physics 2018-04-25 Yan-mei Yu , B. K. Sahoo

Recent theoretical works have proposed atomic clocks based on narrow optical transitions in highly charged ions. The most interesting candidates for searches of new physics are those which occur at rare orbital crossings where the shell…

We calculate the DC Stark effect for three molecular hydrogen ions in the non-relativistic approximation. The effect is calculated both in dependence on the rovibrational state and in dependence on the hyperfine state. We discuss special…

Atomic Physics · Physics 2015-06-19 Stephan Schiller , Dimitar Bakalov , Ashat K. Bekbaev , Vladimir I. Korobov

Highly charged ions (HCIs) are insensitive to external perturbations and are attractive for the development of ultrastable clocks. However, only a few HCI candidates are known to provide optical clock transitions. In this Letter, we show…

Atomic Physics · Physics 2025-01-07 Chunhai Lyu , Christoph H. Keitel , Zoltán Harman

The magnetic dipole transitions in the homonuclear molecular ion H$_2^+$ are obtained for a wide range of $v$ and $L$, vibrational and total orbital momentum quantum numbers, respectively. Calculations are performed in the nonrelativistic…

Atomic Physics · Physics 2023-11-09 D. T. Aznabayev , A. K. Bekbaev , V. I. Korobov

Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider…

Atomic Physics · Physics 2015-06-11 V. A. Dzuba , A. Derevianko , V. V. Flambaum

Ionic clocks exhibit as the most promising candidates for the frequency standards. Recent investigations show the profound advantages of interrogating two laser beams with different frequencies in developing the frequency standards. Here we…

Atomic Physics · Physics 2021-12-07 Arghya Das , Anal Bhowmik , Narendra Nath Dutta , Sonjoy Majumder

Astrophysical molecular spectroscopy is an important method of searching for new physics through probing the variation of the proton-to-electron mass ratio, $\mu$, with existing constraints limiting variation to a fractional change of less…

Chemical Physics · Physics 2020-08-26 Anna-Maree Syme , Adam Mousley , Maria Cunningham , Laura K McKemmish

A procedure is described for the precise nonrelativistic evaluation of the dipole polarizabilities of H_2^+ and D_2^+ that avoids any approximation based on the size of the electron mass relative to the nucleus mass. The procedure is…

Atomic Physics · Physics 2007-05-23 J. M. Taylor , A. Dalgarno , J. F. Babb

Molecular hydrogen absorption in the damped Lyman-alpha system at z = 2.34 towards quasar Q1232+082 is analyzed in order to derive a constraint on a possible temporal variation of the proton-to-electron mass ratio, mu, over cosmological…

Cosmology and Nongalactic Astrophysics · Physics 2017-01-11 M. Daprà , M. van der Laan , M. T. Murphy , W. Ubachs

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

Atomic Physics · Physics 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb

In this work, the $4D_{3/2}|3,\pm2\rangle \rightarrow 4D_{5/2}|3,\pm2\rangle$ transition in the Nb$^{4+}$ ion is identified as a promising candidate for a terahertz (THz) atomic clock, with the transition frequency occurring at 56.0224 THz.…

Atomic Physics · Physics 2025-04-23 Jyoti , A. Chakraborty , Zhiyang Wang , Jia Zhang , Jingbiao Chen , Bindiya Arora , B. K. Sahoo

Absorption lines of H$_2$ and HD molecules observed at high redshift in the line of sight towards quasars are a test ground to search for variation of the proton-to-electron mass ratio $\mu$. For this purpose, results from astronomical…

Cosmology and Nongalactic Astrophysics · Physics 2019-02-13 W. Ubachs , E. J. Salumbides , M. T. Murphy , H. Abgrall , E. Roueff

We report results of a theoretical investigation of hyperfine interactions in two homonuclear isotopologues of the hydrogen molecule: H$_{2}$ and D$_{2}$. We present a set of hyperfine coupling constants: spin-rotation, spin-spin dipole…

Atomic Physics · Physics 2020-07-06 Hubert Jóźwiak , Hubert Cybulski , Piotr Wcisło

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We calculate ionization energies and fundamental vibrational transitions for H$_2^+$, D$_2^+$, and HD$^+$ molecular ions. The NRQED expansion for the energy in terms of the fine structure constant $\alpha$ is used. Previous calculations of…

Atomic Physics · Physics 2017-06-14 Vladimir I. Korobov , Laurent Hilico , Jean-Philippe Karr

Iridium ions near $4f$-$5s$ level crossings are the leading candidates for a new type of atomic clocks with a high projected accuracy and a very high sensitivity to the temporal variation of the fine structure constant $\alpha$. To identify…

Atomic Physics · Physics 2015-08-12 U. I. Safronova , V. V. Flambaum , M. S. Safronova