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Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A…

Condensed Matter · Physics 2009-01-23 Daniel Loss , David P. DiVincenzo , G. Grinstein

We have studied quantum tunneling of large spins in a biaxial spin system and in a single-axial spin system with a transverse magnetic field. The asymptotically exact eigenvalues and eigenstates of the spin systems are obtained by solving…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Bambi Hu , De-gang Zhang , Bo-zang Li

We study the model of a biaxial single ferromagnetic spin Hamiltonian with an external magnetic field applied along the medium axis. The phase transition of the escape rate is investigated. Two different but equivalent methods are…

Mesoscale and Nanoscale Physics · Physics 2014-03-19 S. A. Owerre , M. B. Paranjape

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , N. E. Chakov , G. Christou

Macroscopic quantum tunneling of the phase is a fundamental phenomenon in the quantum dynamics of superconducting nanocircuits. The tunneling rate can be controlled in such circuits, where the potential landscape for the phase can be tuned…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 Nicolas Didier , Frank W. J. Hekking

The oscillation of tunnel splitting in the biaxial spin system within magnetic field along the anisotropy axis is analyzed within the particle mapping approach, rather than in the (\theta-\phi) spin coherent-state representation. In our…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Sahng-Kyoon Yoo , Soo-Young Lee , Dal-Ho Yoon , Chang-Soo Park

We have investigated the escape rate of the nanospin particle with a magnetic field applied along the easy axis. The model studied here is described by the Hamiltonian $\hat{\cal H} = K_1 \hat{S}_z^2 + K_2 \hat{S}_y^2 + g\mu_b H \hat{S}_x…

Condensed Matter · Physics 2007-05-23 Chang Soo Park , Sahng-Kyoon Yoo , D. K. Park , Dal-Ho Yoon

The tunneling decay event of a metastable state in a fully connected quantum spin model can be simulated efficiently by path integral quantum Monte Carlo (QMC) [Isakov $et~al.$, Phys. Rev. Lett. ${\bf 117}$, 180402 (2016).]. This is because…

Quantum Physics · Physics 2017-11-01 Zhang Jiang , Vadim N. Smelyanskiy , Sergio Boixo , Hartmut Neven

In this work, we propose a path integral-inspired formalism for computing the quantum thermal expectation values of spin systems, when subject to magnetic fields that can be time-dependent and can accommodate the presence of Heisenberg…

Quantum Physics · Physics 2025-06-18 Thomas Nussle , Stam Nicolis , Iason Sofos , Joseph Barker

The quantum-classical transitions of the escape rates in a uniaxial spin model relevant to the molecular magnet Mn$_{12}$Ac and a biaxial anisotropic ferromagnetic particle are investigated by applying the periodic instanton method. The…

Soft Condensed Matter · Physics 2009-10-31 Y. -B. Zhang , Y. -H. Nie , S. -P. Kou , J. -Q. Liang , H. J. W. Mueller-Kirsten , F. -C. Pu

In high spin molecules metal ions are coupled by ferro or antiferromagnetic short range interactions so that their magnetic moments are parallel or antiparallel to each other at temperatures (T) much smaller than the coupling constant J.…

Condensed Matter · Physics 2009-09-25 A. Keren , P. Mendels , A. Kratzer , A. Scuiller , M. Verdaguer , Z. Slaman , C. Baines

The escape rate \Gamma of the large-spin model described by the Hamiltonian H = -DS_z^2 - H_zS_z - H_xS_x is investigated with the help of the mapping onto a particle moving in a double-well potential U(x). The transition-state method…

Statistical Mechanics · Physics 2009-10-31 D. A. Garanin , X. Martinez Hidalgo , E. M. Chudnovsky

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

The theory for the quantum tunneling of nano-magnets is developed within the intermediate spin framework. Periodic magnetic effects are seen to reflect that associated with a change of flux by a single flux quantum $\Phi_{0}$. Essential are…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. E. Barnes

We investigate the escape rate of a biaxial spin particle with an arbitrarily dierected magnetic field in the easy plane, described by Hamiltonian ${\cal H} = -AS_z^2 - BS_x^2 -H_x S_x -H_z S_z, (A>B>0)$. We derive an effective particle…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Chang-Soo Park , Sahng-Kyoon Yoo , Dal-Ho Yoon

We have studied numerically the quantum-classical crossover in the escape-rate for an uniaxial spin system with an arbitrarily directed field. Using the simple quantum transition-state theory, we have obtained the boundary separating the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Gwang-Hee Kim , E. M. Chudnovsky

The quantum tunneling of the magnetization vector are studied theoretically in single-domain ferromagnetic nanoparticles placed in an external magnetic field at an arbitrarily directed angle in the $ZX$ plane. We consider the…

Statistical Mechanics · Physics 2009-10-31 Rong Lu , Jia-Lin Zhu , Zhi-Rong Liu , Lee Chang , Bing-Lin Gu

Transitions from classical to quantum behaviour in a spin system with two degenerate ground states separated by twin energy barriers which are asymmetric due to an applied magnetic field are investigated. It is shown that these transitions…

Condensed Matter · Physics 2009-10-31 S. -Y. Lee , H. J. W. Mueller-Kirsten , D. K. Park , F. Zimmerschied

A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 D. Galetti , B. M. Pimentel , C. L. Lima , E. C. Silva

Inspired by path integral molecular dynamics, we build a spin model, in terms of spin coherent states, from which we can compute the quantum expectation values of a spin in a constant magnetic field, at finite temperature. This formulation…

Materials Science · Physics 2023-11-02 Thomas Nussle , Stam Nicolis , Joseph Barker
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